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DNA-Controlled Excitonic Switches

[Image: see text] Fluorescence resonance energy transfer (FRET) is a promising means of enabling information processing in nanoscale devices, but dynamic control over exciton pathways is required. Here, we demonstrate the operation of two complementary switches consisting of diffusive FRET transmiss...

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Autores principales: Graugnard, Elton, Kellis, Donald L., Bui, Hieu, Barnes, Stephanie, Kuang, Wan, Lee, Jeunghoon, Hughes, William L., Knowlton, William B., Yurke, Bernard
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2012
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3324986/
https://www.ncbi.nlm.nih.gov/pubmed/22401838
http://dx.doi.org/10.1021/nl3004336
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author Graugnard, Elton
Kellis, Donald L.
Bui, Hieu
Barnes, Stephanie
Kuang, Wan
Lee, Jeunghoon
Hughes, William L.
Knowlton, William B.
Yurke, Bernard
author_facet Graugnard, Elton
Kellis, Donald L.
Bui, Hieu
Barnes, Stephanie
Kuang, Wan
Lee, Jeunghoon
Hughes, William L.
Knowlton, William B.
Yurke, Bernard
author_sort Graugnard, Elton
collection PubMed
description [Image: see text] Fluorescence resonance energy transfer (FRET) is a promising means of enabling information processing in nanoscale devices, but dynamic control over exciton pathways is required. Here, we demonstrate the operation of two complementary switches consisting of diffusive FRET transmission lines in which exciton flow is controlled by DNA. Repeatable switching is accomplished by the removal or addition of fluorophores through toehold-mediated strand invasion. In principle, these switches can be networked to implement any Boolean function.
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spelling pubmed-33249862012-04-13 DNA-Controlled Excitonic Switches Graugnard, Elton Kellis, Donald L. Bui, Hieu Barnes, Stephanie Kuang, Wan Lee, Jeunghoon Hughes, William L. Knowlton, William B. Yurke, Bernard Nano Lett [Image: see text] Fluorescence resonance energy transfer (FRET) is a promising means of enabling information processing in nanoscale devices, but dynamic control over exciton pathways is required. Here, we demonstrate the operation of two complementary switches consisting of diffusive FRET transmission lines in which exciton flow is controlled by DNA. Repeatable switching is accomplished by the removal or addition of fluorophores through toehold-mediated strand invasion. In principle, these switches can be networked to implement any Boolean function. American Chemical Society 2012-03-08 2012-04-11 /pmc/articles/PMC3324986/ /pubmed/22401838 http://dx.doi.org/10.1021/nl3004336 Text en Copyright © 2012 American Chemical Society http://pubs.acs.org This is an open-access article distributed under the ACS AuthorChoice Terms & Conditions. Any use of this article, must conform to the terms of that license which are available at http://pubs.acs.org.
spellingShingle Graugnard, Elton
Kellis, Donald L.
Bui, Hieu
Barnes, Stephanie
Kuang, Wan
Lee, Jeunghoon
Hughes, William L.
Knowlton, William B.
Yurke, Bernard
DNA-Controlled Excitonic Switches
title DNA-Controlled Excitonic Switches
title_full DNA-Controlled Excitonic Switches
title_fullStr DNA-Controlled Excitonic Switches
title_full_unstemmed DNA-Controlled Excitonic Switches
title_short DNA-Controlled Excitonic Switches
title_sort dna-controlled excitonic switches
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3324986/
https://www.ncbi.nlm.nih.gov/pubmed/22401838
http://dx.doi.org/10.1021/nl3004336
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