Cargando…

Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface

We synthesized a CaZrO(3)/SrTiO(3) oxide heterostructure, which can serve as an alternative to LaAlO(3)/SrTiO(3), and confirmed the generation of 2-dimensional electron gas (2-DEG) at the heterointerface. We analyzed the electrical-transport properties of the 2-DEG to elucidate its intrinsic charact...

Descripción completa

Detalles Bibliográficos
Autores principales: Kwon, Duhyuk, Kwak, Yongsu, Lee, Doopyo, Jo, Wonkeun, Cho, Byeong-Gwan, Koo, Tae-Yeong, Song, Jonghyun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10517959/
https://www.ncbi.nlm.nih.gov/pubmed/37741927
http://dx.doi.org/10.1038/s41598-023-43247-y
_version_ 1785109409284751360
author Kwon, Duhyuk
Kwak, Yongsu
Lee, Doopyo
Jo, Wonkeun
Cho, Byeong-Gwan
Koo, Tae-Yeong
Song, Jonghyun
author_facet Kwon, Duhyuk
Kwak, Yongsu
Lee, Doopyo
Jo, Wonkeun
Cho, Byeong-Gwan
Koo, Tae-Yeong
Song, Jonghyun
author_sort Kwon, Duhyuk
collection PubMed
description We synthesized a CaZrO(3)/SrTiO(3) oxide heterostructure, which can serve as an alternative to LaAlO(3)/SrTiO(3), and confirmed the generation of 2-dimensional electron gas (2-DEG) at the heterointerface. We analyzed the electrical-transport properties of the 2-DEG to elucidate its intrinsic characteristics. Based on the magnetic field dependence of resistance at 2 K, which exhibited Weak Anti-localization (WAL) behaviors, the fitted Rashba parameter values were found to be about 12–15 × 10(–12) eV*m. These values are stronger than the previous reported Rashba parameters obtained from the 2-DEGs in other heterostructure systems and several layered 2D materials. The observed strong spin–orbit coupling (SOC) is attributed to the strong internal electric field generated by the lattice mismatch between the CaZrO(3) layer and SrTiO(3) substrate. This pioneering strong SOC of the 2-DEG at the CaZrO(3)/SrTiO(3) heterointerface may play a pivotal role in the developing future metal oxide-based quantum nanoelectronics devices.
format Online
Article
Text
id pubmed-10517959
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-105179592023-09-25 Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface Kwon, Duhyuk Kwak, Yongsu Lee, Doopyo Jo, Wonkeun Cho, Byeong-Gwan Koo, Tae-Yeong Song, Jonghyun Sci Rep Article We synthesized a CaZrO(3)/SrTiO(3) oxide heterostructure, which can serve as an alternative to LaAlO(3)/SrTiO(3), and confirmed the generation of 2-dimensional electron gas (2-DEG) at the heterointerface. We analyzed the electrical-transport properties of the 2-DEG to elucidate its intrinsic characteristics. Based on the magnetic field dependence of resistance at 2 K, which exhibited Weak Anti-localization (WAL) behaviors, the fitted Rashba parameter values were found to be about 12–15 × 10(–12) eV*m. These values are stronger than the previous reported Rashba parameters obtained from the 2-DEGs in other heterostructure systems and several layered 2D materials. The observed strong spin–orbit coupling (SOC) is attributed to the strong internal electric field generated by the lattice mismatch between the CaZrO(3) layer and SrTiO(3) substrate. This pioneering strong SOC of the 2-DEG at the CaZrO(3)/SrTiO(3) heterointerface may play a pivotal role in the developing future metal oxide-based quantum nanoelectronics devices. Nature Publishing Group UK 2023-09-23 /pmc/articles/PMC10517959/ /pubmed/37741927 http://dx.doi.org/10.1038/s41598-023-43247-y Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Kwon, Duhyuk
Kwak, Yongsu
Lee, Doopyo
Jo, Wonkeun
Cho, Byeong-Gwan
Koo, Tae-Yeong
Song, Jonghyun
Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface
title Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface
title_full Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface
title_fullStr Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface
title_full_unstemmed Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface
title_short Strong Rashba parameter of two-dimensional electron gas at CaZrO(3)/SrTiO(3) heterointerface
title_sort strong rashba parameter of two-dimensional electron gas at cazro(3)/srtio(3) heterointerface
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10517959/
https://www.ncbi.nlm.nih.gov/pubmed/37741927
http://dx.doi.org/10.1038/s41598-023-43247-y
work_keys_str_mv AT kwonduhyuk strongrashbaparameteroftwodimensionalelectrongasatcazro3srtio3heterointerface
AT kwakyongsu strongrashbaparameteroftwodimensionalelectrongasatcazro3srtio3heterointerface
AT leedoopyo strongrashbaparameteroftwodimensionalelectrongasatcazro3srtio3heterointerface
AT jowonkeun strongrashbaparameteroftwodimensionalelectrongasatcazro3srtio3heterointerface
AT chobyeonggwan strongrashbaparameteroftwodimensionalelectrongasatcazro3srtio3heterointerface
AT kootaeyeong strongrashbaparameteroftwodimensionalelectrongasatcazro3srtio3heterointerface
AT songjonghyun strongrashbaparameteroftwodimensionalelectrongasatcazro3srtio3heterointerface