Cargando…

Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)

Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV(6)Sn(6) does not feature a magnetic groundstate or excitations, thus it is often regarded...

Descripción completa

Detalles Bibliográficos
Autores principales: Guguchia, Z., Gawryluk, D. J., Shin, S., Hao, Z., Mielke III, C., Das, D., Plokhikh, I., Liborio, L., Shenton, J. Kane, Hu, Y., Sazgari, V., Medarde, M., Deng, H., Cai, Y., Chen, C., Jiang, Y., Amato, A., Shi, M., Hasan, M. Z., Yin, J.-X., Khasanov, R., Pomjakushina, E., Luetkens, H.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10684576/
https://www.ncbi.nlm.nih.gov/pubmed/38016982
http://dx.doi.org/10.1038/s41467-023-43503-9
_version_ 1785151432797716480
author Guguchia, Z.
Gawryluk, D. J.
Shin, S.
Hao, Z.
Mielke III, C.
Das, D.
Plokhikh, I.
Liborio, L.
Shenton, J. Kane
Hu, Y.
Sazgari, V.
Medarde, M.
Deng, H.
Cai, Y.
Chen, C.
Jiang, Y.
Amato, A.
Shi, M.
Hasan, M. Z.
Yin, J.-X.
Khasanov, R.
Pomjakushina, E.
Luetkens, H.
author_facet Guguchia, Z.
Gawryluk, D. J.
Shin, S.
Hao, Z.
Mielke III, C.
Das, D.
Plokhikh, I.
Liborio, L.
Shenton, J. Kane
Hu, Y.
Sazgari, V.
Medarde, M.
Deng, H.
Cai, Y.
Chen, C.
Jiang, Y.
Amato, A.
Shi, M.
Hasan, M. Z.
Yin, J.-X.
Khasanov, R.
Pomjakushina, E.
Luetkens, H.
author_sort Guguchia, Z.
collection PubMed
description Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV(6)Sn(6) does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe an enhancement of the internal field width sensed by the muon ensemble, which takes place within the charge ordered state. More importantly, the muon spin relaxation rate below the charge ordering temperature is substantially enhanced by applying an external magnetic field. Taken together with the hidden magnetism found in AV(3)Sb(5) (A = K, Rb, Cs) and FeGe kagome systems, our results suggest ubiqitous time-reversal symmetry-breaking in charge ordered kagome lattices.
format Online
Article
Text
id pubmed-10684576
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-106845762023-11-30 Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) Guguchia, Z. Gawryluk, D. J. Shin, S. Hao, Z. Mielke III, C. Das, D. Plokhikh, I. Liborio, L. Shenton, J. Kane Hu, Y. Sazgari, V. Medarde, M. Deng, H. Cai, Y. Chen, C. Jiang, Y. Amato, A. Shi, M. Hasan, M. Z. Yin, J.-X. Khasanov, R. Pomjakushina, E. Luetkens, H. Nat Commun Article Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV(6)Sn(6) does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe an enhancement of the internal field width sensed by the muon ensemble, which takes place within the charge ordered state. More importantly, the muon spin relaxation rate below the charge ordering temperature is substantially enhanced by applying an external magnetic field. Taken together with the hidden magnetism found in AV(3)Sb(5) (A = K, Rb, Cs) and FeGe kagome systems, our results suggest ubiqitous time-reversal symmetry-breaking in charge ordered kagome lattices. Nature Publishing Group UK 2023-11-28 /pmc/articles/PMC10684576/ /pubmed/38016982 http://dx.doi.org/10.1038/s41467-023-43503-9 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Guguchia, Z.
Gawryluk, D. J.
Shin, S.
Hao, Z.
Mielke III, C.
Das, D.
Plokhikh, I.
Liborio, L.
Shenton, J. Kane
Hu, Y.
Sazgari, V.
Medarde, M.
Deng, H.
Cai, Y.
Chen, C.
Jiang, Y.
Amato, A.
Shi, M.
Hasan, M. Z.
Yin, J.-X.
Khasanov, R.
Pomjakushina, E.
Luetkens, H.
Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)
title Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)
title_full Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)
title_fullStr Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)
title_full_unstemmed Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)
title_short Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)
title_sort hidden magnetism uncovered in a charge ordered bilayer kagome material scv(6)sn(6)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10684576/
https://www.ncbi.nlm.nih.gov/pubmed/38016982
http://dx.doi.org/10.1038/s41467-023-43503-9
work_keys_str_mv AT guguchiaz hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT gawrylukdj hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT shins hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT haoz hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT mielkeiiic hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT dasd hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT plokhikhi hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT liboriol hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT shentonjkane hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT huy hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT sazgariv hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT medardem hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT dengh hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT caiy hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT chenc hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT jiangy hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT amatoa hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT shim hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT hasanmz hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT yinjx hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT khasanovr hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT pomjakushinae hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6
AT luetkensh hiddenmagnetismuncoveredinachargeorderedbilayerkagomematerialscv6sn6