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Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2)

[Image: see text] Engineering nontrivial spin textures in magnetic van der Waals materials is highly desirable for spintronic applications based on hybrid heterostructures. The recent observation of labyrinth and bubble domains in the near room-temperature ferromagnet Fe(5–x)GeTe(2) down to a bilaye...

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Autores principales: Högen, Michael, Fujita, Ryuji, Tan, Anthony K. C., Geim, Alexandra, Pitts, Michael, Li, Zhengxian, Guo, Yanfeng, Stefan, Lucio, Hesjedal, Thorsten, Atatüre, Mete
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10510720/
https://www.ncbi.nlm.nih.gov/pubmed/37642321
http://dx.doi.org/10.1021/acsnano.3c03825
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author Högen, Michael
Fujita, Ryuji
Tan, Anthony K. C.
Geim, Alexandra
Pitts, Michael
Li, Zhengxian
Guo, Yanfeng
Stefan, Lucio
Hesjedal, Thorsten
Atatüre, Mete
author_facet Högen, Michael
Fujita, Ryuji
Tan, Anthony K. C.
Geim, Alexandra
Pitts, Michael
Li, Zhengxian
Guo, Yanfeng
Stefan, Lucio
Hesjedal, Thorsten
Atatüre, Mete
author_sort Högen, Michael
collection PubMed
description [Image: see text] Engineering nontrivial spin textures in magnetic van der Waals materials is highly desirable for spintronic applications based on hybrid heterostructures. The recent observation of labyrinth and bubble domains in the near room-temperature ferromagnet Fe(5–x)GeTe(2) down to a bilayer thickness was thus a significant advancement toward van der Waals-based many-body physics. However, the physical mechanism responsible for stabilizing these domains remains unclear and requires further investigation. Here, we combine cryogenic scanning diamond quantum magnetometry and field reversal techniques to elucidate the high-field propagation and nucleation of bubble domains in trilayer Fe(5–x)GeTe(2). We provide evidence of pinning-induced nucleation of magnetic bubbles and further show an unexpectedly high layer-dependent coercive field. These measurements can be easily extended to a wide range of magnetic materials to provide valuable nanoscale insight into domain processes critical for spintronic applications.
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spelling pubmed-105107202023-09-21 Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2) Högen, Michael Fujita, Ryuji Tan, Anthony K. C. Geim, Alexandra Pitts, Michael Li, Zhengxian Guo, Yanfeng Stefan, Lucio Hesjedal, Thorsten Atatüre, Mete ACS Nano [Image: see text] Engineering nontrivial spin textures in magnetic van der Waals materials is highly desirable for spintronic applications based on hybrid heterostructures. The recent observation of labyrinth and bubble domains in the near room-temperature ferromagnet Fe(5–x)GeTe(2) down to a bilayer thickness was thus a significant advancement toward van der Waals-based many-body physics. However, the physical mechanism responsible for stabilizing these domains remains unclear and requires further investigation. Here, we combine cryogenic scanning diamond quantum magnetometry and field reversal techniques to elucidate the high-field propagation and nucleation of bubble domains in trilayer Fe(5–x)GeTe(2). We provide evidence of pinning-induced nucleation of magnetic bubbles and further show an unexpectedly high layer-dependent coercive field. These measurements can be easily extended to a wide range of magnetic materials to provide valuable nanoscale insight into domain processes critical for spintronic applications. American Chemical Society 2023-08-29 /pmc/articles/PMC10510720/ /pubmed/37642321 http://dx.doi.org/10.1021/acsnano.3c03825 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Högen, Michael
Fujita, Ryuji
Tan, Anthony K. C.
Geim, Alexandra
Pitts, Michael
Li, Zhengxian
Guo, Yanfeng
Stefan, Lucio
Hesjedal, Thorsten
Atatüre, Mete
Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2)
title Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2)
title_full Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2)
title_fullStr Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2)
title_full_unstemmed Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2)
title_short Imaging Nucleation and Propagation of Pinned Domains in Few-Layer Fe(5–x)GeTe(2)
title_sort imaging nucleation and propagation of pinned domains in few-layer fe(5–x)gete(2)
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10510720/
https://www.ncbi.nlm.nih.gov/pubmed/37642321
http://dx.doi.org/10.1021/acsnano.3c03825
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