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Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures

The ability to control light-matter interaction is central to several potential applications in lasing, sensing, and communication. Graphene plasmons provide a way of strongly enhancing the interaction and realizing ultrathin optoelectronic devices. Here, we find that photoluminescence (PL) intensit...

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Autores principales: Chen, Yulu, Wu, Qiong, Ma, Yingjie, Liu, Tao, Fan, Yongliang, Yang, Xinju, Zhong, Zhenyang, Xu, Fei, Lu, Jianping, Jiang, Zuimin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4668550/
https://www.ncbi.nlm.nih.gov/pubmed/26631498
http://dx.doi.org/10.1038/srep17688
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author Chen, Yulu
Wu, Qiong
Ma, Yingjie
Liu, Tao
Fan, Yongliang
Yang, Xinju
Zhong, Zhenyang
Xu, Fei
Lu, Jianping
Jiang, Zuimin
author_facet Chen, Yulu
Wu, Qiong
Ma, Yingjie
Liu, Tao
Fan, Yongliang
Yang, Xinju
Zhong, Zhenyang
Xu, Fei
Lu, Jianping
Jiang, Zuimin
author_sort Chen, Yulu
collection PubMed
description The ability to control light-matter interaction is central to several potential applications in lasing, sensing, and communication. Graphene plasmons provide a way of strongly enhancing the interaction and realizing ultrathin optoelectronic devices. Here, we find that photoluminescence (PL) intensities of the graphene/GeSi quantum dots hybrid structures are saturated and quenched under positive and negative voltages at the excitation of 325 nm, respectively. A mechanism called plasmon-gating effect is proposed to reveal the PL dependence of the hybrid structures on the external electric field. On the contrary, the PL intensities at the excitation of 405 and 795 nm of the hybrid structures are quenched due to the charge transfer by tuning the Fermi level of graphene or the blocking of the excitons recombination by excitons separation effect. The results also provide an evidence for the charge transfer mechanism. The plasmon gating effect on the PL provides a new way to control the optical properties of graphene/QD hybrid structures.
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spelling pubmed-46685502015-12-09 Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures Chen, Yulu Wu, Qiong Ma, Yingjie Liu, Tao Fan, Yongliang Yang, Xinju Zhong, Zhenyang Xu, Fei Lu, Jianping Jiang, Zuimin Sci Rep Article The ability to control light-matter interaction is central to several potential applications in lasing, sensing, and communication. Graphene plasmons provide a way of strongly enhancing the interaction and realizing ultrathin optoelectronic devices. Here, we find that photoluminescence (PL) intensities of the graphene/GeSi quantum dots hybrid structures are saturated and quenched under positive and negative voltages at the excitation of 325 nm, respectively. A mechanism called plasmon-gating effect is proposed to reveal the PL dependence of the hybrid structures on the external electric field. On the contrary, the PL intensities at the excitation of 405 and 795 nm of the hybrid structures are quenched due to the charge transfer by tuning the Fermi level of graphene or the blocking of the excitons recombination by excitons separation effect. The results also provide an evidence for the charge transfer mechanism. The plasmon gating effect on the PL provides a new way to control the optical properties of graphene/QD hybrid structures. Nature Publishing Group 2015-12-03 /pmc/articles/PMC4668550/ /pubmed/26631498 http://dx.doi.org/10.1038/srep17688 Text en Copyright © 2015, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Chen, Yulu
Wu, Qiong
Ma, Yingjie
Liu, Tao
Fan, Yongliang
Yang, Xinju
Zhong, Zhenyang
Xu, Fei
Lu, Jianping
Jiang, Zuimin
Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures
title Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures
title_full Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures
title_fullStr Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures
title_full_unstemmed Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures
title_short Plasmon-gating photoluminescence in graphene/GeSi quantum dots hybrid structures
title_sort plasmon-gating photoluminescence in graphene/gesi quantum dots hybrid structures
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4668550/
https://www.ncbi.nlm.nih.gov/pubmed/26631498
http://dx.doi.org/10.1038/srep17688
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