A light-driven selective protocol for on-demand methanol and formic acid syntheses with a recyclable GaN catalyst

Herein, we present a protocol for the on-demand preparation of methanol and formic acid via selective photo-oxidation of methane with H(2)O and O(2) catalyzed by GaN. The detailed photosyntheses of methanol or formic acid from CH(4)/H(2)O or CH(4)/H(2)O/O(2) are described, respectively. In addition,...

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Detalles Bibliográficos
Autores principales: Han, Jing-Tan, Su, Hui, Tan, Lida, Li, Chao-Jun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Elsevier 2023
Materias:
Protocol
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10495642/
https://www.ncbi.nlm.nih.gov/pubmed/37656629
http://dx.doi.org/10.1016/j.xpro.2023.102530
Descripción
Sumario:Herein, we present a protocol for the on-demand preparation of methanol and formic acid via selective photo-oxidation of methane with H(2)O and O(2) catalyzed by GaN. The detailed photosyntheses of methanol or formic acid from CH(4)/H(2)O or CH(4)/H(2)O/O(2) are described, respectively. In addition, we provide experimental details for the accurate quantifications of the final gas/liquid products and photoexcited oxygenated radicals. Finally, we deliver the procedure for scaling up the transformation. For complete details on the use and execution of this protocol, please refer to Han et al. (2023).(1)

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