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Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase

Optical antennas transform light from freely propagating waves into highly localized excitations that interact strongly with matter. Unlike their radio frequency counterparts, optical antennas are nanoscopic and high frequency, making amplitude and phase measurements challenging and leaving some inf...

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Autores principales: Gennaro, Sylvain D., Sonnefraud, Yannick, Verellen, Niels, Van Dorpe, Pol, Moshchalkov, Victor V., Maier, Stefan A., Oulton, Rupert F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Pub. Group 2014
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4015323/
https://www.ncbi.nlm.nih.gov/pubmed/24781663
http://dx.doi.org/10.1038/ncomms4748
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author Gennaro, Sylvain D.
Sonnefraud, Yannick
Verellen, Niels
Van Dorpe, Pol
Moshchalkov, Victor V.
Maier, Stefan A.
Oulton, Rupert F.
author_facet Gennaro, Sylvain D.
Sonnefraud, Yannick
Verellen, Niels
Van Dorpe, Pol
Moshchalkov, Victor V.
Maier, Stefan A.
Oulton, Rupert F.
author_sort Gennaro, Sylvain D.
collection PubMed
description Optical antennas transform light from freely propagating waves into highly localized excitations that interact strongly with matter. Unlike their radio frequency counterparts, optical antennas are nanoscopic and high frequency, making amplitude and phase measurements challenging and leaving some information hidden. Here we report a novel spectral interferometric microscopy technique to expose the amplitude and phase response of individual optical antennas across an octave of the visible to near-infrared spectrum. Although it is a far-field technique, we show that knowledge of the extinction phase allows quantitative estimation of nanoantenna absorption, which is a near-field quantity. To verify our method we characterize gold ring-disk dimers exhibiting Fano interference. Our results reveal that Fano interference only cancels a bright mode’s scattering, leaving residual extinction dominated by absorption. Spectral interference microscopy has the potential for real-time and single-shot phase and amplitude investigations of isolated quantum and classical antennas with applications across the physical and life sciences.
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spelling pubmed-40153232014-05-13 Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase Gennaro, Sylvain D. Sonnefraud, Yannick Verellen, Niels Van Dorpe, Pol Moshchalkov, Victor V. Maier, Stefan A. Oulton, Rupert F. Nat Commun Article Optical antennas transform light from freely propagating waves into highly localized excitations that interact strongly with matter. Unlike their radio frequency counterparts, optical antennas are nanoscopic and high frequency, making amplitude and phase measurements challenging and leaving some information hidden. Here we report a novel spectral interferometric microscopy technique to expose the amplitude and phase response of individual optical antennas across an octave of the visible to near-infrared spectrum. Although it is a far-field technique, we show that knowledge of the extinction phase allows quantitative estimation of nanoantenna absorption, which is a near-field quantity. To verify our method we characterize gold ring-disk dimers exhibiting Fano interference. Our results reveal that Fano interference only cancels a bright mode’s scattering, leaving residual extinction dominated by absorption. Spectral interference microscopy has the potential for real-time and single-shot phase and amplitude investigations of isolated quantum and classical antennas with applications across the physical and life sciences. Nature Pub. Group 2014-04-30 /pmc/articles/PMC4015323/ /pubmed/24781663 http://dx.doi.org/10.1038/ncomms4748 Text en Copyright © 2014, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by-nc-by/3.0/ This work is licensed under a Creative Commons Attribution 3.0 Unported License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/3.0/
spellingShingle Article
Gennaro, Sylvain D.
Sonnefraud, Yannick
Verellen, Niels
Van Dorpe, Pol
Moshchalkov, Victor V.
Maier, Stefan A.
Oulton, Rupert F.
Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase
title Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase
title_full Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase
title_fullStr Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase
title_full_unstemmed Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase
title_short Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase
title_sort spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4015323/
https://www.ncbi.nlm.nih.gov/pubmed/24781663
http://dx.doi.org/10.1038/ncomms4748
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