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Superconfinement tailors fluid flow at microscales

Understanding fluid dynamics under extreme confinement, where device and intrinsic fluid length scales become comparable, is essential to successfully develop the coming generations of fluidic devices. Here we report measurements of advancing fluid fronts in such a regime, which we dub superconfinem...

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Autores principales: Setu, Siti Aminah, Dullens, Roel P.A., Hernández-Machado, Aurora, Pagonabarraga, Ignacio, Aarts, Dirk G.A.L., Ledesma-Aguilar, Rodrigo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Pub. Group 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4490407/
https://www.ncbi.nlm.nih.gov/pubmed/26073752
http://dx.doi.org/10.1038/ncomms8297
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author Setu, Siti Aminah
Dullens, Roel P.A.
Hernández-Machado, Aurora
Pagonabarraga, Ignacio
Aarts, Dirk G.A.L.
Ledesma-Aguilar, Rodrigo
author_facet Setu, Siti Aminah
Dullens, Roel P.A.
Hernández-Machado, Aurora
Pagonabarraga, Ignacio
Aarts, Dirk G.A.L.
Ledesma-Aguilar, Rodrigo
author_sort Setu, Siti Aminah
collection PubMed
description Understanding fluid dynamics under extreme confinement, where device and intrinsic fluid length scales become comparable, is essential to successfully develop the coming generations of fluidic devices. Here we report measurements of advancing fluid fronts in such a regime, which we dub superconfinement. We find that the strong coupling between contact-line friction and geometric confinement gives rise to a new stability regime where the maximum speed for a stable moving front exhibits a distinctive response to changes in the bounding geometry. Unstable fronts develop into drop-emitting jets controlled by thermal fluctuations. Numerical simulations reveal that the dynamics in superconfined systems is dominated by interfacial forces. Henceforth, we present a theory that quantifies our experiments in terms of the relevant interfacial length scale, which in our system is the intrinsic contact-line slip length. Our findings show that length-scale overlap can be used as a new fluid-control mechanism in strongly confined systems.
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spelling pubmed-44904072015-07-13 Superconfinement tailors fluid flow at microscales Setu, Siti Aminah Dullens, Roel P.A. Hernández-Machado, Aurora Pagonabarraga, Ignacio Aarts, Dirk G.A.L. Ledesma-Aguilar, Rodrigo Nat Commun Article Understanding fluid dynamics under extreme confinement, where device and intrinsic fluid length scales become comparable, is essential to successfully develop the coming generations of fluidic devices. Here we report measurements of advancing fluid fronts in such a regime, which we dub superconfinement. We find that the strong coupling between contact-line friction and geometric confinement gives rise to a new stability regime where the maximum speed for a stable moving front exhibits a distinctive response to changes in the bounding geometry. Unstable fronts develop into drop-emitting jets controlled by thermal fluctuations. Numerical simulations reveal that the dynamics in superconfined systems is dominated by interfacial forces. Henceforth, we present a theory that quantifies our experiments in terms of the relevant interfacial length scale, which in our system is the intrinsic contact-line slip length. Our findings show that length-scale overlap can be used as a new fluid-control mechanism in strongly confined systems. Nature Pub. Group 2015-06-15 /pmc/articles/PMC4490407/ /pubmed/26073752 http://dx.doi.org/10.1038/ncomms8297 Text en Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Setu, Siti Aminah
Dullens, Roel P.A.
Hernández-Machado, Aurora
Pagonabarraga, Ignacio
Aarts, Dirk G.A.L.
Ledesma-Aguilar, Rodrigo
Superconfinement tailors fluid flow at microscales
title Superconfinement tailors fluid flow at microscales
title_full Superconfinement tailors fluid flow at microscales
title_fullStr Superconfinement tailors fluid flow at microscales
title_full_unstemmed Superconfinement tailors fluid flow at microscales
title_short Superconfinement tailors fluid flow at microscales
title_sort superconfinement tailors fluid flow at microscales
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4490407/
https://www.ncbi.nlm.nih.gov/pubmed/26073752
http://dx.doi.org/10.1038/ncomms8297
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