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Centrifugal photovoltaic and photogalvanic effects driven by structured light

Much efforts are devoted to material structuring in a quest to enhance the photovoltaic effect. We show that structuring light in a way it transfers orbital angular momentum to semiconductor-based rings results in a steady charge accumulation at the outer boundaries that can be utilized for the gene...

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Detalles Bibliográficos
Autores principales: Wätzel, J., Berakdar, J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4761893/
https://www.ncbi.nlm.nih.gov/pubmed/26900105
http://dx.doi.org/10.1038/srep21475
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author Wätzel, J.
Berakdar, J.
author_facet Wätzel, J.
Berakdar, J.
author_sort Wätzel, J.
collection PubMed
description Much efforts are devoted to material structuring in a quest to enhance the photovoltaic effect. We show that structuring light in a way it transfers orbital angular momentum to semiconductor-based rings results in a steady charge accumulation at the outer boundaries that can be utilized for the generation of an open circuit voltage or a photogalvanic (bulk photovoltaic) type current. This effect which stems both from structuring light and matter confinement potentials, can be magnified even at fixed moderate intensities, by increasing the orbital angular momentum of light which strengthens the effective centrifugal potential that repels the charge outwards. Based on a full numerical time propagation of the carriers wave functions in the presence of light pulses we demonstrate how the charge buildup leads to a useable voltage or directed photocurrent whose amplitudes and directions are controllable by the light pulse parameters.
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spelling pubmed-47618932016-02-29 Centrifugal photovoltaic and photogalvanic effects driven by structured light Wätzel, J. Berakdar, J. Sci Rep Article Much efforts are devoted to material structuring in a quest to enhance the photovoltaic effect. We show that structuring light in a way it transfers orbital angular momentum to semiconductor-based rings results in a steady charge accumulation at the outer boundaries that can be utilized for the generation of an open circuit voltage or a photogalvanic (bulk photovoltaic) type current. This effect which stems both from structuring light and matter confinement potentials, can be magnified even at fixed moderate intensities, by increasing the orbital angular momentum of light which strengthens the effective centrifugal potential that repels the charge outwards. Based on a full numerical time propagation of the carriers wave functions in the presence of light pulses we demonstrate how the charge buildup leads to a useable voltage or directed photocurrent whose amplitudes and directions are controllable by the light pulse parameters. Nature Publishing Group 2016-02-22 /pmc/articles/PMC4761893/ /pubmed/26900105 http://dx.doi.org/10.1038/srep21475 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Wätzel, J.
Berakdar, J.
Centrifugal photovoltaic and photogalvanic effects driven by structured light
title Centrifugal photovoltaic and photogalvanic effects driven by structured light
title_full Centrifugal photovoltaic and photogalvanic effects driven by structured light
title_fullStr Centrifugal photovoltaic and photogalvanic effects driven by structured light
title_full_unstemmed Centrifugal photovoltaic and photogalvanic effects driven by structured light
title_short Centrifugal photovoltaic and photogalvanic effects driven by structured light
title_sort centrifugal photovoltaic and photogalvanic effects driven by structured light
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4761893/
https://www.ncbi.nlm.nih.gov/pubmed/26900105
http://dx.doi.org/10.1038/srep21475
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