Cargando…

Ultra-stable sub-meV monochromator for hard X-rays

A high-resolution silicon monochromator suitable for 21.541 keV synchrotron radiation is presented that produces a bandwidth of 0.27 meV. The operating energy corresponds to a nuclear transition in (151)Eu. The first-of-its-kind, fully cryogenic design achieves an energy-alignment stability of 0.017...

Descripción completa

Detalles Bibliográficos
Autores principales: Toellner, T. S., Collins, J., Goetze, K., Hu, M. Y., Preissner, C., Trakhtenberg, E., Yan, L.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: International Union of Crystallography 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4542453/
https://www.ncbi.nlm.nih.gov/pubmed/26289266
http://dx.doi.org/10.1107/S1600577515012230
_version_ 1782386534925729792
author Toellner, T. S.
Collins, J.
Goetze, K.
Hu, M. Y.
Preissner, C.
Trakhtenberg, E.
Yan, L.
author_facet Toellner, T. S.
Collins, J.
Goetze, K.
Hu, M. Y.
Preissner, C.
Trakhtenberg, E.
Yan, L.
author_sort Toellner, T. S.
collection PubMed
description A high-resolution silicon monochromator suitable for 21.541 keV synchrotron radiation is presented that produces a bandwidth of 0.27 meV. The operating energy corresponds to a nuclear transition in (151)Eu. The first-of-its-kind, fully cryogenic design achieves an energy-alignment stability of 0.017 meV r.m.s. per day, or a 100-fold improvement over other meV-monochromators, and can tolerate higher X-ray power loads than room-temperature designs of comparable resolution. This offers the potential for significantly more accurate measurements of lattice excitation energies using nuclear resonant vibrational spectroscopy if combined with accurate energy calibration using, for example, high-speed Doppler shifting. The design of the monochromator along with its performance and impact on transmitted beam properties are presented.
format Online
Article
Text
id pubmed-4542453
institution National Center for Biotechnology Information
language English
publishDate 2015
publisher International Union of Crystallography
record_format MEDLINE/PubMed
spelling pubmed-45424532015-08-24 Ultra-stable sub-meV monochromator for hard X-rays Toellner, T. S. Collins, J. Goetze, K. Hu, M. Y. Preissner, C. Trakhtenberg, E. Yan, L. J Synchrotron Radiat Research Papers A high-resolution silicon monochromator suitable for 21.541 keV synchrotron radiation is presented that produces a bandwidth of 0.27 meV. The operating energy corresponds to a nuclear transition in (151)Eu. The first-of-its-kind, fully cryogenic design achieves an energy-alignment stability of 0.017 meV r.m.s. per day, or a 100-fold improvement over other meV-monochromators, and can tolerate higher X-ray power loads than room-temperature designs of comparable resolution. This offers the potential for significantly more accurate measurements of lattice excitation energies using nuclear resonant vibrational spectroscopy if combined with accurate energy calibration using, for example, high-speed Doppler shifting. The design of the monochromator along with its performance and impact on transmitted beam properties are presented. International Union of Crystallography 2015-07-17 /pmc/articles/PMC4542453/ /pubmed/26289266 http://dx.doi.org/10.1107/S1600577515012230 Text en © T. S. Toellner et al. 2015 http://creativecommons.org/licenses/by/2.0/uk/ This is an open-access article distributed under the terms of the Creative Commons Attribution Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited.
spellingShingle Research Papers
Toellner, T. S.
Collins, J.
Goetze, K.
Hu, M. Y.
Preissner, C.
Trakhtenberg, E.
Yan, L.
Ultra-stable sub-meV monochromator for hard X-rays
title Ultra-stable sub-meV monochromator for hard X-rays
title_full Ultra-stable sub-meV monochromator for hard X-rays
title_fullStr Ultra-stable sub-meV monochromator for hard X-rays
title_full_unstemmed Ultra-stable sub-meV monochromator for hard X-rays
title_short Ultra-stable sub-meV monochromator for hard X-rays
title_sort ultra-stable sub-mev monochromator for hard x-rays
topic Research Papers
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4542453/
https://www.ncbi.nlm.nih.gov/pubmed/26289266
http://dx.doi.org/10.1107/S1600577515012230
work_keys_str_mv AT toellnerts ultrastablesubmevmonochromatorforhardxrays
AT collinsj ultrastablesubmevmonochromatorforhardxrays
AT goetzek ultrastablesubmevmonochromatorforhardxrays
AT humy ultrastablesubmevmonochromatorforhardxrays
AT preissnerc ultrastablesubmevmonochromatorforhardxrays
AT trakhtenberge ultrastablesubmevmonochromatorforhardxrays
AT yanl ultrastablesubmevmonochromatorforhardxrays