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Polluted dust promotes new particle formation and growth

Understanding new particle formation and their subsequent growth in the troposphere has a critical impact on our ability to predict atmospheric composition and global climate change. High pre-existing particle loadings have been thought to suppress the formation of new atmospheric aerosol particles...

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Autores principales: Nie, Wei, Ding, Aijun, Wang, Tao, Kerminen, Veli-Matti, George, Christian, Xue, Likun, Wang, Wenxing, Zhang, Qingzhu, Petäjä, Tuukka, Qi, Ximeng, Gao, Xiaomei, Wang, Xinfeng, Yang, Xiuqun, Fu, Congbin, Kulmala, Markku
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2014
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4198867/
https://www.ncbi.nlm.nih.gov/pubmed/25319109
http://dx.doi.org/10.1038/srep06634
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author Nie, Wei
Ding, Aijun
Wang, Tao
Kerminen, Veli-Matti
George, Christian
Xue, Likun
Wang, Wenxing
Zhang, Qingzhu
Petäjä, Tuukka
Qi, Ximeng
Gao, Xiaomei
Wang, Xinfeng
Yang, Xiuqun
Fu, Congbin
Kulmala, Markku
author_facet Nie, Wei
Ding, Aijun
Wang, Tao
Kerminen, Veli-Matti
George, Christian
Xue, Likun
Wang, Wenxing
Zhang, Qingzhu
Petäjä, Tuukka
Qi, Ximeng
Gao, Xiaomei
Wang, Xinfeng
Yang, Xiuqun
Fu, Congbin
Kulmala, Markku
author_sort Nie, Wei
collection PubMed
description Understanding new particle formation and their subsequent growth in the troposphere has a critical impact on our ability to predict atmospheric composition and global climate change. High pre-existing particle loadings have been thought to suppress the formation of new atmospheric aerosol particles due to high condensation and coagulation sinks. Here, based on field measurements at a mountain site in South China, we report, for the first time, in situ observational evidence on new particle formation and growth in remote ambient atmosphere during heavy dust episodes mixed with anthropogenic pollution. Both the formation and growth rates of particles in the diameter range 15–50 nm were enhanced during the dust episodes, indicating the influence of photo-induced, dust surface-mediated reactions and resulting condensable vapor production. This study provides unique in situ observations of heterogeneous photochemical processes inducing new particle formation and growth in the real atmosphere, and suggests an unexpected impact of mineral dust on climate and atmospheric chemistry.
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spelling pubmed-41988672014-10-21 Polluted dust promotes new particle formation and growth Nie, Wei Ding, Aijun Wang, Tao Kerminen, Veli-Matti George, Christian Xue, Likun Wang, Wenxing Zhang, Qingzhu Petäjä, Tuukka Qi, Ximeng Gao, Xiaomei Wang, Xinfeng Yang, Xiuqun Fu, Congbin Kulmala, Markku Sci Rep Article Understanding new particle formation and their subsequent growth in the troposphere has a critical impact on our ability to predict atmospheric composition and global climate change. High pre-existing particle loadings have been thought to suppress the formation of new atmospheric aerosol particles due to high condensation and coagulation sinks. Here, based on field measurements at a mountain site in South China, we report, for the first time, in situ observational evidence on new particle formation and growth in remote ambient atmosphere during heavy dust episodes mixed with anthropogenic pollution. Both the formation and growth rates of particles in the diameter range 15–50 nm were enhanced during the dust episodes, indicating the influence of photo-induced, dust surface-mediated reactions and resulting condensable vapor production. This study provides unique in situ observations of heterogeneous photochemical processes inducing new particle formation and growth in the real atmosphere, and suggests an unexpected impact of mineral dust on climate and atmospheric chemistry. Nature Publishing Group 2014-10-16 /pmc/articles/PMC4198867/ /pubmed/25319109 http://dx.doi.org/10.1038/srep06634 Text en Copyright © 2014, Macmillan Publishers Limited. All rights reserved http://creativecommons.org/licenses/by-nc-sa/4.0/ This work is licensed under a Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder in order to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-sa/4.0/
spellingShingle Article
Nie, Wei
Ding, Aijun
Wang, Tao
Kerminen, Veli-Matti
George, Christian
Xue, Likun
Wang, Wenxing
Zhang, Qingzhu
Petäjä, Tuukka
Qi, Ximeng
Gao, Xiaomei
Wang, Xinfeng
Yang, Xiuqun
Fu, Congbin
Kulmala, Markku
Polluted dust promotes new particle formation and growth
title Polluted dust promotes new particle formation and growth
title_full Polluted dust promotes new particle formation and growth
title_fullStr Polluted dust promotes new particle formation and growth
title_full_unstemmed Polluted dust promotes new particle formation and growth
title_short Polluted dust promotes new particle formation and growth
title_sort polluted dust promotes new particle formation and growth
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4198867/
https://www.ncbi.nlm.nih.gov/pubmed/25319109
http://dx.doi.org/10.1038/srep06634
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