Cargando…
Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterost...
Autores principales: | , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Pub. Group
2015
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4595592/ https://www.ncbi.nlm.nih.gov/pubmed/26382137 http://dx.doi.org/10.1038/ncomms9121 |
_version_ | 1782393638229114880 |
---|---|
author | Cronenberger, S. Scalbert, D. Ferrand, D. Boukari, H. Cibert, J. |
author_facet | Cronenberger, S. Scalbert, D. Ferrand, D. Boukari, H. Cibert, J. |
author_sort | Cronenberger, S. |
collection | PubMed |
description | Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterostructures. Here we show that atomic-like spin fluctuations of Mn ions diluted in CdTe (bulk and quantum wells) can be detected through the Kerr rotation associated to excitonic transitions. Zeeman transitions within and between hyperfine multiplets are clearly observed in zero and small magnetic fields and reveal the local symmetry because of crystal field and strain. The linewidths of these resonances are close to the dipolar limit. The sensitivity is high enough to open the way towards the detection of a few spins in systems where the decoherence due to nuclear spins can be suppressed by isotopic enrichment, and towards spin resonance microscopy with important applications in biology and materials science. |
format | Online Article Text |
id | pubmed-4595592 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2015 |
publisher | Nature Pub. Group |
record_format | MEDLINE/PubMed |
spelling | pubmed-45955922015-10-21 Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride Cronenberger, S. Scalbert, D. Ferrand, D. Boukari, H. Cibert, J. Nat Commun Article Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterostructures. Here we show that atomic-like spin fluctuations of Mn ions diluted in CdTe (bulk and quantum wells) can be detected through the Kerr rotation associated to excitonic transitions. Zeeman transitions within and between hyperfine multiplets are clearly observed in zero and small magnetic fields and reveal the local symmetry because of crystal field and strain. The linewidths of these resonances are close to the dipolar limit. The sensitivity is high enough to open the way towards the detection of a few spins in systems where the decoherence due to nuclear spins can be suppressed by isotopic enrichment, and towards spin resonance microscopy with important applications in biology and materials science. Nature Pub. Group 2015-09-18 /pmc/articles/PMC4595592/ /pubmed/26382137 http://dx.doi.org/10.1038/ncomms9121 Text en Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ |
spellingShingle | Article Cronenberger, S. Scalbert, D. Ferrand, D. Boukari, H. Cibert, J. Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride |
title | Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride |
title_full | Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride |
title_fullStr | Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride |
title_full_unstemmed | Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride |
title_short | Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride |
title_sort | atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4595592/ https://www.ncbi.nlm.nih.gov/pubmed/26382137 http://dx.doi.org/10.1038/ncomms9121 |
work_keys_str_mv | AT cronenbergers atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride AT scalbertd atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride AT ferrandd atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride AT boukarih atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride AT cibertj atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride |