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Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles

[Image: see text] We demonstrate the ultrafast generation of electrons from tailored metallic nanoparticles and unravel the role of plasmonic field enhancement in this process by comparing resonant and off-resonant particles, as well as different particle geometries. We find that electrons become st...

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Detalles Bibliográficos
Autores principales: Dombi, Péter, Hörl, Anton, Rácz, Péter, Márton, István, Trügler, Andreas, Krenn, Joachim R., Hohenester, Ulrich
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2013
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3573732/
https://www.ncbi.nlm.nih.gov/pubmed/23339740
http://dx.doi.org/10.1021/nl304365e
Descripción
Sumario:[Image: see text] We demonstrate the ultrafast generation of electrons from tailored metallic nanoparticles and unravel the role of plasmonic field enhancement in this process by comparing resonant and off-resonant particles, as well as different particle geometries. We find that electrons become strongly accelerated within the evanescent fields of the plasmonic nanoparticles and escape along straight trajectories with orientations governed by the particle geometry. These results establish plasmonic nanoparticles as versatile ultrafast, nanoscopic sources of electrons.