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Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover

[Image: see text] Reducing the energy intensity of the mechanical refining-based pretreatment process for producing lignocellulosic-derived sugars without significantly affecting enzymatic hydrolysis sugar yields is challenging. This work investigated the impact of different refining conditions on e...

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Autores principales: Li, Yudong, Davis, Ryan, Tan, Eric C. D., Dempsey, Jacob, Lynch, Kelsey, Sievers, David A., Chen, Xiaowen
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10630967/
https://www.ncbi.nlm.nih.gov/pubmed/37969886
http://dx.doi.org/10.1021/acssuschemeng.3c03796
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author Li, Yudong
Davis, Ryan
Tan, Eric C. D.
Dempsey, Jacob
Lynch, Kelsey
Sievers, David A.
Chen, Xiaowen
author_facet Li, Yudong
Davis, Ryan
Tan, Eric C. D.
Dempsey, Jacob
Lynch, Kelsey
Sievers, David A.
Chen, Xiaowen
author_sort Li, Yudong
collection PubMed
description [Image: see text] Reducing the energy intensity of the mechanical refining-based pretreatment process for producing lignocellulosic-derived sugars without significantly affecting enzymatic hydrolysis sugar yields is challenging. This work investigated the impact of different refining conditions on energy consumption, enzymatic sugar yields, minimum sugar selling price, and environmental impacts for the conversion of corn stover to sugars. A positive proportionate correlation between specific energy consumption and enzymatic sugar yields was observed when changing the refiner plate gap was changed, which agrees with other reported works. However, the correlation between specific energy consumption and enzymatic sugar yields is not straightforward when the rotational speed and refiner plate design change. We observed that, for a corn stover material with low consistency disc refining, specific energy consumption decreased by >50% by decreasing the rotation speed without affecting enzymatic sugar yields. By changing refiner plate designs, a 45% reduction in specific energy consumption could be achieved without affecting the glucose yield, albeit still with a detrimental impact on the xylose yield. Our high-fidelity disc refining model was able to predict the energy consumption for different refiner plate geometry designs and operating conditions. Techno-economic and life-cycle analyses indicate that the plate design and operating conditions have a direct impact on overall process power consumption and sugar yields, with sugar yields strongly dictating the minimum sugar selling price, the life cycle greenhouse gas emissions, and fossil energy consumption. To minimize the environmental impact and maximize process economics, optimization of the mechanical refining process should target maintaining high sugar yields, while lowering refining energy consumption.
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spelling pubmed-106309672023-11-15 Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover Li, Yudong Davis, Ryan Tan, Eric C. D. Dempsey, Jacob Lynch, Kelsey Sievers, David A. Chen, Xiaowen ACS Sustain Chem Eng [Image: see text] Reducing the energy intensity of the mechanical refining-based pretreatment process for producing lignocellulosic-derived sugars without significantly affecting enzymatic hydrolysis sugar yields is challenging. This work investigated the impact of different refining conditions on energy consumption, enzymatic sugar yields, minimum sugar selling price, and environmental impacts for the conversion of corn stover to sugars. A positive proportionate correlation between specific energy consumption and enzymatic sugar yields was observed when changing the refiner plate gap was changed, which agrees with other reported works. However, the correlation between specific energy consumption and enzymatic sugar yields is not straightforward when the rotational speed and refiner plate design change. We observed that, for a corn stover material with low consistency disc refining, specific energy consumption decreased by >50% by decreasing the rotation speed without affecting enzymatic sugar yields. By changing refiner plate designs, a 45% reduction in specific energy consumption could be achieved without affecting the glucose yield, albeit still with a detrimental impact on the xylose yield. Our high-fidelity disc refining model was able to predict the energy consumption for different refiner plate geometry designs and operating conditions. Techno-economic and life-cycle analyses indicate that the plate design and operating conditions have a direct impact on overall process power consumption and sugar yields, with sugar yields strongly dictating the minimum sugar selling price, the life cycle greenhouse gas emissions, and fossil energy consumption. To minimize the environmental impact and maximize process economics, optimization of the mechanical refining process should target maintaining high sugar yields, while lowering refining energy consumption. American Chemical Society 2023-10-21 /pmc/articles/PMC10630967/ /pubmed/37969886 http://dx.doi.org/10.1021/acssuschemeng.3c03796 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Li, Yudong
Davis, Ryan
Tan, Eric C. D.
Dempsey, Jacob
Lynch, Kelsey
Sievers, David A.
Chen, Xiaowen
Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover
title Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover
title_full Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover
title_fullStr Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover
title_full_unstemmed Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover
title_short Impact of Mechanical Refining Conditions on the Energy Consumption, Enzymatic Digestibility, and Economics of Sugar Production from Corn Stover
title_sort impact of mechanical refining conditions on the energy consumption, enzymatic digestibility, and economics of sugar production from corn stover
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10630967/
https://www.ncbi.nlm.nih.gov/pubmed/37969886
http://dx.doi.org/10.1021/acssuschemeng.3c03796
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