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Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source
X-ray free-electron lasers (FELs) have opened unprecedented possibilities to study the structure and dynamics of matter at an atomic level and ultra-fast timescale. Many of the techniques routinely used at storage ring facilities are being adapted for experiments conducted at FELs. In order to take...
Autores principales: | , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
International Union of Crystallography
2015
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4416677/ https://www.ncbi.nlm.nih.gov/pubmed/25931076 http://dx.doi.org/10.1107/S1600577515004488 |
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author | Alonso-Mori, Roberto Sokaras, Dimosthenis Zhu, Diling Kroll, Thomas Chollet, Mathieu Feng, Yiping Glownia, James M. Kern, Jan Lemke, Henrik T. Nordlund, Dennis Robert, Aymeric Sikorski, Marcin Song, Sanghoon Weng, Tsu-Chien Bergmann, Uwe |
author_facet | Alonso-Mori, Roberto Sokaras, Dimosthenis Zhu, Diling Kroll, Thomas Chollet, Mathieu Feng, Yiping Glownia, James M. Kern, Jan Lemke, Henrik T. Nordlund, Dennis Robert, Aymeric Sikorski, Marcin Song, Sanghoon Weng, Tsu-Chien Bergmann, Uwe |
author_sort | Alonso-Mori, Roberto |
collection | PubMed |
description | X-ray free-electron lasers (FELs) have opened unprecedented possibilities to study the structure and dynamics of matter at an atomic level and ultra-fast timescale. Many of the techniques routinely used at storage ring facilities are being adapted for experiments conducted at FELs. In order to take full advantage of these new sources several challenges have to be overcome. They are related to the very different source characteristics and its resulting impact on sample delivery, X-ray optics, X-ray detection and data acquisition. Here it is described how photon-in photon-out hard X-ray spectroscopy techniques can be applied to study the electronic structure and its dynamics of transition metal systems with ultra-bright and ultra-short FEL X-ray pulses. In particular, some of the experimental details that are different compared with synchrotron-based setups are discussed and illustrated by recent measurements performed at the Linac Coherent Light Source. |
format | Online Article Text |
id | pubmed-4416677 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2015 |
publisher | International Union of Crystallography |
record_format | MEDLINE/PubMed |
spelling | pubmed-44166772015-05-20 Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source Alonso-Mori, Roberto Sokaras, Dimosthenis Zhu, Diling Kroll, Thomas Chollet, Mathieu Feng, Yiping Glownia, James M. Kern, Jan Lemke, Henrik T. Nordlund, Dennis Robert, Aymeric Sikorski, Marcin Song, Sanghoon Weng, Tsu-Chien Bergmann, Uwe J Synchrotron Radiat Free-Electron Lasers X-ray free-electron lasers (FELs) have opened unprecedented possibilities to study the structure and dynamics of matter at an atomic level and ultra-fast timescale. Many of the techniques routinely used at storage ring facilities are being adapted for experiments conducted at FELs. In order to take full advantage of these new sources several challenges have to be overcome. They are related to the very different source characteristics and its resulting impact on sample delivery, X-ray optics, X-ray detection and data acquisition. Here it is described how photon-in photon-out hard X-ray spectroscopy techniques can be applied to study the electronic structure and its dynamics of transition metal systems with ultra-bright and ultra-short FEL X-ray pulses. In particular, some of the experimental details that are different compared with synchrotron-based setups are discussed and illustrated by recent measurements performed at the Linac Coherent Light Source. International Union of Crystallography 2015-04-15 /pmc/articles/PMC4416677/ /pubmed/25931076 http://dx.doi.org/10.1107/S1600577515004488 Text en © Roberto Alonso-Mori et al. 2015 http://creativecommons.org/licenses/by/2.0/uk/ This is an open-access article distributed under the terms of the Creative Commons Attribution Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited. |
spellingShingle | Free-Electron Lasers Alonso-Mori, Roberto Sokaras, Dimosthenis Zhu, Diling Kroll, Thomas Chollet, Mathieu Feng, Yiping Glownia, James M. Kern, Jan Lemke, Henrik T. Nordlund, Dennis Robert, Aymeric Sikorski, Marcin Song, Sanghoon Weng, Tsu-Chien Bergmann, Uwe Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source |
title | Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source |
title_full | Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source |
title_fullStr | Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source |
title_full_unstemmed | Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source |
title_short | Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source |
title_sort | photon-in photon-out hard x-ray spectroscopy at the linac coherent light source |
topic | Free-Electron Lasers |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4416677/ https://www.ncbi.nlm.nih.gov/pubmed/25931076 http://dx.doi.org/10.1107/S1600577515004488 |
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