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Large spontaneous emission rate enhancement in grating coupled hyperbolic metamaterials

Hyperbolic metamaterial (HMM), a sub-wavelength periodic artificial structure with hyperbolic dispersion, can enhance the spontaneous emission of quantum emitters. Here, we demonstrate the large spontaneous emission rate enhancement of an organic dye placed in a grating coupled hyperbolic metamateri...

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Detalles Bibliográficos
Autores principales: Sreekanth, Kandammathe Valiyaveedu, Krishna, Koduru Hari, De Luca, Antonio, Strangi, Giuseppe
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2014
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4160708/
https://www.ncbi.nlm.nih.gov/pubmed/25209102
http://dx.doi.org/10.1038/srep06340
Descripción
Sumario:Hyperbolic metamaterial (HMM), a sub-wavelength periodic artificial structure with hyperbolic dispersion, can enhance the spontaneous emission of quantum emitters. Here, we demonstrate the large spontaneous emission rate enhancement of an organic dye placed in a grating coupled hyperbolic metamaterial (GCHMM). A two-dimensional (2D) silver diffraction grating coupled with an Ag/Al(2)O(3) HMM shows 18-fold spontaneous emission decay rate enhancement of dye molecules with respect to the same HMM without grating. The experimental results are compared with analytical models and numerical simulations, which confirm that the observed enhancement of GCHMM is due to the outcoupling of non-radiative plasmonic modes as well as strong plasmon-exciton coupling in HMM via diffracting grating.