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Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2)

[Image: see text] Magnetism in reduced dimensionalities is of great fundamental interest while also providing perspectives for applications of materials with novel functionalities. In particular, spin dynamics in two dimensions (2D) have become a focus of recent research. Here, we report the observa...

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Autores principales: Schulz, Frank, Litzius, Kai, Powalla, Lukas, Birch, Max T., Gallardo, Rodolfo A., Satheesh, Sayooj, Weigand, Markus, Scholz, Tanja, Lotsch, Bettina V., Schütz, Gisela, Burghard, Marko, Wintz, Sebastian
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10683057/
https://www.ncbi.nlm.nih.gov/pubmed/37955345
http://dx.doi.org/10.1021/acs.nanolett.3c02212
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author Schulz, Frank
Litzius, Kai
Powalla, Lukas
Birch, Max T.
Gallardo, Rodolfo A.
Satheesh, Sayooj
Weigand, Markus
Scholz, Tanja
Lotsch, Bettina V.
Schütz, Gisela
Burghard, Marko
Wintz, Sebastian
author_facet Schulz, Frank
Litzius, Kai
Powalla, Lukas
Birch, Max T.
Gallardo, Rodolfo A.
Satheesh, Sayooj
Weigand, Markus
Scholz, Tanja
Lotsch, Bettina V.
Schütz, Gisela
Burghard, Marko
Wintz, Sebastian
author_sort Schulz, Frank
collection PubMed
description [Image: see text] Magnetism in reduced dimensionalities is of great fundamental interest while also providing perspectives for applications of materials with novel functionalities. In particular, spin dynamics in two dimensions (2D) have become a focus of recent research. Here, we report the observation of coherent propagating spin-wave dynamics in a ∼30 nm thick flake of 2D van der Waals ferromagnet Fe(5)GeTe(2) using X-ray microscopy. Both phase and amplitude information were obtained by direct imaging below T(C) for frequencies from 2.77 to 3.84 GHz, and the corresponding spin-wave wavelengths were measured to be between 1.5 and 0.5 μm. Thus, parts of the magnonic dispersion relation were determined despite a relatively high magnetic damping of the material. Numerically solving an analytic multilayer model allowed us to corroborate the experimental dispersion relation and predict the influence of changes in the saturation magnetization or interlayer coupling, which could be exploited in future applications by temperature control or stacking of 2D-heterostructures.
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spelling pubmed-106830572023-11-30 Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2) Schulz, Frank Litzius, Kai Powalla, Lukas Birch, Max T. Gallardo, Rodolfo A. Satheesh, Sayooj Weigand, Markus Scholz, Tanja Lotsch, Bettina V. Schütz, Gisela Burghard, Marko Wintz, Sebastian Nano Lett [Image: see text] Magnetism in reduced dimensionalities is of great fundamental interest while also providing perspectives for applications of materials with novel functionalities. In particular, spin dynamics in two dimensions (2D) have become a focus of recent research. Here, we report the observation of coherent propagating spin-wave dynamics in a ∼30 nm thick flake of 2D van der Waals ferromagnet Fe(5)GeTe(2) using X-ray microscopy. Both phase and amplitude information were obtained by direct imaging below T(C) for frequencies from 2.77 to 3.84 GHz, and the corresponding spin-wave wavelengths were measured to be between 1.5 and 0.5 μm. Thus, parts of the magnonic dispersion relation were determined despite a relatively high magnetic damping of the material. Numerically solving an analytic multilayer model allowed us to corroborate the experimental dispersion relation and predict the influence of changes in the saturation magnetization or interlayer coupling, which could be exploited in future applications by temperature control or stacking of 2D-heterostructures. American Chemical Society 2023-11-13 /pmc/articles/PMC10683057/ /pubmed/37955345 http://dx.doi.org/10.1021/acs.nanolett.3c02212 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Schulz, Frank
Litzius, Kai
Powalla, Lukas
Birch, Max T.
Gallardo, Rodolfo A.
Satheesh, Sayooj
Weigand, Markus
Scholz, Tanja
Lotsch, Bettina V.
Schütz, Gisela
Burghard, Marko
Wintz, Sebastian
Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2)
title Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2)
title_full Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2)
title_fullStr Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2)
title_full_unstemmed Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2)
title_short Direct Observation of Propagating Spin Waves in the 2D van der Waals Ferromagnet Fe(5)GeTe(2)
title_sort direct observation of propagating spin waves in the 2d van der waals ferromagnet fe(5)gete(2)
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10683057/
https://www.ncbi.nlm.nih.gov/pubmed/37955345
http://dx.doi.org/10.1021/acs.nanolett.3c02212
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