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Nanoscale probing of image-dipole interactions in a metallic nanostructure

An emitter near a surface induces an image dipole that can modify the observed emission intensity and radiation pattern. These image-dipole effects are generally not taken into account in single-emitter tracking and super-resolved imaging applications. Here we show that the interference between an e...

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Autores principales: Ropp, Chad, Cummins, Zachary, Nah, Sanghee, Fourkas, John T., Shapiro, Benjamin, Waks, Edo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Pub. Group 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4383001/
https://www.ncbi.nlm.nih.gov/pubmed/25790228
http://dx.doi.org/10.1038/ncomms7558
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author Ropp, Chad
Cummins, Zachary
Nah, Sanghee
Fourkas, John T.
Shapiro, Benjamin
Waks, Edo
author_facet Ropp, Chad
Cummins, Zachary
Nah, Sanghee
Fourkas, John T.
Shapiro, Benjamin
Waks, Edo
author_sort Ropp, Chad
collection PubMed
description An emitter near a surface induces an image dipole that can modify the observed emission intensity and radiation pattern. These image-dipole effects are generally not taken into account in single-emitter tracking and super-resolved imaging applications. Here we show that the interference between an emitter and its image dipole induces a strong polarization anisotropy and a large spatial displacement of the observed emission pattern. We demonstrate these effects by tracking the emission of a single quantum dot along two orthogonal polarizations as it is deterministically positioned near a silver nanowire. The two orthogonally polarized diffraction spots can be displaced by up to 50 nm, which arises from a Young’s interference effect between the quantum dot and its induced image dipole. We show that the observed spatially varying interference fringe provides a useful measure for correcting image-dipole-induced distortions. These results provide a pathway towards probing and correcting image-dipole effects in near-field imaging applications.
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spelling pubmed-43830012015-04-07 Nanoscale probing of image-dipole interactions in a metallic nanostructure Ropp, Chad Cummins, Zachary Nah, Sanghee Fourkas, John T. Shapiro, Benjamin Waks, Edo Nat Commun Article An emitter near a surface induces an image dipole that can modify the observed emission intensity and radiation pattern. These image-dipole effects are generally not taken into account in single-emitter tracking and super-resolved imaging applications. Here we show that the interference between an emitter and its image dipole induces a strong polarization anisotropy and a large spatial displacement of the observed emission pattern. We demonstrate these effects by tracking the emission of a single quantum dot along two orthogonal polarizations as it is deterministically positioned near a silver nanowire. The two orthogonally polarized diffraction spots can be displaced by up to 50 nm, which arises from a Young’s interference effect between the quantum dot and its induced image dipole. We show that the observed spatially varying interference fringe provides a useful measure for correcting image-dipole-induced distortions. These results provide a pathway towards probing and correcting image-dipole effects in near-field imaging applications. Nature Pub. Group 2015-03-19 /pmc/articles/PMC4383001/ /pubmed/25790228 http://dx.doi.org/10.1038/ncomms7558 Text en Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Ropp, Chad
Cummins, Zachary
Nah, Sanghee
Fourkas, John T.
Shapiro, Benjamin
Waks, Edo
Nanoscale probing of image-dipole interactions in a metallic nanostructure
title Nanoscale probing of image-dipole interactions in a metallic nanostructure
title_full Nanoscale probing of image-dipole interactions in a metallic nanostructure
title_fullStr Nanoscale probing of image-dipole interactions in a metallic nanostructure
title_full_unstemmed Nanoscale probing of image-dipole interactions in a metallic nanostructure
title_short Nanoscale probing of image-dipole interactions in a metallic nanostructure
title_sort nanoscale probing of image-dipole interactions in a metallic nanostructure
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4383001/
https://www.ncbi.nlm.nih.gov/pubmed/25790228
http://dx.doi.org/10.1038/ncomms7558
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