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Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires

Gas sensors play a pivotal role in environmental monitoring, with NO(2) sensors standing out due to their exceptional selectivity and sensitivity. Yet, a prevalent challenge remains: the prolonged recovery time of many sensors, often spanning hundreds of seconds, compromises efficiency and undermine...

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Autores principales: Shen, Yunkun, Wang, Kaili, Liu, Hao, Chen, Liping, Jin, Zhihan, Yan, Shancheng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10675235/
https://www.ncbi.nlm.nih.gov/pubmed/38005485
http://dx.doi.org/10.3390/s23229097
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author Shen, Yunkun
Wang, Kaili
Liu, Hao
Chen, Liping
Jin, Zhihan
Yan, Shancheng
author_facet Shen, Yunkun
Wang, Kaili
Liu, Hao
Chen, Liping
Jin, Zhihan
Yan, Shancheng
author_sort Shen, Yunkun
collection PubMed
description Gas sensors play a pivotal role in environmental monitoring, with NO(2) sensors standing out due to their exceptional selectivity and sensitivity. Yet, a prevalent challenge remains: the prolonged recovery time of many sensors, often spanning hundreds of seconds, compromises efficiency and undermines the precision of continuous detection. This paper introduces an efficient NO(2) sensor using TeO(2) nanowires, offering significantly reduced recovery times. The TeO(2) nanowires, prepared through a straightforward thermal oxidation process, exhibit a unique yet smooth surface. The structural characterizations confirm the formation of pure-phase TeO(2) after the anneal oxidation. TeO(2) nanowires are extremely sensitive to NO(2) gas, and the maximum response (defined as the ratio of resistance in the air to that under the target gas) to NO(2) (10 ppm) is 1.559. In addition, TeO(2) nanowire-based sensors can return to the initial state in about 6–7 s at 100 °C. The high sensitivity can be attributed to the length–diameter rate, which adsorbs more NO(2) to facilitate the electron transfer. The fast recovery is due to the smooth surface without pores on TeO(2) nanowires, which may release NO(2) quickly after stopping the gas supply. The present approach for sensing TeO(2) nanowires can be extended to other sensor systems as an efficient, accurate, and low-priced tactic to enhance sensor performance.
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spelling pubmed-106752352023-11-10 Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires Shen, Yunkun Wang, Kaili Liu, Hao Chen, Liping Jin, Zhihan Yan, Shancheng Sensors (Basel) Communication Gas sensors play a pivotal role in environmental monitoring, with NO(2) sensors standing out due to their exceptional selectivity and sensitivity. Yet, a prevalent challenge remains: the prolonged recovery time of many sensors, often spanning hundreds of seconds, compromises efficiency and undermines the precision of continuous detection. This paper introduces an efficient NO(2) sensor using TeO(2) nanowires, offering significantly reduced recovery times. The TeO(2) nanowires, prepared through a straightforward thermal oxidation process, exhibit a unique yet smooth surface. The structural characterizations confirm the formation of pure-phase TeO(2) after the anneal oxidation. TeO(2) nanowires are extremely sensitive to NO(2) gas, and the maximum response (defined as the ratio of resistance in the air to that under the target gas) to NO(2) (10 ppm) is 1.559. In addition, TeO(2) nanowire-based sensors can return to the initial state in about 6–7 s at 100 °C. The high sensitivity can be attributed to the length–diameter rate, which adsorbs more NO(2) to facilitate the electron transfer. The fast recovery is due to the smooth surface without pores on TeO(2) nanowires, which may release NO(2) quickly after stopping the gas supply. The present approach for sensing TeO(2) nanowires can be extended to other sensor systems as an efficient, accurate, and low-priced tactic to enhance sensor performance. MDPI 2023-11-10 /pmc/articles/PMC10675235/ /pubmed/38005485 http://dx.doi.org/10.3390/s23229097 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Communication
Shen, Yunkun
Wang, Kaili
Liu, Hao
Chen, Liping
Jin, Zhihan
Yan, Shancheng
Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires
title Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires
title_full Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires
title_fullStr Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires
title_full_unstemmed Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires
title_short Rapid and Efficient NO(2) Sensing Performance of TeO(2) Nanowires
title_sort rapid and efficient no(2) sensing performance of teo(2) nanowires
topic Communication
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10675235/
https://www.ncbi.nlm.nih.gov/pubmed/38005485
http://dx.doi.org/10.3390/s23229097
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