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Superconducting nonlinear transport in optically driven high-temperature K(3)C(60)

Optically driven quantum materials exhibit a variety of non-equilibrium functional phenomena, which to date have been primarily studied with ultrafast optical, X-Ray and photo-emission spectroscopy. However, little has been done to characterize their transient electrical responses, which are directl...

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Autores principales: Wang, E., Adelinia, J. D., Chavez-Cervantes, M., Matsuyama, T., Fechner, M., Buzzi, M., Meier, G., Cavalleri, A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10636163/
https://www.ncbi.nlm.nih.gov/pubmed/37945698
http://dx.doi.org/10.1038/s41467-023-42989-7
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author Wang, E.
Adelinia, J. D.
Chavez-Cervantes, M.
Matsuyama, T.
Fechner, M.
Buzzi, M.
Meier, G.
Cavalleri, A.
author_facet Wang, E.
Adelinia, J. D.
Chavez-Cervantes, M.
Matsuyama, T.
Fechner, M.
Buzzi, M.
Meier, G.
Cavalleri, A.
author_sort Wang, E.
collection PubMed
description Optically driven quantum materials exhibit a variety of non-equilibrium functional phenomena, which to date have been primarily studied with ultrafast optical, X-Ray and photo-emission spectroscopy. However, little has been done to characterize their transient electrical responses, which are directly associated with the functionality of these materials. Especially interesting are linear and nonlinear current-voltage characteristics at frequencies below 1 THz, which are not easily measured at picosecond temporal resolution. Here, we report on ultrafast transport measurements in photo-excited K(3)C(60). Thin films of this compound were connected to photo-conductive switches with co-planar waveguides. We observe characteristic nonlinear current-voltage responses, which in these films point to photo-induced granular superconductivity. Although these dynamics are not necessarily identical to those reported for the powder samples studied so far, they provide valuable new information on the nature of the light-induced superconducting-like state above equilibrium T(c). Furthermore, integration of non-equilibrium superconductivity into optoelectronic platforms may lead to integration in high-speed devices based on this effect.
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spelling pubmed-106361632023-11-11 Superconducting nonlinear transport in optically driven high-temperature K(3)C(60) Wang, E. Adelinia, J. D. Chavez-Cervantes, M. Matsuyama, T. Fechner, M. Buzzi, M. Meier, G. Cavalleri, A. Nat Commun Article Optically driven quantum materials exhibit a variety of non-equilibrium functional phenomena, which to date have been primarily studied with ultrafast optical, X-Ray and photo-emission spectroscopy. However, little has been done to characterize their transient electrical responses, which are directly associated with the functionality of these materials. Especially interesting are linear and nonlinear current-voltage characteristics at frequencies below 1 THz, which are not easily measured at picosecond temporal resolution. Here, we report on ultrafast transport measurements in photo-excited K(3)C(60). Thin films of this compound were connected to photo-conductive switches with co-planar waveguides. We observe characteristic nonlinear current-voltage responses, which in these films point to photo-induced granular superconductivity. Although these dynamics are not necessarily identical to those reported for the powder samples studied so far, they provide valuable new information on the nature of the light-induced superconducting-like state above equilibrium T(c). Furthermore, integration of non-equilibrium superconductivity into optoelectronic platforms may lead to integration in high-speed devices based on this effect. Nature Publishing Group UK 2023-11-09 /pmc/articles/PMC10636163/ /pubmed/37945698 http://dx.doi.org/10.1038/s41467-023-42989-7 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Wang, E.
Adelinia, J. D.
Chavez-Cervantes, M.
Matsuyama, T.
Fechner, M.
Buzzi, M.
Meier, G.
Cavalleri, A.
Superconducting nonlinear transport in optically driven high-temperature K(3)C(60)
title Superconducting nonlinear transport in optically driven high-temperature K(3)C(60)
title_full Superconducting nonlinear transport in optically driven high-temperature K(3)C(60)
title_fullStr Superconducting nonlinear transport in optically driven high-temperature K(3)C(60)
title_full_unstemmed Superconducting nonlinear transport in optically driven high-temperature K(3)C(60)
title_short Superconducting nonlinear transport in optically driven high-temperature K(3)C(60)
title_sort superconducting nonlinear transport in optically driven high-temperature k(3)c(60)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10636163/
https://www.ncbi.nlm.nih.gov/pubmed/37945698
http://dx.doi.org/10.1038/s41467-023-42989-7
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