Cargando…

Universal dispersion of surface plasmons in flat nanostructures

Dimensionality has a significant impact on the optical properties of solid-state nanostructures. For example, dimensionality-dependent carrier confinement in semiconductors leads to the formation of quantum wells, quantum wires and quantum dots. While semiconductor properties are governed by exciton...

Descripción completa

Detalles Bibliográficos
Autores principales: Schmidt, Franz-Philipp, Ditlbacher, Harald, Hohenester, Ulrich, Hohenau, Andreas, Hofer, Ferdinand, Krenn, Joachim R.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Pub. Group 2014
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4071950/
https://www.ncbi.nlm.nih.gov/pubmed/24717682
http://dx.doi.org/10.1038/ncomms4604
_version_ 1782322878877794304
author Schmidt, Franz-Philipp
Ditlbacher, Harald
Hohenester, Ulrich
Hohenau, Andreas
Hofer, Ferdinand
Krenn, Joachim R.
author_facet Schmidt, Franz-Philipp
Ditlbacher, Harald
Hohenester, Ulrich
Hohenau, Andreas
Hofer, Ferdinand
Krenn, Joachim R.
author_sort Schmidt, Franz-Philipp
collection PubMed
description Dimensionality has a significant impact on the optical properties of solid-state nanostructures. For example, dimensionality-dependent carrier confinement in semiconductors leads to the formation of quantum wells, quantum wires and quantum dots. While semiconductor properties are governed by excitonic effects, the optical response of metal nanostructures is dominated by surface plasmons. Here we find that, in contrast to excitonic systems, the mode dispersions in plasmonic structures of different dimensionality are related by simple scaling rules. Employing electron energy loss spectroscopy, we show that the modes of silver nanodisks can be scaled to the surface and edge modes of extended silver thin films. We thereby introduce a general and intuitive ordering scheme for plasmonic excitations with edge and surface modes as the elementary building blocks.
format Online
Article
Text
id pubmed-4071950
institution National Center for Biotechnology Information
language English
publishDate 2014
publisher Nature Pub. Group
record_format MEDLINE/PubMed
spelling pubmed-40719502014-06-27 Universal dispersion of surface plasmons in flat nanostructures Schmidt, Franz-Philipp Ditlbacher, Harald Hohenester, Ulrich Hohenau, Andreas Hofer, Ferdinand Krenn, Joachim R. Nat Commun Article Dimensionality has a significant impact on the optical properties of solid-state nanostructures. For example, dimensionality-dependent carrier confinement in semiconductors leads to the formation of quantum wells, quantum wires and quantum dots. While semiconductor properties are governed by excitonic effects, the optical response of metal nanostructures is dominated by surface plasmons. Here we find that, in contrast to excitonic systems, the mode dispersions in plasmonic structures of different dimensionality are related by simple scaling rules. Employing electron energy loss spectroscopy, we show that the modes of silver nanodisks can be scaled to the surface and edge modes of extended silver thin films. We thereby introduce a general and intuitive ordering scheme for plasmonic excitations with edge and surface modes as the elementary building blocks. Nature Pub. Group 2014-04-10 /pmc/articles/PMC4071950/ /pubmed/24717682 http://dx.doi.org/10.1038/ncomms4604 Text en Copyright © 2014, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by-nc-by/3.0/ This work is licensed under a Creative Commons Attribution 3.0 Unported License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/3.0/
spellingShingle Article
Schmidt, Franz-Philipp
Ditlbacher, Harald
Hohenester, Ulrich
Hohenau, Andreas
Hofer, Ferdinand
Krenn, Joachim R.
Universal dispersion of surface plasmons in flat nanostructures
title Universal dispersion of surface plasmons in flat nanostructures
title_full Universal dispersion of surface plasmons in flat nanostructures
title_fullStr Universal dispersion of surface plasmons in flat nanostructures
title_full_unstemmed Universal dispersion of surface plasmons in flat nanostructures
title_short Universal dispersion of surface plasmons in flat nanostructures
title_sort universal dispersion of surface plasmons in flat nanostructures
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4071950/
https://www.ncbi.nlm.nih.gov/pubmed/24717682
http://dx.doi.org/10.1038/ncomms4604
work_keys_str_mv AT schmidtfranzphilipp universaldispersionofsurfaceplasmonsinflatnanostructures
AT ditlbacherharald universaldispersionofsurfaceplasmonsinflatnanostructures
AT hohenesterulrich universaldispersionofsurfaceplasmonsinflatnanostructures
AT hohenauandreas universaldispersionofsurfaceplasmonsinflatnanostructures
AT hoferferdinand universaldispersionofsurfaceplasmonsinflatnanostructures
AT krennjoachimr universaldispersionofsurfaceplasmonsinflatnanostructures