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Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)

[Image: see text] Two-dimensional transition metal dichalcogenide semiconductors are intriguing hosts for quantum light sources due to their unique optoelectronic properties. Here, we report that strain gradients, either unintentionally induced or generated by substrate patterning, result in spatial...

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Detalles Bibliográficos
Autores principales: Kumar, S., Kaczmarczyk, A., Gerardot, B. D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2015
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4643357/
https://www.ncbi.nlm.nih.gov/pubmed/26480237
http://dx.doi.org/10.1021/acs.nanolett.5b03312
Descripción
Sumario:[Image: see text] Two-dimensional transition metal dichalcogenide semiconductors are intriguing hosts for quantum light sources due to their unique optoelectronic properties. Here, we report that strain gradients, either unintentionally induced or generated by substrate patterning, result in spatially and spectrally isolated quantum emitters in mono- and bilayer WSe(2). By correlating localized excitons with localized strain variations, we show that the quantum emitter emission energy can be red-tuned up to a remarkable ∼170 meV. We probe the fine-structure, magneto-optics, and second-order coherence of a strained emitter. These results raise the prospect of strain-engineering quantum emitter properties and deterministically creating arrays of quantum emitters in two-dimensional semiconductors.