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High-temperature electrothermal remediation of multi-pollutants in soil
Soil contamination is an environmental issue due to increasing anthropogenic activities. Existing processes for soil remediation suffer from long treatment time and lack generality because of different sources, occurrences, and properties of pollutants. Here, we report a high-temperature electrother...
Autores principales: | , , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10567823/ https://www.ncbi.nlm.nih.gov/pubmed/37821460 http://dx.doi.org/10.1038/s41467-023-41898-z |
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author | Deng, Bing Carter, Robert A. Cheng, Yi Liu, Yuan Eddy, Lucas Wyss, Kevin M. Ucak-Astarlioglu, Mine G. Luong, Duy Xuan Gao, Xiaodong JeBailey, Khalil Kittrell, Carter Xu, Shichen Jana, Debadrita Torres, Mark Albert Braam, Janet Tour, James M. |
author_facet | Deng, Bing Carter, Robert A. Cheng, Yi Liu, Yuan Eddy, Lucas Wyss, Kevin M. Ucak-Astarlioglu, Mine G. Luong, Duy Xuan Gao, Xiaodong JeBailey, Khalil Kittrell, Carter Xu, Shichen Jana, Debadrita Torres, Mark Albert Braam, Janet Tour, James M. |
author_sort | Deng, Bing |
collection | PubMed |
description | Soil contamination is an environmental issue due to increasing anthropogenic activities. Existing processes for soil remediation suffer from long treatment time and lack generality because of different sources, occurrences, and properties of pollutants. Here, we report a high-temperature electrothermal process for rapid, water-free remediation of multiple pollutants in soil. The temperature of contaminated soil with carbon additives ramps up to 1000 to 3000 °C as needed within seconds via pulsed direct current input, enabling the vaporization of heavy metals like Cd, Hg, Pb, Co, Ni, and Cu, and graphitization of persistent organic pollutants like polycyclic aromatic hydrocarbons. The rapid treatment retains soil mineral constituents while increases infiltration rate and exchangeable nutrient supply, leading to soil fertilization and improved germination rates. We propose strategies for upscaling and field applications. Techno-economic analysis indicates the process holds the potential for being more energy-efficient and cost-effective compared to soil washing or thermal desorption. |
format | Online Article Text |
id | pubmed-10567823 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-105678232023-10-13 High-temperature electrothermal remediation of multi-pollutants in soil Deng, Bing Carter, Robert A. Cheng, Yi Liu, Yuan Eddy, Lucas Wyss, Kevin M. Ucak-Astarlioglu, Mine G. Luong, Duy Xuan Gao, Xiaodong JeBailey, Khalil Kittrell, Carter Xu, Shichen Jana, Debadrita Torres, Mark Albert Braam, Janet Tour, James M. Nat Commun Article Soil contamination is an environmental issue due to increasing anthropogenic activities. Existing processes for soil remediation suffer from long treatment time and lack generality because of different sources, occurrences, and properties of pollutants. Here, we report a high-temperature electrothermal process for rapid, water-free remediation of multiple pollutants in soil. The temperature of contaminated soil with carbon additives ramps up to 1000 to 3000 °C as needed within seconds via pulsed direct current input, enabling the vaporization of heavy metals like Cd, Hg, Pb, Co, Ni, and Cu, and graphitization of persistent organic pollutants like polycyclic aromatic hydrocarbons. The rapid treatment retains soil mineral constituents while increases infiltration rate and exchangeable nutrient supply, leading to soil fertilization and improved germination rates. We propose strategies for upscaling and field applications. Techno-economic analysis indicates the process holds the potential for being more energy-efficient and cost-effective compared to soil washing or thermal desorption. Nature Publishing Group UK 2023-10-11 /pmc/articles/PMC10567823/ /pubmed/37821460 http://dx.doi.org/10.1038/s41467-023-41898-z Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Deng, Bing Carter, Robert A. Cheng, Yi Liu, Yuan Eddy, Lucas Wyss, Kevin M. Ucak-Astarlioglu, Mine G. Luong, Duy Xuan Gao, Xiaodong JeBailey, Khalil Kittrell, Carter Xu, Shichen Jana, Debadrita Torres, Mark Albert Braam, Janet Tour, James M. High-temperature electrothermal remediation of multi-pollutants in soil |
title | High-temperature electrothermal remediation of multi-pollutants in soil |
title_full | High-temperature electrothermal remediation of multi-pollutants in soil |
title_fullStr | High-temperature electrothermal remediation of multi-pollutants in soil |
title_full_unstemmed | High-temperature electrothermal remediation of multi-pollutants in soil |
title_short | High-temperature electrothermal remediation of multi-pollutants in soil |
title_sort | high-temperature electrothermal remediation of multi-pollutants in soil |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10567823/ https://www.ncbi.nlm.nih.gov/pubmed/37821460 http://dx.doi.org/10.1038/s41467-023-41898-z |
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