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Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model
[Image: see text] In the concept of a microstructured bubble column reactor, meshes coated with catalyst can cut the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. In previous work, we developed a closure model for the fate of bubbles interacting with a...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2023
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10540184/ https://www.ncbi.nlm.nih.gov/pubmed/37779599 http://dx.doi.org/10.1021/acs.iecr.3c02352 |
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author | Subburaj, Rahul Tang, Yali Deen, Niels G. |
author_facet | Subburaj, Rahul Tang, Yali Deen, Niels G. |
author_sort | Subburaj, Rahul |
collection | PubMed |
description | [Image: see text] In the concept of a microstructured bubble column reactor, meshes coated with catalyst can cut the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. In previous work, we developed a closure model for the fate of bubbles interacting with a wire mesh based on the outcomes of energy balance analysis. In this paper, the model is validated using Euler–Lagrange simulations against two experimental cases of microstructured bubble columns. Before validation of the model, the definition of the deceleration thickness, as used in the calculation of the virtual mass term, is refined to introduce the effects of liquid viscosity and wire thickness. Proceeding with the validation, the inclusion of our cutting closure model results in an excellent match of the bubble size reduction by the wire mesh with the experimental data. Consequently, the simulations produce a more accurate prediction of the reactor performance for the gaseous reaction in view of the pH and gas holdup profiles. The effect of liquid viscosity on the bubble size reduction by the wire mesh is replicated accurately as well. Noticeably, the significance of bubble coalescence and breakup in bubble dynamics overperforms the role of bubble cutting at high superficial gas velocities; thus, further improvement is needed there. Finally, based on the validated cutting model, we share some perspectives on the design of wire meshes to increase the bubble interfacial area. |
format | Online Article Text |
id | pubmed-10540184 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-105401842023-09-30 Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model Subburaj, Rahul Tang, Yali Deen, Niels G. Ind Eng Chem Res [Image: see text] In the concept of a microstructured bubble column reactor, meshes coated with catalyst can cut the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. In previous work, we developed a closure model for the fate of bubbles interacting with a wire mesh based on the outcomes of energy balance analysis. In this paper, the model is validated using Euler–Lagrange simulations against two experimental cases of microstructured bubble columns. Before validation of the model, the definition of the deceleration thickness, as used in the calculation of the virtual mass term, is refined to introduce the effects of liquid viscosity and wire thickness. Proceeding with the validation, the inclusion of our cutting closure model results in an excellent match of the bubble size reduction by the wire mesh with the experimental data. Consequently, the simulations produce a more accurate prediction of the reactor performance for the gaseous reaction in view of the pH and gas holdup profiles. The effect of liquid viscosity on the bubble size reduction by the wire mesh is replicated accurately as well. Noticeably, the significance of bubble coalescence and breakup in bubble dynamics overperforms the role of bubble cutting at high superficial gas velocities; thus, further improvement is needed there. Finally, based on the validated cutting model, we share some perspectives on the design of wire meshes to increase the bubble interfacial area. American Chemical Society 2023-09-12 /pmc/articles/PMC10540184/ /pubmed/37779599 http://dx.doi.org/10.1021/acs.iecr.3c02352 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Subburaj, Rahul Tang, Yali Deen, Niels G. Euler–Lagrange Simulations of Microstructured Bubble Columns Using a Novel Cutting Model |
title | Euler–Lagrange
Simulations of Microstructured Bubble Columns Using a Novel
Cutting
Model |
title_full | Euler–Lagrange
Simulations of Microstructured Bubble Columns Using a Novel
Cutting
Model |
title_fullStr | Euler–Lagrange
Simulations of Microstructured Bubble Columns Using a Novel
Cutting
Model |
title_full_unstemmed | Euler–Lagrange
Simulations of Microstructured Bubble Columns Using a Novel
Cutting
Model |
title_short | Euler–Lagrange
Simulations of Microstructured Bubble Columns Using a Novel
Cutting
Model |
title_sort | euler–lagrange
simulations of microstructured bubble columns using a novel
cutting
model |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10540184/ https://www.ncbi.nlm.nih.gov/pubmed/37779599 http://dx.doi.org/10.1021/acs.iecr.3c02352 |
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