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Numerical Simulation of a High-Pressure Reactive Furnace in Recovering Sulfur from Sour Gas
[Image: see text] Nowadays, the Claus process is one of the most efficient procedures to recover sulfur from acid gases. In the current study, the effect of working pressure and the role of initial species (sour gas, ammonia, carbon dioxide, hydrocarbon, nitrogen, and oxygen) are analyzed using COMS...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2023
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10568715/ https://www.ncbi.nlm.nih.gov/pubmed/37841124 http://dx.doi.org/10.1021/acsomega.3c03065 |
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author | Eskandarzadeh, Hossein Akbari, Ghasem Yazdi, Mohammad Eftekhari Lohrasbi Nichkoohi, Ali |
author_facet | Eskandarzadeh, Hossein Akbari, Ghasem Yazdi, Mohammad Eftekhari Lohrasbi Nichkoohi, Ali |
author_sort | Eskandarzadeh, Hossein |
collection | PubMed |
description | [Image: see text] Nowadays, the Claus process is one of the most efficient procedures to recover sulfur from acid gases. In the current study, the effect of working pressure and the role of initial species (sour gas, ammonia, carbon dioxide, hydrocarbon, nitrogen, and oxygen) are analyzed using COMSOL software. The reaction occurs between acid gases, which contain 88% H(2)S, 10.5% CO(2), 0.49% N(2), and 1.01% CH(4) in terms of molar percentage, and pure air. A good agreement is obtained between the numerical simulation results and experimental data. According to the results, there is a direct correlation between the conversion rate of acid gases and the increase in pressure. However, this rise in reactor pressure also leads to an undesirable increase in the outlet temperature. It is also observed that reduction of hydrogen sulfide inflow decreases the sulfur monoxide production rate, which in turn significantly affects the reactor temperature and the sulfur recovery rate. The more the oxygen that enters the reactor, the more the hydrogen sulfides that change into sulfur. |
format | Online Article Text |
id | pubmed-10568715 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-105687152023-10-13 Numerical Simulation of a High-Pressure Reactive Furnace in Recovering Sulfur from Sour Gas Eskandarzadeh, Hossein Akbari, Ghasem Yazdi, Mohammad Eftekhari Lohrasbi Nichkoohi, Ali ACS Omega [Image: see text] Nowadays, the Claus process is one of the most efficient procedures to recover sulfur from acid gases. In the current study, the effect of working pressure and the role of initial species (sour gas, ammonia, carbon dioxide, hydrocarbon, nitrogen, and oxygen) are analyzed using COMSOL software. The reaction occurs between acid gases, which contain 88% H(2)S, 10.5% CO(2), 0.49% N(2), and 1.01% CH(4) in terms of molar percentage, and pure air. A good agreement is obtained between the numerical simulation results and experimental data. According to the results, there is a direct correlation between the conversion rate of acid gases and the increase in pressure. However, this rise in reactor pressure also leads to an undesirable increase in the outlet temperature. It is also observed that reduction of hydrogen sulfide inflow decreases the sulfur monoxide production rate, which in turn significantly affects the reactor temperature and the sulfur recovery rate. The more the oxygen that enters the reactor, the more the hydrogen sulfides that change into sulfur. American Chemical Society 2023-09-25 /pmc/articles/PMC10568715/ /pubmed/37841124 http://dx.doi.org/10.1021/acsomega.3c03065 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Eskandarzadeh, Hossein Akbari, Ghasem Yazdi, Mohammad Eftekhari Lohrasbi Nichkoohi, Ali Numerical Simulation of a High-Pressure Reactive Furnace in Recovering Sulfur from Sour Gas |
title | Numerical Simulation
of a High-Pressure Reactive Furnace
in Recovering Sulfur from Sour Gas |
title_full | Numerical Simulation
of a High-Pressure Reactive Furnace
in Recovering Sulfur from Sour Gas |
title_fullStr | Numerical Simulation
of a High-Pressure Reactive Furnace
in Recovering Sulfur from Sour Gas |
title_full_unstemmed | Numerical Simulation
of a High-Pressure Reactive Furnace
in Recovering Sulfur from Sour Gas |
title_short | Numerical Simulation
of a High-Pressure Reactive Furnace
in Recovering Sulfur from Sour Gas |
title_sort | numerical simulation
of a high-pressure reactive furnace
in recovering sulfur from sour gas |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10568715/ https://www.ncbi.nlm.nih.gov/pubmed/37841124 http://dx.doi.org/10.1021/acsomega.3c03065 |
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