Toward Sustainable Composites: Graphene‐Modified Jute Fiber Composites with Bio‐Based Epoxy Resin

Sustainable natural fiber reinforced composites have attracted significant interest due to the growing environmental concerns with conventional synthetic fiber as well as petroleum‐based resins. One promising approach to reducing the large carbon footprint of petroleum‐based resins is the use of bio‐based thermoset resins. However, current fiber‐reinforced bio‐based epoxy composites exhibit relatively lower mechanical properties such as tensile, flexural strength, and modulus, which limits their wider application. Here the fabrication of high‐performance composites using jute fibers is reported, modified with graphene nanoplates (GNP) and graphene oxide (GO), and reinforced with bio‐based epoxy resin. It is demonstrated that physical and chemical treatments of jute fibers significantly improve their fiber volume fraction (V(f) ) and matrix adhesion, leading to enhanced mechanical properties of the resulting Jute/Bio‐epoxy (J/BE) composites. Furthermore, the incorporation of GNP and GO further increases the tensile and flexural strength of the J/BE composites. The study reveals the potential of graphene‐based jute fiber‐reinforced composites with bio‐based epoxy resin as a sustainable and high‐performance material for a wide range of applications. This work contributes to the development of sustainable composites that have the potential to reduce the negative environmental impact of conventional materials while also offering improved mechanical properties.