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Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model

[Image: see text] In the concept of a microstructured bubble column reactor, meshes coated with catalyst can cut the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. In previous work, we developed a closure model for the fate of bubbles interacting with a...

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Autores principales: Subburaj, Rahul, Tang, Yali, Deen, Niels G.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10540184/
https://www.ncbi.nlm.nih.gov/pubmed/37779599
http://dx.doi.org/10.1021/acs.iecr.3c02352
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author Subburaj, Rahul
Tang, Yali
Deen, Niels G.
author_facet Subburaj, Rahul
Tang, Yali
Deen, Niels G.
author_sort Subburaj, Rahul
collection PubMed
description [Image: see text] In the concept of a microstructured bubble column reactor, meshes coated with catalyst can cut the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. In previous work, we developed a closure model for the fate of bubbles interacting with a wire mesh based on the outcomes of energy balance analysis. In this paper, the model is validated using Euler–Lagrange simulations against two experimental cases of microstructured bubble columns. Before validation of the model, the definition of the deceleration thickness, as used in the calculation of the virtual mass term, is refined to introduce the effects of liquid viscosity and wire thickness. Proceeding with the validation, the inclusion of our cutting closure model results in an excellent match of the bubble size reduction by the wire mesh with the experimental data. Consequently, the simulations produce a more accurate prediction of the reactor performance for the gaseous reaction in view of the pH and gas holdup profiles. The effect of liquid viscosity on the bubble size reduction by the wire mesh is replicated accurately as well. Noticeably, the significance of bubble coalescence and breakup in bubble dynamics overperforms the role of bubble cutting at high superficial gas velocities; thus, further improvement is needed there. Finally, based on the validated cutting model, we share some perspectives on the design of wire meshes to increase the bubble interfacial area.
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spelling pubmed-105401842023-09-30 Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model Subburaj, Rahul Tang, Yali Deen, Niels G. Ind Eng Chem Res [Image: see text] In the concept of a microstructured bubble column reactor, meshes coated with catalyst can cut the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. In previous work, we developed a closure model for the fate of bubbles interacting with a wire mesh based on the outcomes of energy balance analysis. In this paper, the model is validated using Euler–Lagrange simulations against two experimental cases of microstructured bubble columns. Before validation of the model, the definition of the deceleration thickness, as used in the calculation of the virtual mass term, is refined to introduce the effects of liquid viscosity and wire thickness. Proceeding with the validation, the inclusion of our cutting closure model results in an excellent match of the bubble size reduction by the wire mesh with the experimental data. Consequently, the simulations produce a more accurate prediction of the reactor performance for the gaseous reaction in view of the pH and gas holdup profiles. The effect of liquid viscosity on the bubble size reduction by the wire mesh is replicated accurately as well. Noticeably, the significance of bubble coalescence and breakup in bubble dynamics overperforms the role of bubble cutting at high superficial gas velocities; thus, further improvement is needed there. Finally, based on the validated cutting model, we share some perspectives on the design of wire meshes to increase the bubble interfacial area. American Chemical Society 2023-09-12 /pmc/articles/PMC10540184/ /pubmed/37779599 http://dx.doi.org/10.1021/acs.iecr.3c02352 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Subburaj, Rahul
Tang, Yali
Deen, Niels G.
Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model
title Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model
title_full Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model
title_fullStr Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model
title_full_unstemmed Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model
title_short Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model
title_sort euler–lagrange simulations of microstructured bubble columns using a novel cutting model
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10540184/
https://www.ncbi.nlm.nih.gov/pubmed/37779599
http://dx.doi.org/10.1021/acs.iecr.3c02352
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