Dark Plasmonic Breathing Modes in Silver Nanodisks

[Image: see text] We map the complete plasmonic spectrum of silver nanodisks by electron energy loss spectroscopy and show that the mode which couples strongest to the electron beam has radial symmetry with no net dipole moment. Therefore, this mode does not couple to light and has escaped from obse...

Descripción completa

Detalles Bibliográficos
Autores principales: Schmidt, Franz-Philipp, Ditlbacher, Harald, Hohenester, Ulrich, Hohenau, Andreas, Hofer, Ferdinand, Krenn, Joachim R.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2012
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3558010/
https://www.ncbi.nlm.nih.gov/pubmed/23025804
http://dx.doi.org/10.1021/nl3030938
_version_ 1782257369927909376
author Schmidt, Franz-Philipp
Ditlbacher, Harald
Hohenester, Ulrich
Hohenau, Andreas
Hofer, Ferdinand
Krenn, Joachim R.
author_facet Schmidt, Franz-Philipp
Ditlbacher, Harald
Hohenester, Ulrich
Hohenau, Andreas
Hofer, Ferdinand
Krenn, Joachim R.
author_sort Schmidt, Franz-Philipp
collection PubMed
description [Image: see text] We map the complete plasmonic spectrum of silver nanodisks by electron energy loss spectroscopy and show that the mode which couples strongest to the electron beam has radial symmetry with no net dipole moment. Therefore, this mode does not couple to light and has escaped from observation in optical experiments. This radial breathing mode has the character of an extended two-dimensional surface plasmon with a wavenumber determined by the circular disk confinement. Its strong near fields can impact the hybridization in coupled plasmonic nanoparticles as well as couplings with nearby quantum emitters.
format Online
Article
Text
id pubmed-3558010
institution National Center for Biotechnology Information
language English
publishDate 2012
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-35580102013-01-31 Dark Plasmonic Breathing Modes in Silver Nanodisks Schmidt, Franz-Philipp Ditlbacher, Harald Hohenester, Ulrich Hohenau, Andreas Hofer, Ferdinand Krenn, Joachim R. Nano Lett [Image: see text] We map the complete plasmonic spectrum of silver nanodisks by electron energy loss spectroscopy and show that the mode which couples strongest to the electron beam has radial symmetry with no net dipole moment. Therefore, this mode does not couple to light and has escaped from observation in optical experiments. This radial breathing mode has the character of an extended two-dimensional surface plasmon with a wavenumber determined by the circular disk confinement. Its strong near fields can impact the hybridization in coupled plasmonic nanoparticles as well as couplings with nearby quantum emitters. American Chemical Society 2012-10-01 2012-11-14 /pmc/articles/PMC3558010/ /pubmed/23025804 http://dx.doi.org/10.1021/nl3030938 Text en Copyright © 2012 American Chemical Society Terms of Use (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html)
spellingShingle Schmidt, Franz-Philipp
Ditlbacher, Harald
Hohenester, Ulrich
Hohenau, Andreas
Hofer, Ferdinand
Krenn, Joachim R.
Dark Plasmonic Breathing Modes in Silver Nanodisks
title Dark Plasmonic Breathing Modes in Silver Nanodisks
title_full Dark Plasmonic Breathing Modes in Silver Nanodisks
title_fullStr Dark Plasmonic Breathing Modes in Silver Nanodisks
title_full_unstemmed Dark Plasmonic Breathing Modes in Silver Nanodisks
title_short Dark Plasmonic Breathing Modes in Silver Nanodisks
title_sort dark plasmonic breathing modes in silver nanodisks
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3558010/
https://www.ncbi.nlm.nih.gov/pubmed/23025804
http://dx.doi.org/10.1021/nl3030938
work_keys_str_mv AT schmidtfranzphilipp darkplasmonicbreathingmodesinsilvernanodisks
AT ditlbacherharald darkplasmonicbreathingmodesinsilvernanodisks
AT hohenesterulrich darkplasmonicbreathingmodesinsilvernanodisks
AT hohenauandreas darkplasmonicbreathingmodesinsilvernanodisks
AT hoferferdinand darkplasmonicbreathingmodesinsilvernanodisks
AT krennjoachimr darkplasmonicbreathingmodesinsilvernanodisks

Ejemplares similares