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Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots
We have theoretically studied the thermoelectric properties of serially coupled quantum dots (SCQDs) embedded in an insulator connected to metallic electrodes. In the framework of Keldysh Green’s function technique, the Landauer formula of transmission factor is obtained using the equation of motion...
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Springer
2012
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3505148/ https://www.ncbi.nlm.nih.gov/pubmed/22591807 http://dx.doi.org/10.1186/1556-276X-7-257 |
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author | T Kuo, David M Chang, Yia-Chung |
author_facet | T Kuo, David M Chang, Yia-Chung |
author_sort | T Kuo, David M |
collection | PubMed |
description | We have theoretically studied the thermoelectric properties of serially coupled quantum dots (SCQDs) embedded in an insulator connected to metallic electrodes. In the framework of Keldysh Green’s function technique, the Landauer formula of transmission factor is obtained using the equation of motion method. Based on such analytical expressions of charge and heat currents, we calculate the electrical conductance, Seebeck coefficient, electron thermal conductance, and figure of merit (ZT) of SCQDs in the linear response regime. The effects of interdot hopping and electron Coulomb interactions on ZT are analyzed. We demonstrate that ZT is not a monotonic increasing function of interdot electron hopping strength (t(c)). We also show that in the absence of phonon thermal conductance, SCQD can reach the Carnot efficiency as t(c)approaches zero. |
format | Online Article Text |
id | pubmed-3505148 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2012 |
publisher | Springer |
record_format | MEDLINE/PubMed |
spelling | pubmed-35051482012-12-05 Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots T Kuo, David M Chang, Yia-Chung Nanoscale Res Lett Nano Review We have theoretically studied the thermoelectric properties of serially coupled quantum dots (SCQDs) embedded in an insulator connected to metallic electrodes. In the framework of Keldysh Green’s function technique, the Landauer formula of transmission factor is obtained using the equation of motion method. Based on such analytical expressions of charge and heat currents, we calculate the electrical conductance, Seebeck coefficient, electron thermal conductance, and figure of merit (ZT) of SCQDs in the linear response regime. The effects of interdot hopping and electron Coulomb interactions on ZT are analyzed. We demonstrate that ZT is not a monotonic increasing function of interdot electron hopping strength (t(c)). We also show that in the absence of phonon thermal conductance, SCQD can reach the Carnot efficiency as t(c)approaches zero. Springer 2012-05-16 /pmc/articles/PMC3505148/ /pubmed/22591807 http://dx.doi.org/10.1186/1556-276X-7-257 Text en Copyright ©2012 Kuo and Chang; licensee Springer. http://creativecommons.org/licenses/by/2.0 This is an Open Access article distributed under the terms of the Creative Commons Attribution License ( http://creativecommons.org/licenses/by/2.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. |
spellingShingle | Nano Review T Kuo, David M Chang, Yia-Chung Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots |
title | Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots |
title_full | Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots |
title_fullStr | Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots |
title_full_unstemmed | Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots |
title_short | Effects of interdot hopping and Coulomb blockade on the thermoelectric properties of serially coupled quantum dots |
title_sort | effects of interdot hopping and coulomb blockade on the thermoelectric properties of serially coupled quantum dots |
topic | Nano Review |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3505148/ https://www.ncbi.nlm.nih.gov/pubmed/22591807 http://dx.doi.org/10.1186/1556-276X-7-257 |
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