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A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh
[Image: see text] In the concept of a microstructured bubble column reactor, microstructuring of the catalyst carrier is realized by introducing a static mesh of thin wires coated with catalyst inside the column. Meanwhile, the wires also serve the purpose of cutting the bubbles, which in turn resul...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2023
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10655082/ https://www.ncbi.nlm.nih.gov/pubmed/38020787 http://dx.doi.org/10.1021/acs.iecr.3c00265 |
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author | Subburaj, Rahul Tang, Yali Deen, Niels G. |
author_facet | Subburaj, Rahul Tang, Yali Deen, Niels G. |
author_sort | Subburaj, Rahul |
collection | PubMed |
description | [Image: see text] In the concept of a microstructured bubble column reactor, microstructuring of the catalyst carrier is realized by introducing a static mesh of thin wires coated with catalyst inside the column. Meanwhile, the wires also serve the purpose of cutting the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. However, there are no models that can predict the fate of bubbles (cut/stuck) passing through these wires, thus making the reactor optimization difficult. In this work, based on several typical bubble–wire interacting configurations, we analyze the outcomes by applying the energy balance of the bubble focusing on buoyancy and surface tension. Two limiting cases of viscosity, corresponding to the ability of the bubble to reconfigure into the lowest energy state, are investigated. Upon analysis, it is observed that a narrow mesh spacing and a smaller bubble Eötvös number generally result in bubbles getting stuck underneath the wire. We have obtained the threshold grid spacing and the critical Eötvös number for bubble passage and bubble cutting, which are verified by the direct numerical simulation results of bubble passing through a single mesh opening. The derived energy balance is generalized to large meshes with multiple openings and different configurations. Finally, a closure model based on the outcomes of energy-balance analysis is proposed for Euler–Lagrange simulations of microstructured bubble columns. |
format | Online Article Text |
id | pubmed-10655082 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-106550822023-11-17 A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh Subburaj, Rahul Tang, Yali Deen, Niels G. Ind Eng Chem Res [Image: see text] In the concept of a microstructured bubble column reactor, microstructuring of the catalyst carrier is realized by introducing a static mesh of thin wires coated with catalyst inside the column. Meanwhile, the wires also serve the purpose of cutting the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. However, there are no models that can predict the fate of bubbles (cut/stuck) passing through these wires, thus making the reactor optimization difficult. In this work, based on several typical bubble–wire interacting configurations, we analyze the outcomes by applying the energy balance of the bubble focusing on buoyancy and surface tension. Two limiting cases of viscosity, corresponding to the ability of the bubble to reconfigure into the lowest energy state, are investigated. Upon analysis, it is observed that a narrow mesh spacing and a smaller bubble Eötvös number generally result in bubbles getting stuck underneath the wire. We have obtained the threshold grid spacing and the critical Eötvös number for bubble passage and bubble cutting, which are verified by the direct numerical simulation results of bubble passing through a single mesh opening. The derived energy balance is generalized to large meshes with multiple openings and different configurations. Finally, a closure model based on the outcomes of energy-balance analysis is proposed for Euler–Lagrange simulations of microstructured bubble columns. American Chemical Society 2023-05-08 /pmc/articles/PMC10655082/ /pubmed/38020787 http://dx.doi.org/10.1021/acs.iecr.3c00265 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Subburaj, Rahul Tang, Yali Deen, Niels G. A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh |
title | A Model for the
Fate of a Gas Bubble Interacting with
a Wire Mesh |
title_full | A Model for the
Fate of a Gas Bubble Interacting with
a Wire Mesh |
title_fullStr | A Model for the
Fate of a Gas Bubble Interacting with
a Wire Mesh |
title_full_unstemmed | A Model for the
Fate of a Gas Bubble Interacting with
a Wire Mesh |
title_short | A Model for the
Fate of a Gas Bubble Interacting with
a Wire Mesh |
title_sort | model for the
fate of a gas bubble interacting with
a wire mesh |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10655082/ https://www.ncbi.nlm.nih.gov/pubmed/38020787 http://dx.doi.org/10.1021/acs.iecr.3c00265 |
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