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Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature
Room temperature catalytic oxidation by noble metals is considered to be the most promising strategy for the removal of HCHO, which is one of the major indoor air pollutants. Hierarchically macro-mesoporous structured Pt/γ-Al(2)O(3) hollow spheres with open and accessible pores were synthesized and...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group
2013
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3827609/ https://www.ncbi.nlm.nih.gov/pubmed/24225532 http://dx.doi.org/10.1038/srep03215 |
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author | Nie, Longhui Meng, Aiyun Yu, Jiaguo Jaroniec, Mietek |
author_facet | Nie, Longhui Meng, Aiyun Yu, Jiaguo Jaroniec, Mietek |
author_sort | Nie, Longhui |
collection | PubMed |
description | Room temperature catalytic oxidation by noble metals is considered to be the most promising strategy for the removal of HCHO, which is one of the major indoor air pollutants. Hierarchically macro-mesoporous structured Pt/γ-Al(2)O(3) hollow spheres with open and accessible pores were synthesized and used for catalytic oxidative decomposition of HCHO at room temperature. The prepared composite hollow spheres showed higher catalytic activity than the conventional nanoparticle supports, which is mainly due to their hierarchical macro-mesoporous structure facilitating diffusion of reactants and products, and the high dispersion of accessible catalytic Pt nanoparticles. This work may contribute to the development of hierarchically structured materials and high-performance catalysts for indoor air purification and related catalytic processes. |
format | Online Article Text |
id | pubmed-3827609 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2013 |
publisher | Nature Publishing Group |
record_format | MEDLINE/PubMed |
spelling | pubmed-38276092013-11-15 Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature Nie, Longhui Meng, Aiyun Yu, Jiaguo Jaroniec, Mietek Sci Rep Article Room temperature catalytic oxidation by noble metals is considered to be the most promising strategy for the removal of HCHO, which is one of the major indoor air pollutants. Hierarchically macro-mesoporous structured Pt/γ-Al(2)O(3) hollow spheres with open and accessible pores were synthesized and used for catalytic oxidative decomposition of HCHO at room temperature. The prepared composite hollow spheres showed higher catalytic activity than the conventional nanoparticle supports, which is mainly due to their hierarchical macro-mesoporous structure facilitating diffusion of reactants and products, and the high dispersion of accessible catalytic Pt nanoparticles. This work may contribute to the development of hierarchically structured materials and high-performance catalysts for indoor air purification and related catalytic processes. Nature Publishing Group 2013-11-14 /pmc/articles/PMC3827609/ /pubmed/24225532 http://dx.doi.org/10.1038/srep03215 Text en Copyright © 2013, Macmillan Publishers Limited. All rights reserved http://creativecommons.org/licenses/by-nc-nd/3.0/ This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivs 3.0 Unported License. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-nd/3.0/ |
spellingShingle | Article Nie, Longhui Meng, Aiyun Yu, Jiaguo Jaroniec, Mietek Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature |
title | Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature |
title_full | Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature |
title_fullStr | Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature |
title_full_unstemmed | Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature |
title_short | Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature |
title_sort | hierarchically macro-mesoporous pt/γ-al(2)o(3) composite microspheres for efficient formaldehyde oxidation at room temperature |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3827609/ https://www.ncbi.nlm.nih.gov/pubmed/24225532 http://dx.doi.org/10.1038/srep03215 |
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