Cargando…

Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride

Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterost...

Descripción completa

Detalles Bibliográficos
Autores principales: Cronenberger, S., Scalbert, D., Ferrand, D., Boukari, H., Cibert, J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Pub. Group 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4595592/
https://www.ncbi.nlm.nih.gov/pubmed/26382137
http://dx.doi.org/10.1038/ncomms9121
_version_ 1782393638229114880
author Cronenberger, S.
Scalbert, D.
Ferrand, D.
Boukari, H.
Cibert, J.
author_facet Cronenberger, S.
Scalbert, D.
Ferrand, D.
Boukari, H.
Cibert, J.
author_sort Cronenberger, S.
collection PubMed
description Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterostructures. Here we show that atomic-like spin fluctuations of Mn ions diluted in CdTe (bulk and quantum wells) can be detected through the Kerr rotation associated to excitonic transitions. Zeeman transitions within and between hyperfine multiplets are clearly observed in zero and small magnetic fields and reveal the local symmetry because of crystal field and strain. The linewidths of these resonances are close to the dipolar limit. The sensitivity is high enough to open the way towards the detection of a few spins in systems where the decoherence due to nuclear spins can be suppressed by isotopic enrichment, and towards spin resonance microscopy with important applications in biology and materials science.
format Online
Article
Text
id pubmed-4595592
institution National Center for Biotechnology Information
language English
publishDate 2015
publisher Nature Pub. Group
record_format MEDLINE/PubMed
spelling pubmed-45955922015-10-21 Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride Cronenberger, S. Scalbert, D. Ferrand, D. Boukari, H. Cibert, J. Nat Commun Article Spin noise spectroscopy is an optical technique which can probe spin resonances non-perturbatively. First applied to atomic vapours, it revealed detailed information about nuclear magnetism and the hyperfine interaction. In solids, this approach has been limited to carriers in semiconductor heterostructures. Here we show that atomic-like spin fluctuations of Mn ions diluted in CdTe (bulk and quantum wells) can be detected through the Kerr rotation associated to excitonic transitions. Zeeman transitions within and between hyperfine multiplets are clearly observed in zero and small magnetic fields and reveal the local symmetry because of crystal field and strain. The linewidths of these resonances are close to the dipolar limit. The sensitivity is high enough to open the way towards the detection of a few spins in systems where the decoherence due to nuclear spins can be suppressed by isotopic enrichment, and towards spin resonance microscopy with important applications in biology and materials science. Nature Pub. Group 2015-09-18 /pmc/articles/PMC4595592/ /pubmed/26382137 http://dx.doi.org/10.1038/ncomms9121 Text en Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Cronenberger, S.
Scalbert, D.
Ferrand, D.
Boukari, H.
Cibert, J.
Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
title Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
title_full Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
title_fullStr Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
title_full_unstemmed Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
title_short Atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
title_sort atomic-like spin noise in solid-state demonstrated with manganese in cadmium telluride
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4595592/
https://www.ncbi.nlm.nih.gov/pubmed/26382137
http://dx.doi.org/10.1038/ncomms9121
work_keys_str_mv AT cronenbergers atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride
AT scalbertd atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride
AT ferrandd atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride
AT boukarih atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride
AT cibertj atomiclikespinnoiseinsolidstatedemonstratedwithmanganeseincadmiumtelluride