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A full-sunlight-driven photocatalyst with super long-persistent energy storage ability

A major drawback of traditional photocatalysts like TiO(2) is that they can only work under illumination, and the light has to be UV. As a solution for this limitation, visible-light-driven energy storage photocatalysts have been developed in recent years. However, energy storage photocatalysts that...

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Autores principales: Li, Jie, Liu, Yuan, Zhu, Zhijian, Zhang, Guozhu, Zou, Tao, Zou, Zhijun, Zhang, Shunping, Zeng, Dawen, Xie, Changsheng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2013
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3740289/
https://www.ncbi.nlm.nih.gov/pubmed/23934407
http://dx.doi.org/10.1038/srep02409
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author Li, Jie
Liu, Yuan
Zhu, Zhijian
Zhang, Guozhu
Zou, Tao
Zou, Zhijun
Zhang, Shunping
Zeng, Dawen
Xie, Changsheng
author_facet Li, Jie
Liu, Yuan
Zhu, Zhijian
Zhang, Guozhu
Zou, Tao
Zou, Zhijun
Zhang, Shunping
Zeng, Dawen
Xie, Changsheng
author_sort Li, Jie
collection PubMed
description A major drawback of traditional photocatalysts like TiO(2) is that they can only work under illumination, and the light has to be UV. As a solution for this limitation, visible-light-driven energy storage photocatalysts have been developed in recent years. However, energy storage photocatalysts that are full-sunlight-driven (UV-visible-NIR) and possess long-lasting energy storage ability are lacking. Here we report, a Pt-loaded and hydrogen-treated WO(3) that exhibits a strong absorption at full-sunlight spectrum (300–1,000 nm), and with a super-long energy storage time of more than 300 h to have formaldehyde degraded in dark. In this new material system, the hydrogen treated WO(3) functions as the light harvesting material and energy storage material simultaneously, while Pt mainly acts as the cocatalyst to have the energy storage effect displayed. The extraordinary full-spectrum absorption effect and long persistent energy storage ability make the material a potential solar-energy storage and an effective photocatalyst in practice.
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spelling pubmed-37402892013-08-12 A full-sunlight-driven photocatalyst with super long-persistent energy storage ability Li, Jie Liu, Yuan Zhu, Zhijian Zhang, Guozhu Zou, Tao Zou, Zhijun Zhang, Shunping Zeng, Dawen Xie, Changsheng Sci Rep Article A major drawback of traditional photocatalysts like TiO(2) is that they can only work under illumination, and the light has to be UV. As a solution for this limitation, visible-light-driven energy storage photocatalysts have been developed in recent years. However, energy storage photocatalysts that are full-sunlight-driven (UV-visible-NIR) and possess long-lasting energy storage ability are lacking. Here we report, a Pt-loaded and hydrogen-treated WO(3) that exhibits a strong absorption at full-sunlight spectrum (300–1,000 nm), and with a super-long energy storage time of more than 300 h to have formaldehyde degraded in dark. In this new material system, the hydrogen treated WO(3) functions as the light harvesting material and energy storage material simultaneously, while Pt mainly acts as the cocatalyst to have the energy storage effect displayed. The extraordinary full-spectrum absorption effect and long persistent energy storage ability make the material a potential solar-energy storage and an effective photocatalyst in practice. Nature Publishing Group 2013-08-12 /pmc/articles/PMC3740289/ /pubmed/23934407 http://dx.doi.org/10.1038/srep02409 Text en Copyright © 2013, Macmillan Publishers Limited. All rights reserved http://creativecommons.org/licenses/by-nc-nd/3.0/ This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivs 3.0 Unported License. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-nd/3.0/
spellingShingle Article
Li, Jie
Liu, Yuan
Zhu, Zhijian
Zhang, Guozhu
Zou, Tao
Zou, Zhijun
Zhang, Shunping
Zeng, Dawen
Xie, Changsheng
A full-sunlight-driven photocatalyst with super long-persistent energy storage ability
title A full-sunlight-driven photocatalyst with super long-persistent energy storage ability
title_full A full-sunlight-driven photocatalyst with super long-persistent energy storage ability
title_fullStr A full-sunlight-driven photocatalyst with super long-persistent energy storage ability
title_full_unstemmed A full-sunlight-driven photocatalyst with super long-persistent energy storage ability
title_short A full-sunlight-driven photocatalyst with super long-persistent energy storage ability
title_sort full-sunlight-driven photocatalyst with super long-persistent energy storage ability
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3740289/
https://www.ncbi.nlm.nih.gov/pubmed/23934407
http://dx.doi.org/10.1038/srep02409
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