Cargando…

High-temperature electrothermal remediation of multi-pollutants in soil

Soil contamination is an environmental issue due to increasing anthropogenic activities. Existing processes for soil remediation suffer from long treatment time and lack generality because of different sources, occurrences, and properties of pollutants. Here, we report a high-temperature electrother...

Descripción completa

Detalles Bibliográficos
Autores principales: Deng, Bing, Carter, Robert A., Cheng, Yi, Liu, Yuan, Eddy, Lucas, Wyss, Kevin M., Ucak-Astarlioglu, Mine G., Luong, Duy Xuan, Gao, Xiaodong, JeBailey, Khalil, Kittrell, Carter, Xu, Shichen, Jana, Debadrita, Torres, Mark Albert, Braam, Janet, Tour, James M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10567823/
https://www.ncbi.nlm.nih.gov/pubmed/37821460
http://dx.doi.org/10.1038/s41467-023-41898-z
_version_ 1785119220316504064
author Deng, Bing
Carter, Robert A.
Cheng, Yi
Liu, Yuan
Eddy, Lucas
Wyss, Kevin M.
Ucak-Astarlioglu, Mine G.
Luong, Duy Xuan
Gao, Xiaodong
JeBailey, Khalil
Kittrell, Carter
Xu, Shichen
Jana, Debadrita
Torres, Mark Albert
Braam, Janet
Tour, James M.
author_facet Deng, Bing
Carter, Robert A.
Cheng, Yi
Liu, Yuan
Eddy, Lucas
Wyss, Kevin M.
Ucak-Astarlioglu, Mine G.
Luong, Duy Xuan
Gao, Xiaodong
JeBailey, Khalil
Kittrell, Carter
Xu, Shichen
Jana, Debadrita
Torres, Mark Albert
Braam, Janet
Tour, James M.
author_sort Deng, Bing
collection PubMed
description Soil contamination is an environmental issue due to increasing anthropogenic activities. Existing processes for soil remediation suffer from long treatment time and lack generality because of different sources, occurrences, and properties of pollutants. Here, we report a high-temperature electrothermal process for rapid, water-free remediation of multiple pollutants in soil. The temperature of contaminated soil with carbon additives ramps up to 1000 to 3000 °C as needed within seconds via pulsed direct current input, enabling the vaporization of heavy metals like Cd, Hg, Pb, Co, Ni, and Cu, and graphitization of persistent organic pollutants like polycyclic aromatic hydrocarbons. The rapid treatment retains soil mineral constituents while increases infiltration rate and exchangeable nutrient supply, leading to soil fertilization and improved germination rates. We propose strategies for upscaling and field applications. Techno-economic analysis indicates the process holds the potential for being more energy-efficient and cost-effective compared to soil washing or thermal desorption.
format Online
Article
Text
id pubmed-10567823
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-105678232023-10-13 High-temperature electrothermal remediation of multi-pollutants in soil Deng, Bing Carter, Robert A. Cheng, Yi Liu, Yuan Eddy, Lucas Wyss, Kevin M. Ucak-Astarlioglu, Mine G. Luong, Duy Xuan Gao, Xiaodong JeBailey, Khalil Kittrell, Carter Xu, Shichen Jana, Debadrita Torres, Mark Albert Braam, Janet Tour, James M. Nat Commun Article Soil contamination is an environmental issue due to increasing anthropogenic activities. Existing processes for soil remediation suffer from long treatment time and lack generality because of different sources, occurrences, and properties of pollutants. Here, we report a high-temperature electrothermal process for rapid, water-free remediation of multiple pollutants in soil. The temperature of contaminated soil with carbon additives ramps up to 1000 to 3000 °C as needed within seconds via pulsed direct current input, enabling the vaporization of heavy metals like Cd, Hg, Pb, Co, Ni, and Cu, and graphitization of persistent organic pollutants like polycyclic aromatic hydrocarbons. The rapid treatment retains soil mineral constituents while increases infiltration rate and exchangeable nutrient supply, leading to soil fertilization and improved germination rates. We propose strategies for upscaling and field applications. Techno-economic analysis indicates the process holds the potential for being more energy-efficient and cost-effective compared to soil washing or thermal desorption. Nature Publishing Group UK 2023-10-11 /pmc/articles/PMC10567823/ /pubmed/37821460 http://dx.doi.org/10.1038/s41467-023-41898-z Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Deng, Bing
Carter, Robert A.
Cheng, Yi
Liu, Yuan
Eddy, Lucas
Wyss, Kevin M.
Ucak-Astarlioglu, Mine G.
Luong, Duy Xuan
Gao, Xiaodong
JeBailey, Khalil
Kittrell, Carter
Xu, Shichen
Jana, Debadrita
Torres, Mark Albert
Braam, Janet
Tour, James M.
High-temperature electrothermal remediation of multi-pollutants in soil
title High-temperature electrothermal remediation of multi-pollutants in soil
title_full High-temperature electrothermal remediation of multi-pollutants in soil
title_fullStr High-temperature electrothermal remediation of multi-pollutants in soil
title_full_unstemmed High-temperature electrothermal remediation of multi-pollutants in soil
title_short High-temperature electrothermal remediation of multi-pollutants in soil
title_sort high-temperature electrothermal remediation of multi-pollutants in soil
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10567823/
https://www.ncbi.nlm.nih.gov/pubmed/37821460
http://dx.doi.org/10.1038/s41467-023-41898-z
work_keys_str_mv AT dengbing hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT carterroberta hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT chengyi hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT liuyuan hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT eddylucas hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT wysskevinm hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT ucakastarlioglumineg hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT luongduyxuan hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT gaoxiaodong hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT jebaileykhalil hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT kittrellcarter hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT xushichen hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT janadebadrita hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT torresmarkalbert hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT braamjanet hightemperatureelectrothermalremediationofmultipollutantsinsoil
AT tourjamesm hightemperatureelectrothermalremediationofmultipollutantsinsoil