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Quasiparticles and Fermi liquid behaviour in an organic metal

Many organic metals display exotic properties such as superconductivity, spin-charge separation and so on and have been described as quasi-one-dimensional Luttinger liquids. However, a genuine Fermi liquid behaviour with quasiparticles and Fermi surfaces have not been reported to date for any organi...

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Autores principales: Kiss, T., Chainani, A., Yamamoto, H.M., Miyazaki, T., Akimoto, T., Shimojima, T., Ishizaka, K., Watanabe, S., Chen, C.-T., Fukaya, A., Kato, R., Shin, S.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Pub. Group 2012
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3658098/
https://www.ncbi.nlm.nih.gov/pubmed/23011143
http://dx.doi.org/10.1038/ncomms2079
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author Kiss, T.
Chainani, A.
Yamamoto, H.M.
Miyazaki, T.
Akimoto, T.
Shimojima, T.
Ishizaka, K.
Watanabe, S.
Chen, C.-T.
Fukaya, A.
Kato, R.
Shin, S.
author_facet Kiss, T.
Chainani, A.
Yamamoto, H.M.
Miyazaki, T.
Akimoto, T.
Shimojima, T.
Ishizaka, K.
Watanabe, S.
Chen, C.-T.
Fukaya, A.
Kato, R.
Shin, S.
author_sort Kiss, T.
collection PubMed
description Many organic metals display exotic properties such as superconductivity, spin-charge separation and so on and have been described as quasi-one-dimensional Luttinger liquids. However, a genuine Fermi liquid behaviour with quasiparticles and Fermi surfaces have not been reported to date for any organic metal. Here, we report the experimental Fermi surface and band structure of an organic metal (BEDT-TTF)(3)Br(pBIB) obtained using angle-resolved photoelectron spectroscopy, and show its consistency with first-principles band structure calculations. Our results reveal a quasiparticle renormalization at low energy scales (effective mass m*=1.9 m(e)) and ω(2) dependence of the imaginary part of the self energy, limited by a kink at ~50 meV arising from coupling to molecular vibrations. The study unambiguously proves that (BEDT-TTF)(3)Br(pBIB) is a quasi-2D organic Fermi liquid with a Fermi surface consistent with Shubnikov-de Haas results.
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spelling pubmed-36580982013-05-20 Quasiparticles and Fermi liquid behaviour in an organic metal Kiss, T. Chainani, A. Yamamoto, H.M. Miyazaki, T. Akimoto, T. Shimojima, T. Ishizaka, K. Watanabe, S. Chen, C.-T. Fukaya, A. Kato, R. Shin, S. Nat Commun Article Many organic metals display exotic properties such as superconductivity, spin-charge separation and so on and have been described as quasi-one-dimensional Luttinger liquids. However, a genuine Fermi liquid behaviour with quasiparticles and Fermi surfaces have not been reported to date for any organic metal. Here, we report the experimental Fermi surface and band structure of an organic metal (BEDT-TTF)(3)Br(pBIB) obtained using angle-resolved photoelectron spectroscopy, and show its consistency with first-principles band structure calculations. Our results reveal a quasiparticle renormalization at low energy scales (effective mass m*=1.9 m(e)) and ω(2) dependence of the imaginary part of the self energy, limited by a kink at ~50 meV arising from coupling to molecular vibrations. The study unambiguously proves that (BEDT-TTF)(3)Br(pBIB) is a quasi-2D organic Fermi liquid with a Fermi surface consistent with Shubnikov-de Haas results. Nature Pub. Group 2012-09-25 /pmc/articles/PMC3658098/ /pubmed/23011143 http://dx.doi.org/10.1038/ncomms2079 Text en Copyright © 2012, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by-nc-sa/3.0/ This work is licensed under a Creative Commons Attribution-NonCommercial-Share Alike 3.0 Unported License. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-sa/3.0/
spellingShingle Article
Kiss, T.
Chainani, A.
Yamamoto, H.M.
Miyazaki, T.
Akimoto, T.
Shimojima, T.
Ishizaka, K.
Watanabe, S.
Chen, C.-T.
Fukaya, A.
Kato, R.
Shin, S.
Quasiparticles and Fermi liquid behaviour in an organic metal
title Quasiparticles and Fermi liquid behaviour in an organic metal
title_full Quasiparticles and Fermi liquid behaviour in an organic metal
title_fullStr Quasiparticles and Fermi liquid behaviour in an organic metal
title_full_unstemmed Quasiparticles and Fermi liquid behaviour in an organic metal
title_short Quasiparticles and Fermi liquid behaviour in an organic metal
title_sort quasiparticles and fermi liquid behaviour in an organic metal
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3658098/
https://www.ncbi.nlm.nih.gov/pubmed/23011143
http://dx.doi.org/10.1038/ncomms2079
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