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Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators
[Image: see text] The development of quantum simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. Here we introduce artificial lattices...
Autores principales: | , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2023
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10683068/ https://www.ncbi.nlm.nih.gov/pubmed/37948635 http://dx.doi.org/10.1021/acs.nanolett.3c03715 |
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author | Milloch, Alessandra Filippi, Umberto Franceschini, Paolo Galvani, Michele Mor, Selene Pagliara, Stefania Ferrini, Gabriele Banfi, Francesco Capone, Massimo Baranov, Dmitry Manna, Liberato Giannetti, Claudio |
author_facet | Milloch, Alessandra Filippi, Umberto Franceschini, Paolo Galvani, Michele Mor, Selene Pagliara, Stefania Ferrini, Gabriele Banfi, Francesco Capone, Massimo Baranov, Dmitry Manna, Liberato Giannetti, Claudio |
author_sort | Milloch, Alessandra |
collection | PubMed |
description | [Image: see text] The development of quantum simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. Here we introduce artificial lattices made of lead halide perovskite nanocubes as a new platform to simulate and investigate the physics of correlated quantum materials. We demonstrate that optical injection of quantum confined excitons in this system realizes the two main features that ubiquitously pervade the phase diagram of many quantum materials: collective phenomena, in which long-range orders emerge from incoherent fluctuations, and the excitonic Mott transition, which has one-to-one correspondence with the insulator-to-metal transition described by the repulsive Hubbard model in a magnetic field. Our results demonstrate that time-resolved experiments provide a quantum simulator that is able to span a parameter range relevant for a broad class of phenomena, such as superconductivity and charge-density waves. |
format | Online Article Text |
id | pubmed-10683068 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-106830682023-11-30 Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators Milloch, Alessandra Filippi, Umberto Franceschini, Paolo Galvani, Michele Mor, Selene Pagliara, Stefania Ferrini, Gabriele Banfi, Francesco Capone, Massimo Baranov, Dmitry Manna, Liberato Giannetti, Claudio Nano Lett [Image: see text] The development of quantum simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. Here we introduce artificial lattices made of lead halide perovskite nanocubes as a new platform to simulate and investigate the physics of correlated quantum materials. We demonstrate that optical injection of quantum confined excitons in this system realizes the two main features that ubiquitously pervade the phase diagram of many quantum materials: collective phenomena, in which long-range orders emerge from incoherent fluctuations, and the excitonic Mott transition, which has one-to-one correspondence with the insulator-to-metal transition described by the repulsive Hubbard model in a magnetic field. Our results demonstrate that time-resolved experiments provide a quantum simulator that is able to span a parameter range relevant for a broad class of phenomena, such as superconductivity and charge-density waves. American Chemical Society 2023-11-10 /pmc/articles/PMC10683068/ /pubmed/37948635 http://dx.doi.org/10.1021/acs.nanolett.3c03715 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Milloch, Alessandra Filippi, Umberto Franceschini, Paolo Galvani, Michele Mor, Selene Pagliara, Stefania Ferrini, Gabriele Banfi, Francesco Capone, Massimo Baranov, Dmitry Manna, Liberato Giannetti, Claudio Halide Perovskite Artificial Solids as a New Platform to Simulate Collective Phenomena in Doped Mott Insulators |
title | Halide Perovskite Artificial Solids as a New Platform
to Simulate Collective Phenomena in Doped Mott Insulators |
title_full | Halide Perovskite Artificial Solids as a New Platform
to Simulate Collective Phenomena in Doped Mott Insulators |
title_fullStr | Halide Perovskite Artificial Solids as a New Platform
to Simulate Collective Phenomena in Doped Mott Insulators |
title_full_unstemmed | Halide Perovskite Artificial Solids as a New Platform
to Simulate Collective Phenomena in Doped Mott Insulators |
title_short | Halide Perovskite Artificial Solids as a New Platform
to Simulate Collective Phenomena in Doped Mott Insulators |
title_sort | halide perovskite artificial solids as a new platform
to simulate collective phenomena in doped mott insulators |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10683068/ https://www.ncbi.nlm.nih.gov/pubmed/37948635 http://dx.doi.org/10.1021/acs.nanolett.3c03715 |
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