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Identification of Ice Nucleation Active Sites on Feldspar Dust Particles
[Image: see text] Mineral dusts originating from Earth’s crust are known to be important atmospheric ice nuclei. In agreement with earlier studies, feldspar was found as the most active of the tested natural mineral dusts. Here we investigated in closer detail the reasons for its activity and the di...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical
Society
2015
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4368087/ https://www.ncbi.nlm.nih.gov/pubmed/25584435 http://dx.doi.org/10.1021/jp509839x |
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author | Zolles, Tobias Burkart, Julia Häusler, Thomas Pummer, Bernhard Hitzenberger, Regina Grothe, Hinrich |
author_facet | Zolles, Tobias Burkart, Julia Häusler, Thomas Pummer, Bernhard Hitzenberger, Regina Grothe, Hinrich |
author_sort | Zolles, Tobias |
collection | PubMed |
description | [Image: see text] Mineral dusts originating from Earth’s crust are known to be important atmospheric ice nuclei. In agreement with earlier studies, feldspar was found as the most active of the tested natural mineral dusts. Here we investigated in closer detail the reasons for its activity and the difference in the activity of the different feldspars. Conclusions are drawn from scanning electron microscopy, X-ray powder diffraction, infrared spectroscopy, and oil-immersion freezing experiments. K-feldspar showed by far the highest ice nucleation activity. Finally, we give a potential explanation of this effect, finding alkali-metal ions having different hydration shells and thus an influence on the ice nucleation activity of feldspar surfaces. |
format | Online Article Text |
id | pubmed-4368087 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2015 |
publisher | American Chemical
Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-43680872015-03-31 Identification of Ice Nucleation Active Sites on Feldspar Dust Particles Zolles, Tobias Burkart, Julia Häusler, Thomas Pummer, Bernhard Hitzenberger, Regina Grothe, Hinrich J Phys Chem A [Image: see text] Mineral dusts originating from Earth’s crust are known to be important atmospheric ice nuclei. In agreement with earlier studies, feldspar was found as the most active of the tested natural mineral dusts. Here we investigated in closer detail the reasons for its activity and the difference in the activity of the different feldspars. Conclusions are drawn from scanning electron microscopy, X-ray powder diffraction, infrared spectroscopy, and oil-immersion freezing experiments. K-feldspar showed by far the highest ice nucleation activity. Finally, we give a potential explanation of this effect, finding alkali-metal ions having different hydration shells and thus an influence on the ice nucleation activity of feldspar surfaces. American Chemical Society 2015-01-13 2015-03-19 /pmc/articles/PMC4368087/ /pubmed/25584435 http://dx.doi.org/10.1021/jp509839x Text en Copyright © 2015 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited. |
spellingShingle | Zolles, Tobias Burkart, Julia Häusler, Thomas Pummer, Bernhard Hitzenberger, Regina Grothe, Hinrich Identification of Ice Nucleation Active Sites on Feldspar Dust Particles |
title | Identification
of Ice Nucleation Active Sites on Feldspar
Dust Particles |
title_full | Identification
of Ice Nucleation Active Sites on Feldspar
Dust Particles |
title_fullStr | Identification
of Ice Nucleation Active Sites on Feldspar
Dust Particles |
title_full_unstemmed | Identification
of Ice Nucleation Active Sites on Feldspar
Dust Particles |
title_short | Identification
of Ice Nucleation Active Sites on Feldspar
Dust Particles |
title_sort | identification
of ice nucleation active sites on feldspar
dust particles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4368087/ https://www.ncbi.nlm.nih.gov/pubmed/25584435 http://dx.doi.org/10.1021/jp509839x |
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