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Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6)
Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV(6)Sn(6) does not feature a magnetic groundstate or excitations, thus it is often regarded...
Autores principales: | , , , , , , , , , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10684576/ https://www.ncbi.nlm.nih.gov/pubmed/38016982 http://dx.doi.org/10.1038/s41467-023-43503-9 |
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author | Guguchia, Z. Gawryluk, D. J. Shin, S. Hao, Z. Mielke III, C. Das, D. Plokhikh, I. Liborio, L. Shenton, J. Kane Hu, Y. Sazgari, V. Medarde, M. Deng, H. Cai, Y. Chen, C. Jiang, Y. Amato, A. Shi, M. Hasan, M. Z. Yin, J.-X. Khasanov, R. Pomjakushina, E. Luetkens, H. |
author_facet | Guguchia, Z. Gawryluk, D. J. Shin, S. Hao, Z. Mielke III, C. Das, D. Plokhikh, I. Liborio, L. Shenton, J. Kane Hu, Y. Sazgari, V. Medarde, M. Deng, H. Cai, Y. Chen, C. Jiang, Y. Amato, A. Shi, M. Hasan, M. Z. Yin, J.-X. Khasanov, R. Pomjakushina, E. Luetkens, H. |
author_sort | Guguchia, Z. |
collection | PubMed |
description | Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV(6)Sn(6) does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe an enhancement of the internal field width sensed by the muon ensemble, which takes place within the charge ordered state. More importantly, the muon spin relaxation rate below the charge ordering temperature is substantially enhanced by applying an external magnetic field. Taken together with the hidden magnetism found in AV(3)Sb(5) (A = K, Rb, Cs) and FeGe kagome systems, our results suggest ubiqitous time-reversal symmetry-breaking in charge ordered kagome lattices. |
format | Online Article Text |
id | pubmed-10684576 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-106845762023-11-30 Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) Guguchia, Z. Gawryluk, D. J. Shin, S. Hao, Z. Mielke III, C. Das, D. Plokhikh, I. Liborio, L. Shenton, J. Kane Hu, Y. Sazgari, V. Medarde, M. Deng, H. Cai, Y. Chen, C. Jiang, Y. Amato, A. Shi, M. Hasan, M. Z. Yin, J.-X. Khasanov, R. Pomjakushina, E. Luetkens, H. Nat Commun Article Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV(6)Sn(6) does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe an enhancement of the internal field width sensed by the muon ensemble, which takes place within the charge ordered state. More importantly, the muon spin relaxation rate below the charge ordering temperature is substantially enhanced by applying an external magnetic field. Taken together with the hidden magnetism found in AV(3)Sb(5) (A = K, Rb, Cs) and FeGe kagome systems, our results suggest ubiqitous time-reversal symmetry-breaking in charge ordered kagome lattices. Nature Publishing Group UK 2023-11-28 /pmc/articles/PMC10684576/ /pubmed/38016982 http://dx.doi.org/10.1038/s41467-023-43503-9 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Guguchia, Z. Gawryluk, D. J. Shin, S. Hao, Z. Mielke III, C. Das, D. Plokhikh, I. Liborio, L. Shenton, J. Kane Hu, Y. Sazgari, V. Medarde, M. Deng, H. Cai, Y. Chen, C. Jiang, Y. Amato, A. Shi, M. Hasan, M. Z. Yin, J.-X. Khasanov, R. Pomjakushina, E. Luetkens, H. Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) |
title | Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) |
title_full | Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) |
title_fullStr | Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) |
title_full_unstemmed | Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) |
title_short | Hidden magnetism uncovered in a charge ordered bilayer kagome material ScV(6)Sn(6) |
title_sort | hidden magnetism uncovered in a charge ordered bilayer kagome material scv(6)sn(6) |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10684576/ https://www.ncbi.nlm.nih.gov/pubmed/38016982 http://dx.doi.org/10.1038/s41467-023-43503-9 |
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