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Synchrotron Mössbauer spectroscopy using high-speed shutters

A new method of performing Mössbauer spectroscopy with synchrotron radiation is demonstrated that involves using a high-speed periodic shutter near the focal spot of a microfocused X-ray beam. This fast microshuttering technique operates without a high-resolution monochromator and has the potential...

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Detalles Bibliográficos
Autores principales: Toellner, T. S., Alp, E. E., Graber, T., Henning, R. W., Shastri, S. D., Shenoy, G., Sturhahn, W.
Formato: Texto
Lenguaje:English
Publicado: International Union of Crystallography 2011
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3042327/
https://www.ncbi.nlm.nih.gov/pubmed/21335904
http://dx.doi.org/10.1107/S090904951003863X
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author Toellner, T. S.
Alp, E. E.
Graber, T.
Henning, R. W.
Shastri, S. D.
Shenoy, G.
Sturhahn, W.
author_facet Toellner, T. S.
Alp, E. E.
Graber, T.
Henning, R. W.
Shastri, S. D.
Shenoy, G.
Sturhahn, W.
author_sort Toellner, T. S.
collection PubMed
description A new method of performing Mössbauer spectroscopy with synchrotron radiation is demonstrated that involves using a high-speed periodic shutter near the focal spot of a microfocused X-ray beam. This fast microshuttering technique operates without a high-resolution monochromator and has the potential to produce much higher signal rates. It also offers orders of magnitude more suppression of unwanted electronic charge scattering. Measurement results are shown that prove the principle of the method and improvements are discussed to deliver a very pure beam of Mössbauer photons (E/ΔE ≃ 10(12)) with previously unavailable spectral brightness. Such a source will allow both Mössbauer spectroscopy in the energy domain with the many advantageous characteristics of synchrotron radiation and new opportunities for measurements using X-rays with ultra-high energy resolution.
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spelling pubmed-30423272011-03-10 Synchrotron Mössbauer spectroscopy using high-speed shutters Toellner, T. S. Alp, E. E. Graber, T. Henning, R. W. Shastri, S. D. Shenoy, G. Sturhahn, W. J Synchrotron Radiat Research Papers A new method of performing Mössbauer spectroscopy with synchrotron radiation is demonstrated that involves using a high-speed periodic shutter near the focal spot of a microfocused X-ray beam. This fast microshuttering technique operates without a high-resolution monochromator and has the potential to produce much higher signal rates. It also offers orders of magnitude more suppression of unwanted electronic charge scattering. Measurement results are shown that prove the principle of the method and improvements are discussed to deliver a very pure beam of Mössbauer photons (E/ΔE ≃ 10(12)) with previously unavailable spectral brightness. Such a source will allow both Mössbauer spectroscopy in the energy domain with the many advantageous characteristics of synchrotron radiation and new opportunities for measurements using X-rays with ultra-high energy resolution. International Union of Crystallography 2011-03-01 2010-11-23 /pmc/articles/PMC3042327/ /pubmed/21335904 http://dx.doi.org/10.1107/S090904951003863X Text en © T. S. Toellner et al. 2011 http://creativecommons.org/licenses/by/2.0/uk/ This is an open-access article distributed under the terms of the Creative Commons Attribution Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited.
spellingShingle Research Papers
Toellner, T. S.
Alp, E. E.
Graber, T.
Henning, R. W.
Shastri, S. D.
Shenoy, G.
Sturhahn, W.
Synchrotron Mössbauer spectroscopy using high-speed shutters
title Synchrotron Mössbauer spectroscopy using high-speed shutters
title_full Synchrotron Mössbauer spectroscopy using high-speed shutters
title_fullStr Synchrotron Mössbauer spectroscopy using high-speed shutters
title_full_unstemmed Synchrotron Mössbauer spectroscopy using high-speed shutters
title_short Synchrotron Mössbauer spectroscopy using high-speed shutters
title_sort synchrotron mössbauer spectroscopy using high-speed shutters
topic Research Papers
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3042327/
https://www.ncbi.nlm.nih.gov/pubmed/21335904
http://dx.doi.org/10.1107/S090904951003863X
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