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All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters

White quantum dot light-emitting diodes (QD-LEDs) have been a promising candidate for high-efficiency and color-saturated displays. However, it is challenging to integrate various QD emitters into one device and also to obtain efficient blue QDs. Here, we report a simply solution-processed white QD-...

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Autores principales: Chen, Jing, Zhao, Dewei, Li, Chi, Xu, Feng, Lei, Wei, Sun, Litao, Nathan, Arokia, Sun, Xiao Wei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2014
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3923213/
https://www.ncbi.nlm.nih.gov/pubmed/24522341
http://dx.doi.org/10.1038/srep04085
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author Chen, Jing
Zhao, Dewei
Li, Chi
Xu, Feng
Lei, Wei
Sun, Litao
Nathan, Arokia
Sun, Xiao Wei
author_facet Chen, Jing
Zhao, Dewei
Li, Chi
Xu, Feng
Lei, Wei
Sun, Litao
Nathan, Arokia
Sun, Xiao Wei
author_sort Chen, Jing
collection PubMed
description White quantum dot light-emitting diodes (QD-LEDs) have been a promising candidate for high-efficiency and color-saturated displays. However, it is challenging to integrate various QD emitters into one device and also to obtain efficient blue QDs. Here, we report a simply solution-processed white QD-LED using a hybrid ZnO@TiO(2) as electron injection layer and ZnCdSeS QD emitters. The white emission is obtained by integrating the yellow emission from QD emitters and the blue emission generated from hybrid ZnO@TiO(2) layer. We show that the performance of white QD-LEDs can be adjusted by controlling the driving force for hole transport and electroluminescence recombination region via varying the thickness of hole transport layer. The device is demonstrated with a maximum luminance of 730 cd/m(2) and power efficiency of 1.7 lm/W, exhibiting the Commission Internationale de l'Enclairage (CIE) coordinates of (0.33, 0.33). The unencapsulated white QD-LED has a long lifetime of 96 h at its initial luminance of 730 cd/m(2), primarily due to the fact that the device with hybrid ZnO@TiO(2) has low leakage current and is insensitive to the oxygen and the moisture. These results indicate that hybrid ZnO@TiO(2) provides an alternate and effective approach to achieve high-performance white QD-LEDs and also other optoelectronic devices.
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spelling pubmed-39232132014-02-13 All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters Chen, Jing Zhao, Dewei Li, Chi Xu, Feng Lei, Wei Sun, Litao Nathan, Arokia Sun, Xiao Wei Sci Rep Article White quantum dot light-emitting diodes (QD-LEDs) have been a promising candidate for high-efficiency and color-saturated displays. However, it is challenging to integrate various QD emitters into one device and also to obtain efficient blue QDs. Here, we report a simply solution-processed white QD-LED using a hybrid ZnO@TiO(2) as electron injection layer and ZnCdSeS QD emitters. The white emission is obtained by integrating the yellow emission from QD emitters and the blue emission generated from hybrid ZnO@TiO(2) layer. We show that the performance of white QD-LEDs can be adjusted by controlling the driving force for hole transport and electroluminescence recombination region via varying the thickness of hole transport layer. The device is demonstrated with a maximum luminance of 730 cd/m(2) and power efficiency of 1.7 lm/W, exhibiting the Commission Internationale de l'Enclairage (CIE) coordinates of (0.33, 0.33). The unencapsulated white QD-LED has a long lifetime of 96 h at its initial luminance of 730 cd/m(2), primarily due to the fact that the device with hybrid ZnO@TiO(2) has low leakage current and is insensitive to the oxygen and the moisture. These results indicate that hybrid ZnO@TiO(2) provides an alternate and effective approach to achieve high-performance white QD-LEDs and also other optoelectronic devices. Nature Publishing Group 2014-02-13 /pmc/articles/PMC3923213/ /pubmed/24522341 http://dx.doi.org/10.1038/srep04085 Text en Copyright © 2014, Macmillan Publishers Limited. All rights reserved http://creativecommons.org/licenses/by/3.0/ This work is licensed under a Creative Commons Attribution 3.0 Unported License. To view a copy of this license, visit http://creativecommons.org/licenses/by/3.0/
spellingShingle Article
Chen, Jing
Zhao, Dewei
Li, Chi
Xu, Feng
Lei, Wei
Sun, Litao
Nathan, Arokia
Sun, Xiao Wei
All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters
title All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters
title_full All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters
title_fullStr All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters
title_full_unstemmed All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters
title_short All Solution-processed Stable White Quantum Dot Light-emitting Diodes with Hybrid ZnO@TiO(2) as Blue Emitters
title_sort all solution-processed stable white quantum dot light-emitting diodes with hybrid zno@tio(2) as blue emitters
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC3923213/
https://www.ncbi.nlm.nih.gov/pubmed/24522341
http://dx.doi.org/10.1038/srep04085
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