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Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application

[Image: see text] Despite the high sensitivity and selectivity, the high operating temperature required for activation energy of tin oxide (SnO(2)) still stands as a drawback for SnO(2) based gas sensors. In this work, the SnO(2) thin films were deposited through spray pyrolysis and were subjected t...

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Autores principales: Thomas, Anju, Thirumalaisamy, Logu, Madanagurusamy, Sridharan, Sivaperuman, Kalainathan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10500894/
https://www.ncbi.nlm.nih.gov/pubmed/37720763
http://dx.doi.org/10.1021/acsomega.3c04038
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author Thomas, Anju
Thirumalaisamy, Logu
Madanagurusamy, Sridharan
Sivaperuman, Kalainathan
author_facet Thomas, Anju
Thirumalaisamy, Logu
Madanagurusamy, Sridharan
Sivaperuman, Kalainathan
author_sort Thomas, Anju
collection PubMed
description [Image: see text] Despite the high sensitivity and selectivity, the high operating temperature required for activation energy of tin oxide (SnO(2)) still stands as a drawback for SnO(2) based gas sensors. In this work, the SnO(2) thin films were deposited through spray pyrolysis and were subjected to gas sensing at 27 °C (room temperature) towards different gases. The films exhibited a consistently low response of approximately 1 when tested to various VOCs. The type, concentration, and mobility of charge carriers were determined from the Hall measurements. The high carrier concentration accompanied by poor mobility and grain boundary scattering is supposed to hinder its performance at room temperature. The obtained film had spherical morphology, which lead to grain boundary scatterings and decreased the mobility of carriers.
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spelling pubmed-105008942023-09-15 Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application Thomas, Anju Thirumalaisamy, Logu Madanagurusamy, Sridharan Sivaperuman, Kalainathan ACS Omega [Image: see text] Despite the high sensitivity and selectivity, the high operating temperature required for activation energy of tin oxide (SnO(2)) still stands as a drawback for SnO(2) based gas sensors. In this work, the SnO(2) thin films were deposited through spray pyrolysis and were subjected to gas sensing at 27 °C (room temperature) towards different gases. The films exhibited a consistently low response of approximately 1 when tested to various VOCs. The type, concentration, and mobility of charge carriers were determined from the Hall measurements. The high carrier concentration accompanied by poor mobility and grain boundary scattering is supposed to hinder its performance at room temperature. The obtained film had spherical morphology, which lead to grain boundary scatterings and decreased the mobility of carriers. American Chemical Society 2023-08-30 /pmc/articles/PMC10500894/ /pubmed/37720763 http://dx.doi.org/10.1021/acsomega.3c04038 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Thomas, Anju
Thirumalaisamy, Logu
Madanagurusamy, Sridharan
Sivaperuman, Kalainathan
Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application
title Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application
title_full Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application
title_fullStr Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application
title_full_unstemmed Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application
title_short Incompatibility of Pure SnO(2) Thin Films for Room-Temperature Gas Sensing Application
title_sort incompatibility of pure sno(2) thin films for room-temperature gas sensing application
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10500894/
https://www.ncbi.nlm.nih.gov/pubmed/37720763
http://dx.doi.org/10.1021/acsomega.3c04038
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