Cargando…

Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators

[Image: see text] The development of quantum simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. Here we introduce artificial lattices...

Descripción completa

Detalles Bibliográficos
Autores principales: Milloch, Alessandra, Filippi, Umberto, Franceschini, Paolo, Galvani, Michele, Mor, Selene, Pagliara, Stefania, Ferrini, Gabriele, Banfi, Francesco, Capone, Massimo, Baranov, Dmitry, Manna, Liberato, Giannetti, Claudio
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10683068/
https://www.ncbi.nlm.nih.gov/pubmed/37948635
http://dx.doi.org/10.1021/acs.nanolett.3c03715
_version_ 1785151110198067200
author Milloch, Alessandra
Filippi, Umberto
Franceschini, Paolo
Galvani, Michele
Mor, Selene
Pagliara, Stefania
Ferrini, Gabriele
Banfi, Francesco
Capone, Massimo
Baranov, Dmitry
Manna, Liberato
Giannetti, Claudio
author_facet Milloch, Alessandra
Filippi, Umberto
Franceschini, Paolo
Galvani, Michele
Mor, Selene
Pagliara, Stefania
Ferrini, Gabriele
Banfi, Francesco
Capone, Massimo
Baranov, Dmitry
Manna, Liberato
Giannetti, Claudio
author_sort Milloch, Alessandra
collection PubMed
description [Image: see text] The development of quantum simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. Here we introduce artificial lattices made of lead halide perovskite nanocubes as a new platform to simulate and investigate the physics of correlated quantum materials. We demonstrate that optical injection of quantum confined excitons in this system realizes the two main features that ubiquitously pervade the phase diagram of many quantum materials: collective phenomena, in which long-range orders emerge from incoherent fluctuations, and the excitonic Mott transition, which has one-to-one correspondence with the insulator-to-metal transition described by the repulsive Hubbard model in a magnetic field. Our results demonstrate that time-resolved experiments provide a quantum simulator that is able to span a parameter range relevant for a broad class of phenomena, such as superconductivity and charge-density waves.
format Online
Article
Text
id pubmed-10683068
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-106830682023-11-30 Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators Milloch, Alessandra Filippi, Umberto Franceschini, Paolo Galvani, Michele Mor, Selene Pagliara, Stefania Ferrini, Gabriele Banfi, Francesco Capone, Massimo Baranov, Dmitry Manna, Liberato Giannetti, Claudio Nano Lett [Image: see text] The development of quantum simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. Here we introduce artificial lattices made of lead halide perovskite nanocubes as a new platform to simulate and investigate the physics of correlated quantum materials. We demonstrate that optical injection of quantum confined excitons in this system realizes the two main features that ubiquitously pervade the phase diagram of many quantum materials: collective phenomena, in which long-range orders emerge from incoherent fluctuations, and the excitonic Mott transition, which has one-to-one correspondence with the insulator-to-metal transition described by the repulsive Hubbard model in a magnetic field. Our results demonstrate that time-resolved experiments provide a quantum simulator that is able to span a parameter range relevant for a broad class of phenomena, such as superconductivity and charge-density waves. American Chemical Society 2023-11-10 /pmc/articles/PMC10683068/ /pubmed/37948635 http://dx.doi.org/10.1021/acs.nanolett.3c03715 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Milloch, Alessandra
Filippi, Umberto
Franceschini, Paolo
Galvani, Michele
Mor, Selene
Pagliara, Stefania
Ferrini, Gabriele
Banfi, Francesco
Capone, Massimo
Baranov, Dmitry
Manna, Liberato
Giannetti, Claudio
Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators
title Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators
title_full Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators
title_fullStr Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators
title_full_unstemmed Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators
title_short Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators
title_sort halide perovskite artificial solids as a new platform to simulate collective phenomena in doped mott insulators
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10683068/
https://www.ncbi.nlm.nih.gov/pubmed/37948635
http://dx.doi.org/10.1021/acs.nanolett.3c03715
work_keys_str_mv AT millochalessandra halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT filippiumberto halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT franceschinipaolo halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT galvanimichele halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT morselene halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT pagliarastefania halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT ferrinigabriele halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT banfifrancesco halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT caponemassimo halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT baranovdmitry halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT mannaliberato halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators
AT giannetticlaudio halideperovskiteartificialsolidsasanewplatformtosimulatecollectivephenomenaindopedmottinsulators