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Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films

Kagome lattice hosts a plethora of quantum states arising from the interplay of topology, spin-orbit coupling, and electron correlations. Here, we report symmetry-breaking electronic orders tunable by an applied magnetic field in a model Kagome magnet FeSn consisting of alternating stacks of two-dim...

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Autores principales: Zhang, Huimin, Oli, Basu Dev, Zou, Qiang, Guo, Xu, Wang, Zhengfei, Li, Lian
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10550950/
https://www.ncbi.nlm.nih.gov/pubmed/37794009
http://dx.doi.org/10.1038/s41467-023-41831-4
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author Zhang, Huimin
Oli, Basu Dev
Zou, Qiang
Guo, Xu
Wang, Zhengfei
Li, Lian
author_facet Zhang, Huimin
Oli, Basu Dev
Zou, Qiang
Guo, Xu
Wang, Zhengfei
Li, Lian
author_sort Zhang, Huimin
collection PubMed
description Kagome lattice hosts a plethora of quantum states arising from the interplay of topology, spin-orbit coupling, and electron correlations. Here, we report symmetry-breaking electronic orders tunable by an applied magnetic field in a model Kagome magnet FeSn consisting of alternating stacks of two-dimensional Fe(3)Sn Kagome and Sn(2) honeycomb layers. On the Fe(3)Sn layer terminated FeSn thin films epitaxially grown on SrTiO(3)(111) substrates, we observe trimerization of the Kagome lattice using scanning tunneling microscopy/spectroscopy, breaking its six-fold rotational symmetry while preserving the translational symmetry. Such a trimerized Kagome lattice shows an energy-dependent contrast reversal in dI/dV maps, which is significantly enhanced by bound states induced by Sn vacancy defects. This trimerized Kagome lattice also exhibits stripe modulations that are energy-dependent and tunable by an applied in-plane magnetic field, indicating symmetry-breaking nematicity from the entangled magnetic and charge degrees of freedom in antiferromagnet FeSn.
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spelling pubmed-105509502023-10-06 Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films Zhang, Huimin Oli, Basu Dev Zou, Qiang Guo, Xu Wang, Zhengfei Li, Lian Nat Commun Article Kagome lattice hosts a plethora of quantum states arising from the interplay of topology, spin-orbit coupling, and electron correlations. Here, we report symmetry-breaking electronic orders tunable by an applied magnetic field in a model Kagome magnet FeSn consisting of alternating stacks of two-dimensional Fe(3)Sn Kagome and Sn(2) honeycomb layers. On the Fe(3)Sn layer terminated FeSn thin films epitaxially grown on SrTiO(3)(111) substrates, we observe trimerization of the Kagome lattice using scanning tunneling microscopy/spectroscopy, breaking its six-fold rotational symmetry while preserving the translational symmetry. Such a trimerized Kagome lattice shows an energy-dependent contrast reversal in dI/dV maps, which is significantly enhanced by bound states induced by Sn vacancy defects. This trimerized Kagome lattice also exhibits stripe modulations that are energy-dependent and tunable by an applied in-plane magnetic field, indicating symmetry-breaking nematicity from the entangled magnetic and charge degrees of freedom in antiferromagnet FeSn. Nature Publishing Group UK 2023-10-04 /pmc/articles/PMC10550950/ /pubmed/37794009 http://dx.doi.org/10.1038/s41467-023-41831-4 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Zhang, Huimin
Oli, Basu Dev
Zou, Qiang
Guo, Xu
Wang, Zhengfei
Li, Lian
Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
title Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
title_full Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
title_fullStr Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
title_full_unstemmed Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
title_short Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
title_sort visualizing symmetry-breaking electronic orders in epitaxial kagome magnet fesn films
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10550950/
https://www.ncbi.nlm.nih.gov/pubmed/37794009
http://dx.doi.org/10.1038/s41467-023-41831-4
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