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Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline

Developing a sustainable environment requires addressing primitive water scarcity and water contamination. Antibiotics such as oxytetracycline (OTC) may accumulate in the environment and in the human body, increasing the risks to the ecosystem. The treatment of polluted water and the production of p...

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Autores principales: Alomar, Muneerah, Arshad, Naila, Irshad, Muhammad Sultan, Abdelmohsen, Shaimaa A. M., Ahmed, Iftikhar, Alhoshani, Nawal, Alqarni, Areej S.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10609317/
https://www.ncbi.nlm.nih.gov/pubmed/37887915
http://dx.doi.org/10.3390/nano13202764
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author Alomar, Muneerah
Arshad, Naila
Irshad, Muhammad Sultan
Abdelmohsen, Shaimaa A. M.
Ahmed, Iftikhar
Alhoshani, Nawal
Alqarni, Areej S.
author_facet Alomar, Muneerah
Arshad, Naila
Irshad, Muhammad Sultan
Abdelmohsen, Shaimaa A. M.
Ahmed, Iftikhar
Alhoshani, Nawal
Alqarni, Areej S.
author_sort Alomar, Muneerah
collection PubMed
description Developing a sustainable environment requires addressing primitive water scarcity and water contamination. Antibiotics such as oxytetracycline (OTC) may accumulate in the environment and in the human body, increasing the risks to the ecosystem. The treatment of polluted water and the production of potable water can be achieved in a variety of ways, including photodegradation, solar distillation, and filtration. Freshwater supplies can be increased by implementing energy-efficient technologies for the production of clean water. Solar water evaporation combined with photocatalytic degradation and sterilization offers a promising avenue for integration into the clean water and energy production fields. The present study reports the synthesis of a 3D solar steam generator comprised of BiVO(4) and carbon nanotubes (CNT) nanocomposite decorated over a cigarette filter as the light-to-heat conversion layer for solar steam generation. The BiVO(4)@CNT-based 3D solar evaporator over the hydrophilic cellulosic fibers of the cigarette filter endowed excellent evaporation rates (2.36 kg m(−2) h(−1)) under 1 kW m(−2) solar irradiation, owing to its superior hydrophilicity and broadband solar absorption (96%) equipped with localized heating at microscale thermal confinement optimized by the minimum thermal conductivity of the overall system. Furthermore, the BiVO(4)@CNT composite exhibited a heightened photo activity up to 83% of the photodegradation of oxytetracycline (OTC) antibiotic due to the inhibition of charge recombination from the industrial effluents. This approach transforms the water-energy nexus into a synergistic bond that offers opportunities to meet expected demand, rather than being competitive.
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spelling pubmed-106093172023-10-28 Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline Alomar, Muneerah Arshad, Naila Irshad, Muhammad Sultan Abdelmohsen, Shaimaa A. M. Ahmed, Iftikhar Alhoshani, Nawal Alqarni, Areej S. Nanomaterials (Basel) Article Developing a sustainable environment requires addressing primitive water scarcity and water contamination. Antibiotics such as oxytetracycline (OTC) may accumulate in the environment and in the human body, increasing the risks to the ecosystem. The treatment of polluted water and the production of potable water can be achieved in a variety of ways, including photodegradation, solar distillation, and filtration. Freshwater supplies can be increased by implementing energy-efficient technologies for the production of clean water. Solar water evaporation combined with photocatalytic degradation and sterilization offers a promising avenue for integration into the clean water and energy production fields. The present study reports the synthesis of a 3D solar steam generator comprised of BiVO(4) and carbon nanotubes (CNT) nanocomposite decorated over a cigarette filter as the light-to-heat conversion layer for solar steam generation. The BiVO(4)@CNT-based 3D solar evaporator over the hydrophilic cellulosic fibers of the cigarette filter endowed excellent evaporation rates (2.36 kg m(−2) h(−1)) under 1 kW m(−2) solar irradiation, owing to its superior hydrophilicity and broadband solar absorption (96%) equipped with localized heating at microscale thermal confinement optimized by the minimum thermal conductivity of the overall system. Furthermore, the BiVO(4)@CNT composite exhibited a heightened photo activity up to 83% of the photodegradation of oxytetracycline (OTC) antibiotic due to the inhibition of charge recombination from the industrial effluents. This approach transforms the water-energy nexus into a synergistic bond that offers opportunities to meet expected demand, rather than being competitive. MDPI 2023-10-15 /pmc/articles/PMC10609317/ /pubmed/37887915 http://dx.doi.org/10.3390/nano13202764 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Alomar, Muneerah
Arshad, Naila
Irshad, Muhammad Sultan
Abdelmohsen, Shaimaa A. M.
Ahmed, Iftikhar
Alhoshani, Nawal
Alqarni, Areej S.
Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline
title Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline
title_full Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline
title_fullStr Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline
title_full_unstemmed Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline
title_short Multi-Walled CNTs/BiVO(4) Heterostructures for Solar-Driven Evaporation System and Efficient Photocatalytic Activity against Oxytetracycline
title_sort multi-walled cnts/bivo(4) heterostructures for solar-driven evaporation system and efficient photocatalytic activity against oxytetracycline
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10609317/
https://www.ncbi.nlm.nih.gov/pubmed/37887915
http://dx.doi.org/10.3390/nano13202764
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