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Long-lived spin waves in a metallic antiferromagnet

Collective spin excitations in magnetically ordered crystals, called magnons or spin waves, can serve as carriers in novel spintronic devices with ultralow energy consumption. The generation of well-detectable spin flows requires long lifetimes of high-frequency magnons. In general, the lifetime of...

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Autores principales: Poelchen, G., Hellwig, J., Peters, M., Usachov, D. Yu., Kliemt, K., Laubschat, C., Echenique, P. M., Chulkov, E. V., Krellner, C., Parkin, S. S. P., Vyalikh, D. V., Ernst, A., Kummer, K.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10480465/
https://www.ncbi.nlm.nih.gov/pubmed/37669952
http://dx.doi.org/10.1038/s41467-023-40963-x
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author Poelchen, G.
Hellwig, J.
Peters, M.
Usachov, D. Yu.
Kliemt, K.
Laubschat, C.
Echenique, P. M.
Chulkov, E. V.
Krellner, C.
Parkin, S. S. P.
Vyalikh, D. V.
Ernst, A.
Kummer, K.
author_facet Poelchen, G.
Hellwig, J.
Peters, M.
Usachov, D. Yu.
Kliemt, K.
Laubschat, C.
Echenique, P. M.
Chulkov, E. V.
Krellner, C.
Parkin, S. S. P.
Vyalikh, D. V.
Ernst, A.
Kummer, K.
author_sort Poelchen, G.
collection PubMed
description Collective spin excitations in magnetically ordered crystals, called magnons or spin waves, can serve as carriers in novel spintronic devices with ultralow energy consumption. The generation of well-detectable spin flows requires long lifetimes of high-frequency magnons. In general, the lifetime of spin waves in a metal is substantially reduced due to a strong coupling of magnons to the Stoner continuum. This makes metals unattractive for use as components for magnonic devices. Here, we present the metallic antiferromagnet CeCo(2)P(2), which exhibits long-living magnons even in the terahertz (THz) regime. For CeCo(2)P(2), our first-principle calculations predict a suppression of low-energy spin-flip Stoner excitations, which is verified by resonant inelastic X-ray scattering measurements. By comparison to the isostructural compound LaCo(2)P(2), we show how small structural changes can dramatically alter the electronic structure around the Fermi level leading to the classical picture of the strongly damped magnons intrinsic to metallic systems. Our results not only demonstrate that long-lived magnons in the THz regime can exist in bulk metallic systems, but they also open a path for an efficient search for metallic magnetic systems in which undamped THz magnons can be excited.
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spelling pubmed-104804652023-09-07 Long-lived spin waves in a metallic antiferromagnet Poelchen, G. Hellwig, J. Peters, M. Usachov, D. Yu. Kliemt, K. Laubschat, C. Echenique, P. M. Chulkov, E. V. Krellner, C. Parkin, S. S. P. Vyalikh, D. V. Ernst, A. Kummer, K. Nat Commun Article Collective spin excitations in magnetically ordered crystals, called magnons or spin waves, can serve as carriers in novel spintronic devices with ultralow energy consumption. The generation of well-detectable spin flows requires long lifetimes of high-frequency magnons. In general, the lifetime of spin waves in a metal is substantially reduced due to a strong coupling of magnons to the Stoner continuum. This makes metals unattractive for use as components for magnonic devices. Here, we present the metallic antiferromagnet CeCo(2)P(2), which exhibits long-living magnons even in the terahertz (THz) regime. For CeCo(2)P(2), our first-principle calculations predict a suppression of low-energy spin-flip Stoner excitations, which is verified by resonant inelastic X-ray scattering measurements. By comparison to the isostructural compound LaCo(2)P(2), we show how small structural changes can dramatically alter the electronic structure around the Fermi level leading to the classical picture of the strongly damped magnons intrinsic to metallic systems. Our results not only demonstrate that long-lived magnons in the THz regime can exist in bulk metallic systems, but they also open a path for an efficient search for metallic magnetic systems in which undamped THz magnons can be excited. Nature Publishing Group UK 2023-09-05 /pmc/articles/PMC10480465/ /pubmed/37669952 http://dx.doi.org/10.1038/s41467-023-40963-x Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Poelchen, G.
Hellwig, J.
Peters, M.
Usachov, D. Yu.
Kliemt, K.
Laubschat, C.
Echenique, P. M.
Chulkov, E. V.
Krellner, C.
Parkin, S. S. P.
Vyalikh, D. V.
Ernst, A.
Kummer, K.
Long-lived spin waves in a metallic antiferromagnet
title Long-lived spin waves in a metallic antiferromagnet
title_full Long-lived spin waves in a metallic antiferromagnet
title_fullStr Long-lived spin waves in a metallic antiferromagnet
title_full_unstemmed Long-lived spin waves in a metallic antiferromagnet
title_short Long-lived spin waves in a metallic antiferromagnet
title_sort long-lived spin waves in a metallic antiferromagnet
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10480465/
https://www.ncbi.nlm.nih.gov/pubmed/37669952
http://dx.doi.org/10.1038/s41467-023-40963-x
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