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Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline

Tetracycline (TC), a commonly used antibiotic for studying bacterial illnesses in living organisms, poses a significant risk to the aquatic environment. Despite various conventional methods having been attempted to remove TC antibiotics from water solutions, they have not proven effective. Consequen...

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Autores principales: Varghese, Davis, Joe Raja Ruban, M., Joselene Suzan Jennifer, P., AnnieCanisius, D., Chakko, Seena, Muthupandi, S., Madhavan, J., Victor Antony Raj, M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10520693/
https://www.ncbi.nlm.nih.gov/pubmed/37767116
http://dx.doi.org/10.1039/d3ra05398a
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author Varghese, Davis
Joe Raja Ruban, M.
Joselene Suzan Jennifer, P.
AnnieCanisius, D.
Chakko, Seena
Muthupandi, S.
Madhavan, J.
Victor Antony Raj, M.
author_facet Varghese, Davis
Joe Raja Ruban, M.
Joselene Suzan Jennifer, P.
AnnieCanisius, D.
Chakko, Seena
Muthupandi, S.
Madhavan, J.
Victor Antony Raj, M.
author_sort Varghese, Davis
collection PubMed
description Tetracycline (TC), a commonly used antibiotic for studying bacterial illnesses in living organisms, poses a significant risk to the aquatic environment. Despite various conventional methods having been attempted to remove TC antibiotics from water solutions, they have not proven effective. Consequently, the focus of the research is on the photocatalytic degradation of TC. According to the research, MWCNTs were successfully incorporated into NiFe(2)O(4) nanoparticles, which reduced the pace at which charge carriers recombined after joining with MWCNTs. Subsequently, the catalyst's efficacy was assessed in a batch reactor by analyzing the weight percentage change of the nanocomposite, the initial concentration of TC antibiotics, the effects of pH and contact time. The identical operational parameters were employed to investigate the degradation of TC using NiFe(2)O(4) and MWCNTs as individual pure materials. The findings indicated that the photocatalytic process using NiFe(2)O(4)/MWCNTs achieved a degradation efficiency of 95.8% for TC at a pH value of 9. This result was obtained after a reaction time of 120 minutes, the concentration of TC solution was 10 mg L(−1), with a nanocomposite dose of 0.6 g L(−1) of TN 04 and 120 W m(−2). The pseudo-first-order approach was used to estimate the rate at which TC degrades. After four consecutive uses, it was observed that the photocatalysts maintained their original properties, with only a slight decrease of approximately 2.4% in the removal efficiency. The study demonstrated that the NiFe(2)O(4)/MWCNTs nanocomposite exhibited considerable efficiency in degrading TC. Due to its simple manufacture and useful recovery, it has the potential to function well as a catalyst for the removal and degradation of pharmaceutical organic contaminants.
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spelling pubmed-105206932023-09-27 Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline Varghese, Davis Joe Raja Ruban, M. Joselene Suzan Jennifer, P. AnnieCanisius, D. Chakko, Seena Muthupandi, S. Madhavan, J. Victor Antony Raj, M. RSC Adv Chemistry Tetracycline (TC), a commonly used antibiotic for studying bacterial illnesses in living organisms, poses a significant risk to the aquatic environment. Despite various conventional methods having been attempted to remove TC antibiotics from water solutions, they have not proven effective. Consequently, the focus of the research is on the photocatalytic degradation of TC. According to the research, MWCNTs were successfully incorporated into NiFe(2)O(4) nanoparticles, which reduced the pace at which charge carriers recombined after joining with MWCNTs. Subsequently, the catalyst's efficacy was assessed in a batch reactor by analyzing the weight percentage change of the nanocomposite, the initial concentration of TC antibiotics, the effects of pH and contact time. The identical operational parameters were employed to investigate the degradation of TC using NiFe(2)O(4) and MWCNTs as individual pure materials. The findings indicated that the photocatalytic process using NiFe(2)O(4)/MWCNTs achieved a degradation efficiency of 95.8% for TC at a pH value of 9. This result was obtained after a reaction time of 120 minutes, the concentration of TC solution was 10 mg L(−1), with a nanocomposite dose of 0.6 g L(−1) of TN 04 and 120 W m(−2). The pseudo-first-order approach was used to estimate the rate at which TC degrades. After four consecutive uses, it was observed that the photocatalysts maintained their original properties, with only a slight decrease of approximately 2.4% in the removal efficiency. The study demonstrated that the NiFe(2)O(4)/MWCNTs nanocomposite exhibited considerable efficiency in degrading TC. Due to its simple manufacture and useful recovery, it has the potential to function well as a catalyst for the removal and degradation of pharmaceutical organic contaminants. The Royal Society of Chemistry 2023-09-26 /pmc/articles/PMC10520693/ /pubmed/37767116 http://dx.doi.org/10.1039/d3ra05398a Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Varghese, Davis
Joe Raja Ruban, M.
Joselene Suzan Jennifer, P.
AnnieCanisius, D.
Chakko, Seena
Muthupandi, S.
Madhavan, J.
Victor Antony Raj, M.
Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline
title Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline
title_full Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline
title_fullStr Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline
title_full_unstemmed Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline
title_short Comprehensive analysis of NiFe(2)O(4)/MWCNTs nanocomposite to degrade a healthcare waste – tetracycline
title_sort comprehensive analysis of nife(2)o(4)/mwcnts nanocomposite to degrade a healthcare waste – tetracycline
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10520693/
https://www.ncbi.nlm.nih.gov/pubmed/37767116
http://dx.doi.org/10.1039/d3ra05398a
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