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Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)

[Image: see text] Two-dimensional transition metal dichalcogenide semiconductors are intriguing hosts for quantum light sources due to their unique optoelectronic properties. Here, we report that strain gradients, either unintentionally induced or generated by substrate patterning, result in spatial...

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Autores principales: Kumar, S., Kaczmarczyk, A., Gerardot, B. D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2015
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4643357/
https://www.ncbi.nlm.nih.gov/pubmed/26480237
http://dx.doi.org/10.1021/acs.nanolett.5b03312
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author Kumar, S.
Kaczmarczyk, A.
Gerardot, B. D.
author_facet Kumar, S.
Kaczmarczyk, A.
Gerardot, B. D.
author_sort Kumar, S.
collection PubMed
description [Image: see text] Two-dimensional transition metal dichalcogenide semiconductors are intriguing hosts for quantum light sources due to their unique optoelectronic properties. Here, we report that strain gradients, either unintentionally induced or generated by substrate patterning, result in spatially and spectrally isolated quantum emitters in mono- and bilayer WSe(2). By correlating localized excitons with localized strain variations, we show that the quantum emitter emission energy can be red-tuned up to a remarkable ∼170 meV. We probe the fine-structure, magneto-optics, and second-order coherence of a strained emitter. These results raise the prospect of strain-engineering quantum emitter properties and deterministically creating arrays of quantum emitters in two-dimensional semiconductors.
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spelling pubmed-46433572015-11-27 Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2) Kumar, S. Kaczmarczyk, A. Gerardot, B. D. Nano Lett [Image: see text] Two-dimensional transition metal dichalcogenide semiconductors are intriguing hosts for quantum light sources due to their unique optoelectronic properties. Here, we report that strain gradients, either unintentionally induced or generated by substrate patterning, result in spatially and spectrally isolated quantum emitters in mono- and bilayer WSe(2). By correlating localized excitons with localized strain variations, we show that the quantum emitter emission energy can be red-tuned up to a remarkable ∼170 meV. We probe the fine-structure, magneto-optics, and second-order coherence of a strained emitter. These results raise the prospect of strain-engineering quantum emitter properties and deterministically creating arrays of quantum emitters in two-dimensional semiconductors. American Chemical Society 2015-10-19 2015-11-11 /pmc/articles/PMC4643357/ /pubmed/26480237 http://dx.doi.org/10.1021/acs.nanolett.5b03312 Text en Copyright © 2015 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
spellingShingle Kumar, S.
Kaczmarczyk, A.
Gerardot, B. D.
Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)
title Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)
title_full Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)
title_fullStr Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)
title_full_unstemmed Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)
title_short Strain-Induced Spatial and Spectral Isolation of Quantum Emitters in Mono- and Bilayer WSe(2)
title_sort strain-induced spatial and spectral isolation of quantum emitters in mono- and bilayer wse(2)
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4643357/
https://www.ncbi.nlm.nih.gov/pubmed/26480237
http://dx.doi.org/10.1021/acs.nanolett.5b03312
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