Cargando…

Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles

[Image: see text] We demonstrate the ultrafast generation of electrons from tailored metallic nanoparticles and unravel the role of plasmonic field enhancement in this process by comparing resonant and off-resonant particles, as well as different particle geometries. We find that electrons become st...

Descripción completa

Detalles Bibliográficos
Autores principales: Dombi, Péter, Hörl, Anton, Rácz, Péter, Márton, István, Trügler, Andreas, Krenn, Joachim R., Hohenester, Ulrich
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2013
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3573732/
https://www.ncbi.nlm.nih.gov/pubmed/23339740
http://dx.doi.org/10.1021/nl304365e
_version_ 1782259490604711936
author Dombi, Péter
Hörl, Anton
Rácz, Péter
Márton, István
Trügler, Andreas
Krenn, Joachim R.
Hohenester, Ulrich
author_facet Dombi, Péter
Hörl, Anton
Rácz, Péter
Márton, István
Trügler, Andreas
Krenn, Joachim R.
Hohenester, Ulrich
author_sort Dombi, Péter
collection PubMed
description [Image: see text] We demonstrate the ultrafast generation of electrons from tailored metallic nanoparticles and unravel the role of plasmonic field enhancement in this process by comparing resonant and off-resonant particles, as well as different particle geometries. We find that electrons become strongly accelerated within the evanescent fields of the plasmonic nanoparticles and escape along straight trajectories with orientations governed by the particle geometry. These results establish plasmonic nanoparticles as versatile ultrafast, nanoscopic sources of electrons.
format Online
Article
Text
id pubmed-3573732
institution National Center for Biotechnology Information
language English
publishDate 2013
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-35737322013-02-19 Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles Dombi, Péter Hörl, Anton Rácz, Péter Márton, István Trügler, Andreas Krenn, Joachim R. Hohenester, Ulrich Nano Lett [Image: see text] We demonstrate the ultrafast generation of electrons from tailored metallic nanoparticles and unravel the role of plasmonic field enhancement in this process by comparing resonant and off-resonant particles, as well as different particle geometries. We find that electrons become strongly accelerated within the evanescent fields of the plasmonic nanoparticles and escape along straight trajectories with orientations governed by the particle geometry. These results establish plasmonic nanoparticles as versatile ultrafast, nanoscopic sources of electrons. American Chemical Society 2013-01-22 2013-02-13 /pmc/articles/PMC3573732/ /pubmed/23339740 http://dx.doi.org/10.1021/nl304365e Text en Copyright © 2013 American Chemical Society Terms of Use (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html)
spellingShingle Dombi, Péter
Hörl, Anton
Rácz, Péter
Márton, István
Trügler, Andreas
Krenn, Joachim R.
Hohenester, Ulrich
Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles
title Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles
title_full Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles
title_fullStr Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles
title_full_unstemmed Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles
title_short Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles
title_sort ultrafast strong-field photoemission from plasmonic nanoparticles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3573732/
https://www.ncbi.nlm.nih.gov/pubmed/23339740
http://dx.doi.org/10.1021/nl304365e
work_keys_str_mv AT dombipeter ultrafaststrongfieldphotoemissionfromplasmonicnanoparticles
AT horlanton ultrafaststrongfieldphotoemissionfromplasmonicnanoparticles
AT raczpeter ultrafaststrongfieldphotoemissionfromplasmonicnanoparticles
AT martonistvan ultrafaststrongfieldphotoemissionfromplasmonicnanoparticles
AT truglerandreas ultrafaststrongfieldphotoemissionfromplasmonicnanoparticles
AT krennjoachimr ultrafaststrongfieldphotoemissionfromplasmonicnanoparticles
AT hohenesterulrich ultrafaststrongfieldphotoemissionfromplasmonicnanoparticles