Cargando…
Charge stripes in the graphene-based materials
We present an analytical model of the charge density wave instability in graphene sheets within the intercalated graphite CaC(6) compound. The instability yields the experimentally observed uniaxial charge stripes of periodically modulated electron density, coupled to the softest phonon mode of the...
Autores principales: | , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10622548/ https://www.ncbi.nlm.nih.gov/pubmed/37919346 http://dx.doi.org/10.1038/s41598-023-46157-1 |
_version_ | 1785130563522265088 |
---|---|
author | Grozić, Petra Keran, Barbara Kadigrobov, Anatoly M. Radić, Danko |
author_facet | Grozić, Petra Keran, Barbara Kadigrobov, Anatoly M. Radić, Danko |
author_sort | Grozić, Petra |
collection | PubMed |
description | We present an analytical model of the charge density wave instability in graphene sheets within the intercalated graphite CaC(6) compound. The instability yields the experimentally observed uniaxial charge stripes of periodically modulated electron density, coupled to the softest phonon mode of the superlattice consisting of the Ca atoms intercalated between graphene planes. The Fermi surface of the chemically doped graphene undergoes the novel type of instability driven by the mechanism that gains the condensation energy of the stripe state by the topological reconstruction of the Fermi surface. This mechanism appears to be entirely different from the one based on the Fermi surface nesting, which has been considered a paradigm in the present literature concerning the onset of charge density waves. |
format | Online Article Text |
id | pubmed-10622548 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-106225482023-11-04 Charge stripes in the graphene-based materials Grozić, Petra Keran, Barbara Kadigrobov, Anatoly M. Radić, Danko Sci Rep Article We present an analytical model of the charge density wave instability in graphene sheets within the intercalated graphite CaC(6) compound. The instability yields the experimentally observed uniaxial charge stripes of periodically modulated electron density, coupled to the softest phonon mode of the superlattice consisting of the Ca atoms intercalated between graphene planes. The Fermi surface of the chemically doped graphene undergoes the novel type of instability driven by the mechanism that gains the condensation energy of the stripe state by the topological reconstruction of the Fermi surface. This mechanism appears to be entirely different from the one based on the Fermi surface nesting, which has been considered a paradigm in the present literature concerning the onset of charge density waves. Nature Publishing Group UK 2023-11-02 /pmc/articles/PMC10622548/ /pubmed/37919346 http://dx.doi.org/10.1038/s41598-023-46157-1 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Grozić, Petra Keran, Barbara Kadigrobov, Anatoly M. Radić, Danko Charge stripes in the graphene-based materials |
title | Charge stripes in the graphene-based materials |
title_full | Charge stripes in the graphene-based materials |
title_fullStr | Charge stripes in the graphene-based materials |
title_full_unstemmed | Charge stripes in the graphene-based materials |
title_short | Charge stripes in the graphene-based materials |
title_sort | charge stripes in the graphene-based materials |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10622548/ https://www.ncbi.nlm.nih.gov/pubmed/37919346 http://dx.doi.org/10.1038/s41598-023-46157-1 |
work_keys_str_mv | AT grozicpetra chargestripesinthegraphenebasedmaterials AT keranbarbara chargestripesinthegraphenebasedmaterials AT kadigrobovanatolym chargestripesinthegraphenebasedmaterials AT radicdanko chargestripesinthegraphenebasedmaterials |