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Origin of uranium isotope variations in early solar nebula condensates

High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) =...

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Detalles Bibliográficos
Autores principales: Tissot, François L. H., Dauphas, Nicolas, Grossman, Lawrence
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4783122/
https://www.ncbi.nlm.nih.gov/pubmed/26973874
http://dx.doi.org/10.1126/sciadv.1501400
Descripción
Sumario:High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) = 15.6 My) into (235)U, but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of (235)U reaching ~+6% relative to average solar system composition, which can only be due to the decay of (247)Cm. This allows us to constrain the (247)Cm/(235)U ratio at solar system formation to (1.1 ± 0.3) × 10(−4). This value provides new clues on the universality of the nucleosynthetic r-process of rapid neutron capture.