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Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings

Resonant absorbers based on nanostructured materials are promising for variety of applications including optical filters, thermophotovoltaics, thermal emitters, and hot-electron collection. One of the significant challenges for such micro/nanoscale featured medium or surface, however, is costly lith...

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Autores principales: Li, Zhongyang, Palacios, Edgar, Butun, Serkan, Kocer, Hasan, Aydin, Koray
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4598830/
https://www.ncbi.nlm.nih.gov/pubmed/26450563
http://dx.doi.org/10.1038/srep15137
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author Li, Zhongyang
Palacios, Edgar
Butun, Serkan
Kocer, Hasan
Aydin, Koray
author_facet Li, Zhongyang
Palacios, Edgar
Butun, Serkan
Kocer, Hasan
Aydin, Koray
author_sort Li, Zhongyang
collection PubMed
description Resonant absorbers based on nanostructured materials are promising for variety of applications including optical filters, thermophotovoltaics, thermal emitters, and hot-electron collection. One of the significant challenges for such micro/nanoscale featured medium or surface, however, is costly lithographic processes for structural patterning which restricted from industrial production of complex designs. Here, we demonstrate lithography-free, broadband, polarization-independent optical absorbers based on a three-layer ultrathin film composed of subwavelength chromium (Cr) and oxide film coatings. We have measured almost perfect absorption as high as 99.5% across the entire visible regime and beyond (400–800 nm). In addition to near-ideal absorption, our absorbers exhibit omnidirectional independence for incidence angle over ±60 degrees. Broadband absorbers introduced in this study perform better than nanostructured plasmonic absorber counterparts in terms of bandwidth, polarization and angle independence. Improvements of such “blackbody” samples based on uniform thin-film coatings is attributed to extremely low quality factor of asymmetric highly-lossy Fabry-Perot cavities. Such broadband absorber designs are ultrathin compared to carbon nanotube based black materials, and does not require lithographic processes. This demonstration redirects the broadband super absorber design to extreme simplicity, higher performance and cost effective manufacturing convenience for practical industrial production.
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spelling pubmed-45988302015-10-13 Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings Li, Zhongyang Palacios, Edgar Butun, Serkan Kocer, Hasan Aydin, Koray Sci Rep Article Resonant absorbers based on nanostructured materials are promising for variety of applications including optical filters, thermophotovoltaics, thermal emitters, and hot-electron collection. One of the significant challenges for such micro/nanoscale featured medium or surface, however, is costly lithographic processes for structural patterning which restricted from industrial production of complex designs. Here, we demonstrate lithography-free, broadband, polarization-independent optical absorbers based on a three-layer ultrathin film composed of subwavelength chromium (Cr) and oxide film coatings. We have measured almost perfect absorption as high as 99.5% across the entire visible regime and beyond (400–800 nm). In addition to near-ideal absorption, our absorbers exhibit omnidirectional independence for incidence angle over ±60 degrees. Broadband absorbers introduced in this study perform better than nanostructured plasmonic absorber counterparts in terms of bandwidth, polarization and angle independence. Improvements of such “blackbody” samples based on uniform thin-film coatings is attributed to extremely low quality factor of asymmetric highly-lossy Fabry-Perot cavities. Such broadband absorber designs are ultrathin compared to carbon nanotube based black materials, and does not require lithographic processes. This demonstration redirects the broadband super absorber design to extreme simplicity, higher performance and cost effective manufacturing convenience for practical industrial production. Nature Publishing Group 2015-10-09 /pmc/articles/PMC4598830/ /pubmed/26450563 http://dx.doi.org/10.1038/srep15137 Text en Copyright © 2015, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Li, Zhongyang
Palacios, Edgar
Butun, Serkan
Kocer, Hasan
Aydin, Koray
Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings
title Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings
title_full Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings
title_fullStr Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings
title_full_unstemmed Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings
title_short Omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings
title_sort omnidirectional, broadband light absorption using large-area, ultrathin lossy metallic film coatings
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4598830/
https://www.ncbi.nlm.nih.gov/pubmed/26450563
http://dx.doi.org/10.1038/srep15137
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