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Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature

Room temperature catalytic oxidation by noble metals is considered to be the most promising strategy for the removal of HCHO, which is one of the major indoor air pollutants. Hierarchically macro-mesoporous structured Pt/γ-Al(2)O(3) hollow spheres with open and accessible pores were synthesized and...

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Detalles Bibliográficos
Autores principales: Nie, Longhui, Meng, Aiyun, Yu, Jiaguo, Jaroniec, Mietek
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2013
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3827609/
https://www.ncbi.nlm.nih.gov/pubmed/24225532
http://dx.doi.org/10.1038/srep03215
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author Nie, Longhui
Meng, Aiyun
Yu, Jiaguo
Jaroniec, Mietek
author_facet Nie, Longhui
Meng, Aiyun
Yu, Jiaguo
Jaroniec, Mietek
author_sort Nie, Longhui
collection PubMed
description Room temperature catalytic oxidation by noble metals is considered to be the most promising strategy for the removal of HCHO, which is one of the major indoor air pollutants. Hierarchically macro-mesoporous structured Pt/γ-Al(2)O(3) hollow spheres with open and accessible pores were synthesized and used for catalytic oxidative decomposition of HCHO at room temperature. The prepared composite hollow spheres showed higher catalytic activity than the conventional nanoparticle supports, which is mainly due to their hierarchical macro-mesoporous structure facilitating diffusion of reactants and products, and the high dispersion of accessible catalytic Pt nanoparticles. This work may contribute to the development of hierarchically structured materials and high-performance catalysts for indoor air purification and related catalytic processes.
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spelling pubmed-38276092013-11-15 Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature Nie, Longhui Meng, Aiyun Yu, Jiaguo Jaroniec, Mietek Sci Rep Article Room temperature catalytic oxidation by noble metals is considered to be the most promising strategy for the removal of HCHO, which is one of the major indoor air pollutants. Hierarchically macro-mesoporous structured Pt/γ-Al(2)O(3) hollow spheres with open and accessible pores were synthesized and used for catalytic oxidative decomposition of HCHO at room temperature. The prepared composite hollow spheres showed higher catalytic activity than the conventional nanoparticle supports, which is mainly due to their hierarchical macro-mesoporous structure facilitating diffusion of reactants and products, and the high dispersion of accessible catalytic Pt nanoparticles. This work may contribute to the development of hierarchically structured materials and high-performance catalysts for indoor air purification and related catalytic processes. Nature Publishing Group 2013-11-14 /pmc/articles/PMC3827609/ /pubmed/24225532 http://dx.doi.org/10.1038/srep03215 Text en Copyright © 2013, Macmillan Publishers Limited. All rights reserved http://creativecommons.org/licenses/by-nc-nd/3.0/ This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivs 3.0 Unported License. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-nd/3.0/
spellingShingle Article
Nie, Longhui
Meng, Aiyun
Yu, Jiaguo
Jaroniec, Mietek
Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature
title Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature
title_full Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature
title_fullStr Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature
title_full_unstemmed Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature
title_short Hierarchically Macro-Mesoporous Pt/γ-Al(2)O(3) Composite Microspheres for Efficient Formaldehyde Oxidation at Room Temperature
title_sort hierarchically macro-mesoporous pt/γ-al(2)o(3) composite microspheres for efficient formaldehyde oxidation at room temperature
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3827609/
https://www.ncbi.nlm.nih.gov/pubmed/24225532
http://dx.doi.org/10.1038/srep03215
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