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Universal dispersion of surface plasmons in flat nanostructures
Dimensionality has a significant impact on the optical properties of solid-state nanostructures. For example, dimensionality-dependent carrier confinement in semiconductors leads to the formation of quantum wells, quantum wires and quantum dots. While semiconductor properties are governed by exciton...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Pub. Group
2014
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4071950/ https://www.ncbi.nlm.nih.gov/pubmed/24717682 http://dx.doi.org/10.1038/ncomms4604 |
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author | Schmidt, Franz-Philipp Ditlbacher, Harald Hohenester, Ulrich Hohenau, Andreas Hofer, Ferdinand Krenn, Joachim R. |
author_facet | Schmidt, Franz-Philipp Ditlbacher, Harald Hohenester, Ulrich Hohenau, Andreas Hofer, Ferdinand Krenn, Joachim R. |
author_sort | Schmidt, Franz-Philipp |
collection | PubMed |
description | Dimensionality has a significant impact on the optical properties of solid-state nanostructures. For example, dimensionality-dependent carrier confinement in semiconductors leads to the formation of quantum wells, quantum wires and quantum dots. While semiconductor properties are governed by excitonic effects, the optical response of metal nanostructures is dominated by surface plasmons. Here we find that, in contrast to excitonic systems, the mode dispersions in plasmonic structures of different dimensionality are related by simple scaling rules. Employing electron energy loss spectroscopy, we show that the modes of silver nanodisks can be scaled to the surface and edge modes of extended silver thin films. We thereby introduce a general and intuitive ordering scheme for plasmonic excitations with edge and surface modes as the elementary building blocks. |
format | Online Article Text |
id | pubmed-4071950 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2014 |
publisher | Nature Pub. Group |
record_format | MEDLINE/PubMed |
spelling | pubmed-40719502014-06-27 Universal dispersion of surface plasmons in flat nanostructures Schmidt, Franz-Philipp Ditlbacher, Harald Hohenester, Ulrich Hohenau, Andreas Hofer, Ferdinand Krenn, Joachim R. Nat Commun Article Dimensionality has a significant impact on the optical properties of solid-state nanostructures. For example, dimensionality-dependent carrier confinement in semiconductors leads to the formation of quantum wells, quantum wires and quantum dots. While semiconductor properties are governed by excitonic effects, the optical response of metal nanostructures is dominated by surface plasmons. Here we find that, in contrast to excitonic systems, the mode dispersions in plasmonic structures of different dimensionality are related by simple scaling rules. Employing electron energy loss spectroscopy, we show that the modes of silver nanodisks can be scaled to the surface and edge modes of extended silver thin films. We thereby introduce a general and intuitive ordering scheme for plasmonic excitations with edge and surface modes as the elementary building blocks. Nature Pub. Group 2014-04-10 /pmc/articles/PMC4071950/ /pubmed/24717682 http://dx.doi.org/10.1038/ncomms4604 Text en Copyright © 2014, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by-nc-by/3.0/ This work is licensed under a Creative Commons Attribution 3.0 Unported License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/3.0/ |
spellingShingle | Article Schmidt, Franz-Philipp Ditlbacher, Harald Hohenester, Ulrich Hohenau, Andreas Hofer, Ferdinand Krenn, Joachim R. Universal dispersion of surface plasmons in flat nanostructures |
title | Universal dispersion of surface plasmons in flat nanostructures |
title_full | Universal dispersion of surface plasmons in flat nanostructures |
title_fullStr | Universal dispersion of surface plasmons in flat nanostructures |
title_full_unstemmed | Universal dispersion of surface plasmons in flat nanostructures |
title_short | Universal dispersion of surface plasmons in flat nanostructures |
title_sort | universal dispersion of surface plasmons in flat nanostructures |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4071950/ https://www.ncbi.nlm.nih.gov/pubmed/24717682 http://dx.doi.org/10.1038/ncomms4604 |
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