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Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface

Low dimensionality, broken symmetry and easily-modulated carrier concentrations provoke novel electronic phase emergence at oxide interfaces. However, the spatial extent of such reconstructions - i.e. the interfacial “depth” - remains unclear. Examining LaAlO(3)/SrTiO(3) heterostructures at previous...

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Autores principales: Petrović, A. P., Paré, A., Paudel, T. R., Lee, K., Holmes, S., Barnes, C. H. W., David, A., Wu, T., Tsymbal, E. Y., Panagopoulos, C.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2014
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4061544/
https://www.ncbi.nlm.nih.gov/pubmed/24939804
http://dx.doi.org/10.1038/srep05338
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author Petrović, A. P.
Paré, A.
Paudel, T. R.
Lee, K.
Holmes, S.
Barnes, C. H. W.
David, A.
Wu, T.
Tsymbal, E. Y.
Panagopoulos, C.
author_facet Petrović, A. P.
Paré, A.
Paudel, T. R.
Lee, K.
Holmes, S.
Barnes, C. H. W.
David, A.
Wu, T.
Tsymbal, E. Y.
Panagopoulos, C.
author_sort Petrović, A. P.
collection PubMed
description Low dimensionality, broken symmetry and easily-modulated carrier concentrations provoke novel electronic phase emergence at oxide interfaces. However, the spatial extent of such reconstructions - i.e. the interfacial “depth” - remains unclear. Examining LaAlO(3)/SrTiO(3) heterostructures at previously unexplored carrier densities n(2D) ≥ 6.9 × 10(14) cm(−2), we observe a Shubnikov-de Haas effect for small in-plane fields, characteristic of an anisotropic 3D Fermi surface with preferential d(xz,yz) orbital occupancy extending over at least 100 nm perpendicular to the interface. Quantum oscillations from the 3D Fermi surface of bulk doped SrTiO(3) emerge simultaneously at higher n(2D). We distinguish three areas in doped perovskite heterostructures: narrow (<20 nm) 2D interfaces housing superconductivity and/or other emergent phases, electronically isotropic regions far (>120 nm) from the interface and new intermediate zones where interfacial proximity renormalises the electronic structure relative to the bulk.
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spelling pubmed-40615442014-06-18 Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface Petrović, A. P. Paré, A. Paudel, T. R. Lee, K. Holmes, S. Barnes, C. H. W. David, A. Wu, T. Tsymbal, E. Y. Panagopoulos, C. Sci Rep Article Low dimensionality, broken symmetry and easily-modulated carrier concentrations provoke novel electronic phase emergence at oxide interfaces. However, the spatial extent of such reconstructions - i.e. the interfacial “depth” - remains unclear. Examining LaAlO(3)/SrTiO(3) heterostructures at previously unexplored carrier densities n(2D) ≥ 6.9 × 10(14) cm(−2), we observe a Shubnikov-de Haas effect for small in-plane fields, characteristic of an anisotropic 3D Fermi surface with preferential d(xz,yz) orbital occupancy extending over at least 100 nm perpendicular to the interface. Quantum oscillations from the 3D Fermi surface of bulk doped SrTiO(3) emerge simultaneously at higher n(2D). We distinguish three areas in doped perovskite heterostructures: narrow (<20 nm) 2D interfaces housing superconductivity and/or other emergent phases, electronically isotropic regions far (>120 nm) from the interface and new intermediate zones where interfacial proximity renormalises the electronic structure relative to the bulk. Nature Publishing Group 2014-06-18 /pmc/articles/PMC4061544/ /pubmed/24939804 http://dx.doi.org/10.1038/srep05338 Text en Copyright © 2014, Macmillan Publishers Limited. All rights reserved http://creativecommons.org/licenses/by-nc-nd/4.0/ This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivs 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder in order to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-nd/4.0/
spellingShingle Article
Petrović, A. P.
Paré, A.
Paudel, T. R.
Lee, K.
Holmes, S.
Barnes, C. H. W.
David, A.
Wu, T.
Tsymbal, E. Y.
Panagopoulos, C.
Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface
title Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface
title_full Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface
title_fullStr Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface
title_full_unstemmed Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface
title_short Long-range electronic reconstruction to a d(xz,yz)-dominated Fermi surface below the LaAlO(3)/SrTiO(3) interface
title_sort long-range electronic reconstruction to a d(xz,yz)-dominated fermi surface below the laalo(3)/srtio(3) interface
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4061544/
https://www.ncbi.nlm.nih.gov/pubmed/24939804
http://dx.doi.org/10.1038/srep05338
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