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Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View?

The German government has decided for the nuclear phase out, but a decision on a strategy for the management of the highly radioactive waste is not defined yet. Partitioning and Transmutation (P&T) could be considered as a technological option for the management of highly radioactive waste, ther...

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Autores principales: Merk, Bruno, Litskevich, Dzianis
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Public Library of Science 2015
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4696651/
https://www.ncbi.nlm.nih.gov/pubmed/26717509
http://dx.doi.org/10.1371/journal.pone.0145652
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author Merk, Bruno
Litskevich, Dzianis
author_facet Merk, Bruno
Litskevich, Dzianis
author_sort Merk, Bruno
collection PubMed
description The German government has decided for the nuclear phase out, but a decision on a strategy for the management of the highly radioactive waste is not defined yet. Partitioning and Transmutation (P&T) could be considered as a technological option for the management of highly radioactive waste, therefore a wide study has been conducted. In the study group objectives for P&T and the boundary conditions of the phase out have been discussed. The fulfillment of the given objectives is analyzed from neutronics point of view using simulations of a molten salt reactor with fast neutron spectrum. It is shown that the efficient transmutation of all existing transuranium isotopes would be possible from neutronic point of view in a time frame of about 60 years. For this task three reactors of a mostly new technology would have to be developed and a twofold life cycle consisting of a transmuter operation and a deep burn phase would be required. A basic insight for the optimization of the time duration of the deep burn phase is given. Further on, a detailed balance of different isotopic inventories is given to allow a deeper understanding of the processes during transmutation in the molten salt fast reactor. The effect of modeling and simulation is investigated based on three different modeling strategies and two different code versions.
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spelling pubmed-46966512016-01-13 Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View? Merk, Bruno Litskevich, Dzianis PLoS One Research Article The German government has decided for the nuclear phase out, but a decision on a strategy for the management of the highly radioactive waste is not defined yet. Partitioning and Transmutation (P&T) could be considered as a technological option for the management of highly radioactive waste, therefore a wide study has been conducted. In the study group objectives for P&T and the boundary conditions of the phase out have been discussed. The fulfillment of the given objectives is analyzed from neutronics point of view using simulations of a molten salt reactor with fast neutron spectrum. It is shown that the efficient transmutation of all existing transuranium isotopes would be possible from neutronic point of view in a time frame of about 60 years. For this task three reactors of a mostly new technology would have to be developed and a twofold life cycle consisting of a transmuter operation and a deep burn phase would be required. A basic insight for the optimization of the time duration of the deep burn phase is given. Further on, a detailed balance of different isotopic inventories is given to allow a deeper understanding of the processes during transmutation in the molten salt fast reactor. The effect of modeling and simulation is investigated based on three different modeling strategies and two different code versions. Public Library of Science 2015-12-30 /pmc/articles/PMC4696651/ /pubmed/26717509 http://dx.doi.org/10.1371/journal.pone.0145652 Text en © 2015 Merk, Litskevich http://creativecommons.org/licenses/by/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are properly credited.
spellingShingle Research Article
Merk, Bruno
Litskevich, Dzianis
Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View?
title Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View?
title_full Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View?
title_fullStr Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View?
title_full_unstemmed Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View?
title_short Transmutation of All German Transuranium under Nuclear Phase Out Conditions – Is This Feasible from Neutronic Point of View?
title_sort transmutation of all german transuranium under nuclear phase out conditions – is this feasible from neutronic point of view?
topic Research Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4696651/
https://www.ncbi.nlm.nih.gov/pubmed/26717509
http://dx.doi.org/10.1371/journal.pone.0145652
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