Ultrahigh spin thermopower and pure spin current in a single-molecule magnet

Using the non-equilibrium Green's function (NEGF) formalism within the sequential regime, we studied ultrahigh spin thermopower and pure spin current in single-molecule magnet(SMM), which is attached to nonmagnetic metal wires with spin bias and angle (θ) between the easy axis of SMM and the spin orientation in the electrodes. A pure spin current can be generated by tuning the gate voltage and temperature difference with finite spin bias and the arbitrary angle except of [Image: see text]. In the linear regime, large thermopower can be obtained by modifying V(g) and the angles (θ). These results are useful in fabricating and advantaging SMM devices based on spin caloritronics.