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Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide

The magnetic graphene oxide (MGO) was successfully synthesised by the in situ chemical co-precipitation method with Fe(3+), Fe(2+) and graphene oxide (GO) in laboratory and, was used as an adsorbent for disinfection by-product (DBP) precursors removing from four natural surface water samples. The re...

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Autores principales: Liu, Zhongmou, Wang, Xianze, Luo, Zhen, Huo, Mingxin, Wu, Jinghui, Huo, Hongliang, Yang, Wu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Public Library of Science 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4666622/
https://www.ncbi.nlm.nih.gov/pubmed/26623652
http://dx.doi.org/10.1371/journal.pone.0143819
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author Liu, Zhongmou
Wang, Xianze
Luo, Zhen
Huo, Mingxin
Wu, Jinghui
Huo, Hongliang
Yang, Wu
author_facet Liu, Zhongmou
Wang, Xianze
Luo, Zhen
Huo, Mingxin
Wu, Jinghui
Huo, Hongliang
Yang, Wu
author_sort Liu, Zhongmou
collection PubMed
description The magnetic graphene oxide (MGO) was successfully synthesised by the in situ chemical co-precipitation method with Fe(3+), Fe(2+) and graphene oxide (GO) in laboratory and, was used as an adsorbent for disinfection by-product (DBP) precursors removing from four natural surface water samples. The results indicate that various DBPs formation significantly decreased by 7–19% to 78–98% for the four samples after MGO treatment and, the treatment process was rapidly reached equilibrium within 20 minutes. The DBP precursors removal efficiency decreased with the increasing pH value from 4 to 10. Hydrophobic compounds (humic acid and fulvic acid) are more sensitive to MGO, whereas hydrophilic and nitrogenous compounds (aromatic proteins) are more insensitive. MGO could be regenerated by using 20% (v/v) ethanol and, the DBP precursors removal efficiency can stay stable after five cycles. These results indicate that MGO can be utilized as a promising adsorbent for the removal of DBP precursors from natural surface water.
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spelling pubmed-46666222015-12-10 Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide Liu, Zhongmou Wang, Xianze Luo, Zhen Huo, Mingxin Wu, Jinghui Huo, Hongliang Yang, Wu PLoS One Research Article The magnetic graphene oxide (MGO) was successfully synthesised by the in situ chemical co-precipitation method with Fe(3+), Fe(2+) and graphene oxide (GO) in laboratory and, was used as an adsorbent for disinfection by-product (DBP) precursors removing from four natural surface water samples. The results indicate that various DBPs formation significantly decreased by 7–19% to 78–98% for the four samples after MGO treatment and, the treatment process was rapidly reached equilibrium within 20 minutes. The DBP precursors removal efficiency decreased with the increasing pH value from 4 to 10. Hydrophobic compounds (humic acid and fulvic acid) are more sensitive to MGO, whereas hydrophilic and nitrogenous compounds (aromatic proteins) are more insensitive. MGO could be regenerated by using 20% (v/v) ethanol and, the DBP precursors removal efficiency can stay stable after five cycles. These results indicate that MGO can be utilized as a promising adsorbent for the removal of DBP precursors from natural surface water. Public Library of Science 2015-12-01 /pmc/articles/PMC4666622/ /pubmed/26623652 http://dx.doi.org/10.1371/journal.pone.0143819 Text en © 2015 Liu et al http://creativecommons.org/licenses/by/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are properly credited.
spellingShingle Research Article
Liu, Zhongmou
Wang, Xianze
Luo, Zhen
Huo, Mingxin
Wu, Jinghui
Huo, Hongliang
Yang, Wu
Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide
title Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide
title_full Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide
title_fullStr Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide
title_full_unstemmed Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide
title_short Removing of Disinfection By-Product Precursors from Surface Water by Using Magnetic Graphene Oxide
title_sort removing of disinfection by-product precursors from surface water by using magnetic graphene oxide
topic Research Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4666622/
https://www.ncbi.nlm.nih.gov/pubmed/26623652
http://dx.doi.org/10.1371/journal.pone.0143819
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