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A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh

[Image: see text] In the concept of a microstructured bubble column reactor, microstructuring of the catalyst carrier is realized by introducing a static mesh of thin wires coated with catalyst inside the column. Meanwhile, the wires also serve the purpose of cutting the bubbles, which in turn resul...

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Autores principales: Subburaj, Rahul, Tang, Yali, Deen, Niels G.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10655082/
https://www.ncbi.nlm.nih.gov/pubmed/38020787
http://dx.doi.org/10.1021/acs.iecr.3c00265
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author Subburaj, Rahul
Tang, Yali
Deen, Niels G.
author_facet Subburaj, Rahul
Tang, Yali
Deen, Niels G.
author_sort Subburaj, Rahul
collection PubMed
description [Image: see text] In the concept of a microstructured bubble column reactor, microstructuring of the catalyst carrier is realized by introducing a static mesh of thin wires coated with catalyst inside the column. Meanwhile, the wires also serve the purpose of cutting the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. However, there are no models that can predict the fate of bubbles (cut/stuck) passing through these wires, thus making the reactor optimization difficult. In this work, based on several typical bubble–wire interacting configurations, we analyze the outcomes by applying the energy balance of the bubble focusing on buoyancy and surface tension. Two limiting cases of viscosity, corresponding to the ability of the bubble to reconfigure into the lowest energy state, are investigated. Upon analysis, it is observed that a narrow mesh spacing and a smaller bubble Eötvös number generally result in bubbles getting stuck underneath the wire. We have obtained the threshold grid spacing and the critical Eötvös number for bubble passage and bubble cutting, which are verified by the direct numerical simulation results of bubble passing through a single mesh opening. The derived energy balance is generalized to large meshes with multiple openings and different configurations. Finally, a closure model based on the outcomes of energy-balance analysis is proposed for Euler–Lagrange simulations of microstructured bubble columns.
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spelling pubmed-106550822023-11-17 A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh Subburaj, Rahul Tang, Yali Deen, Niels G. Ind Eng Chem Res [Image: see text] In the concept of a microstructured bubble column reactor, microstructuring of the catalyst carrier is realized by introducing a static mesh of thin wires coated with catalyst inside the column. Meanwhile, the wires also serve the purpose of cutting the bubbles, which in turn results in high interfacial area and enhanced interface hydrodynamics. However, there are no models that can predict the fate of bubbles (cut/stuck) passing through these wires, thus making the reactor optimization difficult. In this work, based on several typical bubble–wire interacting configurations, we analyze the outcomes by applying the energy balance of the bubble focusing on buoyancy and surface tension. Two limiting cases of viscosity, corresponding to the ability of the bubble to reconfigure into the lowest energy state, are investigated. Upon analysis, it is observed that a narrow mesh spacing and a smaller bubble Eötvös number generally result in bubbles getting stuck underneath the wire. We have obtained the threshold grid spacing and the critical Eötvös number for bubble passage and bubble cutting, which are verified by the direct numerical simulation results of bubble passing through a single mesh opening. The derived energy balance is generalized to large meshes with multiple openings and different configurations. Finally, a closure model based on the outcomes of energy-balance analysis is proposed for Euler–Lagrange simulations of microstructured bubble columns. American Chemical Society 2023-05-08 /pmc/articles/PMC10655082/ /pubmed/38020787 http://dx.doi.org/10.1021/acs.iecr.3c00265 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Subburaj, Rahul
Tang, Yali
Deen, Niels G.
A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh
title A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh
title_full A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh
title_fullStr A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh
title_full_unstemmed A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh
title_short A Model for the Fate of a Gas Bubble Interacting with a Wire Mesh
title_sort model for the fate of a gas bubble interacting with a wire mesh
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10655082/
https://www.ncbi.nlm.nih.gov/pubmed/38020787
http://dx.doi.org/10.1021/acs.iecr.3c00265
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