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Synchrotron Mössbauer spectroscopy using high-speed shutters
A new method of performing Mössbauer spectroscopy with synchrotron radiation is demonstrated that involves using a high-speed periodic shutter near the focal spot of a microfocused X-ray beam. This fast microshuttering technique operates without a high-resolution monochromator and has the potential...
Autores principales: | , , , , , , |
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Formato: | Texto |
Lenguaje: | English |
Publicado: |
International Union of Crystallography
2011
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3042327/ https://www.ncbi.nlm.nih.gov/pubmed/21335904 http://dx.doi.org/10.1107/S090904951003863X |
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author | Toellner, T. S. Alp, E. E. Graber, T. Henning, R. W. Shastri, S. D. Shenoy, G. Sturhahn, W. |
author_facet | Toellner, T. S. Alp, E. E. Graber, T. Henning, R. W. Shastri, S. D. Shenoy, G. Sturhahn, W. |
author_sort | Toellner, T. S. |
collection | PubMed |
description | A new method of performing Mössbauer spectroscopy with synchrotron radiation is demonstrated that involves using a high-speed periodic shutter near the focal spot of a microfocused X-ray beam. This fast microshuttering technique operates without a high-resolution monochromator and has the potential to produce much higher signal rates. It also offers orders of magnitude more suppression of unwanted electronic charge scattering. Measurement results are shown that prove the principle of the method and improvements are discussed to deliver a very pure beam of Mössbauer photons (E/ΔE ≃ 10(12)) with previously unavailable spectral brightness. Such a source will allow both Mössbauer spectroscopy in the energy domain with the many advantageous characteristics of synchrotron radiation and new opportunities for measurements using X-rays with ultra-high energy resolution. |
format | Text |
id | pubmed-3042327 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2011 |
publisher | International Union of Crystallography |
record_format | MEDLINE/PubMed |
spelling | pubmed-30423272011-03-10 Synchrotron Mössbauer spectroscopy using high-speed shutters Toellner, T. S. Alp, E. E. Graber, T. Henning, R. W. Shastri, S. D. Shenoy, G. Sturhahn, W. J Synchrotron Radiat Research Papers A new method of performing Mössbauer spectroscopy with synchrotron radiation is demonstrated that involves using a high-speed periodic shutter near the focal spot of a microfocused X-ray beam. This fast microshuttering technique operates without a high-resolution monochromator and has the potential to produce much higher signal rates. It also offers orders of magnitude more suppression of unwanted electronic charge scattering. Measurement results are shown that prove the principle of the method and improvements are discussed to deliver a very pure beam of Mössbauer photons (E/ΔE ≃ 10(12)) with previously unavailable spectral brightness. Such a source will allow both Mössbauer spectroscopy in the energy domain with the many advantageous characteristics of synchrotron radiation and new opportunities for measurements using X-rays with ultra-high energy resolution. International Union of Crystallography 2011-03-01 2010-11-23 /pmc/articles/PMC3042327/ /pubmed/21335904 http://dx.doi.org/10.1107/S090904951003863X Text en © T. S. Toellner et al. 2011 http://creativecommons.org/licenses/by/2.0/uk/ This is an open-access article distributed under the terms of the Creative Commons Attribution Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited. |
spellingShingle | Research Papers Toellner, T. S. Alp, E. E. Graber, T. Henning, R. W. Shastri, S. D. Shenoy, G. Sturhahn, W. Synchrotron Mössbauer spectroscopy using high-speed shutters |
title | Synchrotron Mössbauer spectroscopy using high-speed shutters |
title_full | Synchrotron Mössbauer spectroscopy using high-speed shutters |
title_fullStr | Synchrotron Mössbauer spectroscopy using high-speed shutters |
title_full_unstemmed | Synchrotron Mössbauer spectroscopy using high-speed shutters |
title_short | Synchrotron Mössbauer spectroscopy using high-speed shutters |
title_sort | synchrotron mössbauer spectroscopy using high-speed shutters |
topic | Research Papers |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3042327/ https://www.ncbi.nlm.nih.gov/pubmed/21335904 http://dx.doi.org/10.1107/S090904951003863X |
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